Enhancing C─C Bond Cleavage of Glycerol Electrooxidation Through Spin‐Selective Electron Donation in Pd–PdS2–Cox Heterostructural Nanosheets

As a 4d transition metal, the spin state of Pd is extremely difficult to directly regulate for the optimized d orbital states owing to the strong spin‐orbit coupling effect and further extended d orbital. Herein, we devise a “spin‐selective electron donation” strategy to tune specific d orbital elec...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 64; H. 27; S. e202506032 - n/a
Hauptverfasser:	Liu, Pei, Ma, Hao, Qin, Yuchen, Li, Junjun, Li, Fengwang, Ye, Jinyu, Guo, Qiudi, Su, Ning, Gao, Chao, Xie, Lixia, Sheng, Xia, Zhao, Shiju, Jiang, Guangce, Ren, Yunlai, Sun, Yuanmiao, Zhang, Zhicheng
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Weinheim Wiley Subscription Services, Inc 01.07.2025
Ausgabe:	International ed. in English
Schlagworte:	Alcohols Carbon dioxide Chemical bonds Chemical reduction Cleavage Cobalt Coupling C─C bond cleavage Electricity consumption Electron spin Electrons Ethanol Ethylene glycol Formic acid Glycerol Glycerol oxidation reaction Low voltage Orbitals Oxidation Palladium Pd–PdS2–Co heterostructural nanosheets Spin state regulation Spin‐selective electron donation Transition metals
ISSN:	1433-7851, 1521-3773, 1521-3773
Online-Zugang:	Volltext
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