Enhancing C─C Bond Cleavage of Glycerol Electrooxidation Through Spin‐Selective Electron Donation in Pd–PdS2–Cox Heterostructural Nanosheets

As a 4d transition metal, the spin state of Pd is extremely difficult to directly regulate for the optimized d orbital states owing to the strong spin‐orbit coupling effect and further extended d orbital. Herein, we devise a “spin‐selective electron donation” strategy to tune specific d orbital elec...

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Vydané v:	Angewandte Chemie International Edition Ročník 64; číslo 27; s. e202506032 - n/a
Hlavní autori:	Liu, Pei, Ma, Hao, Qin, Yuchen, Li, Junjun, Li, Fengwang, Ye, Jinyu, Guo, Qiudi, Su, Ning, Gao, Chao, Xie, Lixia, Sheng, Xia, Zhao, Shiju, Jiang, Guangce, Ren, Yunlai, Sun, Yuanmiao, Zhang, Zhicheng
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Weinheim Wiley Subscription Services, Inc 01.07.2025
Vydanie:	International ed. in English
Predmet:	Alcohols Carbon dioxide Chemical bonds Chemical reduction Cleavage Cobalt Coupling C─C bond cleavage Electricity consumption Electron spin Electrons Ethanol Ethylene glycol Formic acid Glycerol Glycerol oxidation reaction Low voltage Orbitals Oxidation Palladium Pd–PdS2–Co heterostructural nanosheets Spin state regulation Spin‐selective electron donation Transition metals
ISSN:	1433-7851, 1521-3773, 1521-3773
On-line prístup:	Získať plný text
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