Deciphering the Role of Anions and Secondary Coordination Sphere in Tuning Anisotropy in Dy(III) Air‐Stable D5h SIMs

Precise control of the crystal field and symmetry around the paramagnetic spin centre has recently facilitated the engineering of high‐temperature single‐ion magnets (SIMs), the smallest possible units for future spin‐based devices. In the present work, we report a series of air‐stable seven coordin...

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