Molecular docking and simulation studies on SARS-CoV-2 Mpro reveals Mitoxantrone, Leucovorin, Birinapant, and Dynasore as potent drugs against COVID-19

The outbreak of novel coronavirus (COVID-19), which began from Wuhan City, Hubei, China, and declared as a Public Health Emergency of International Concern by World Health Organization (WHO) on 30 th January 2020. The present study describes how the available drug candidates can be used as a potenti...

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Published in:Journal of biomolecular structure & dynamics Vol. 39; no. 18; pp. 7294 - 7305
Main Authors: Lokhande, Kiran Bharat, Doiphode, Sayali, Vyas, Renu, Swamy, K. Venkateswara
Format: Journal Article
Language:English
Published: Taylor & Francis 12.12.2021
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ISSN:0739-1102, 1538-0254, 1538-0254
Online Access:Get full text
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Summary:The outbreak of novel coronavirus (COVID-19), which began from Wuhan City, Hubei, China, and declared as a Public Health Emergency of International Concern by World Health Organization (WHO) on 30 th January 2020. The present study describes how the available drug candidates can be used as a potential SARS-CoV-2 M pro inhibitor by molecular docking and molecular dynamic simulation studies. Drug repurposing strategy is applied by using the library of antiviral and FDA approved drugs retrieved from the Selleckchem Inc. (Houston, TX, http://www.selleckchem.com ) and DrugBank database respectively. Computational methods like molecular docking and molecular dynamics simulation were used. The molecular docking calculations were performed using LeadIT FlexX software. The molecular dynamics simulations of 100 ns were performed to study conformational stability for all complex systems. Mitoxantrone and Leucovorin from FDA approved drug library and Birinapant and Dynasore from anti-viral drug libraries interact with SARS-CoV-2 M pro at higher efficiency as a result of the improved steric and hydrophobic environment in the binding cavity to make stable complex. Also, the molecular dynamics simulations of 100 ns revealed the mean RMSD value of 2.25 Å for all the complex systems. This shows that lead compounds bound tightly within the M pro cavity and thus having conformational stability. Glutamic acid (Glu166) of M pro is a key residue to hold and form a stable complex of reported lead compounds by forming hydrogen bonds and salt bridge. Our findings suggest that Mitoxantrone, Leucovorin, Birinapant, and Dynasore represents potential inhibitors of SARS-CoV-2 M pro . Communicated by Ramaswamy H. Sarma
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Communicated by Ramaswamy H. Sarma
Supplemental data for this article can be accessed online at https://doi.org/10.1080/07391102.2020.1805019.
ISSN:0739-1102
1538-0254
1538-0254
DOI:10.1080/07391102.2020.1805019