Unveiling the Proton‐Feeding Effect in Sulfur‐Doped Fe−N−C Single‐Atom Catalyst for Enhanced CO2 Electroreduction

Heteroatom‐doping in metal‐nitrogen‐carbon single‐atom catalysts (SACs) is considered a powerful strategy to promote the electrocatalytic CO2 reduction reaction (CO2RR), but the origin of enhanced catalytic activity is still elusive. Here, we disclose that sulfur doping induces an obvious proton‐fee...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 61; H. 32; S. e202206233 - n/a
Hauptverfasser:	Chen, Shanyong, Li, Xiaoqing, Kao, Cheng‐Wei, Luo, Tao, Chen, Kejun, Fu, Junwei, Ma, Chao, Li, Hongmei, Li, Ming, Chan, Ting‐Shan, Liu, Min
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 08.08.2022
Ausgabe:	International ed. in English
Schlagworte:	Absorption spectroscopy Carbon dioxide Catalysts Catalytic activity Chemical reduction CO2 Electroreduction Doping Heteroatom Doping Proton-Feeding Effect Protons Reaction Kinetics Scanning transmission electron microscopy Single atom catalysts Sulfur Transmission electron microscopy CO2 electroreduction single-atom catalyst proton-feeding effect Heteroatom doping Reaction kinetics
ISSN:	1433-7851, 1521-3773, 1521-3773
Online-Zugang:	Volltext
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