Defect-Engineered Metal-Organic Frameworks

Defect engineering in metal–organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical...

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Published in:	Angewandte Chemie International Edition Vol. 54; no. 25; pp. 7234 - 7254
Main Authors:	Fang, Zhenlan, Bueken, Bart, De Vos, Dirk E., Fischer, Roland A.
Format:	Journal Article
Language:	English
Published:	Weinheim WILEY-VCH Verlag 15.06.2015 WILEY‐VCH Verlag Wiley Subscription Services, Inc
Edition:	International ed. in English
Subjects:	Catalysis Classification Computer numerical control coordination chemistry Crystal defects Crystal structure Defects defects engineering Electrically conductive heterogeneity Metal-organic frameworks Networks Physical properties porous materials Review Zeolites porous materials coordination chemistry heterogeneity defects engineering metal-organic frameworks
ISSN:	1433-7851, 1521-3773, 1521-3773
Online Access:	Get full text
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Abstract	Defect engineering in metal–organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of “defect‐engineering” concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect‐engineered CNCs. Designer defects: Defects in coordination network compounds (CNCs) are defined as “sites that locally break the regular periodic arrangement of atoms or ions of the static crystalline parent framework due to missing or incorrectly dislocated atoms or ions”. This Review provides both a concise overview of defects in CNCs (including their classification and characterizations) and applications of defective CNCs/MOFs.
AbstractList	Defect engineering in metal-organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of "defect-engineering" concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect-engineered CNCs. Defect engineering in metal-organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of "defect-engineering" concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect-engineered CNCs.Defect engineering in metal-organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of "defect-engineering" concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect-engineered CNCs. Defect engineering in metal-organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of "defect-engineering" concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect-engineered CNCs. Designer defects: Defects in coordination network compounds (CNCs) are defined as "sites that locally break the regular periodic arrangement of atoms or ions of the static crystalline parent framework due to missing or incorrectly dislocated atoms or ions". This Review provides both a concise overview of defects in CNCs (including their classification and characterizations) and applications of defective CNCs/MOFs. Defect engineering in metal–organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of “defect‐engineering” concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect‐engineered CNCs. Designer defects: Defects in coordination network compounds (CNCs) are defined as “sites that locally break the regular periodic arrangement of atoms or ions of the static crystalline parent framework due to missing or incorrectly dislocated atoms or ions”. This Review provides both a concise overview of defects in CNCs (including their classification and characterizations) and applications of defective CNCs/MOFs.
Author	De Vos, Dirk E. Fischer, Roland A. Fang, Zhenlan Bueken, Bart
Author_xml	– sequence: 1 givenname: Zhenlan surname: Fang fullname: Fang, Zhenlan email: iamzlfang@njtech.edu.cn organization: Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (NanjingTech), 30 South Puzhu Road, Nanjing 211816 (V.R. China) – sequence: 2 givenname: Bart surname: Bueken fullname: Bueken, Bart email: bart.bueken@biw.kuleuven.be organization: Centre for Surface Chemistry and Catalysis, KULeuven, Kasteelpark Arenberg 23, 3001 Leuven (Belgien) – sequence: 3 givenname: Dirk E. surname: De Vos fullname: De Vos, Dirk E. email: dirk.devos@biw.kuleuven.be organization: Centre for Surface Chemistry and Catalysis, KULeuven, Kasteelpark Arenberg 23, 3001 Leuven (Belgien) – sequence: 4 givenname: Roland A. surname: Fischer fullname: Fischer, Roland A. email: roland.fischer@rub.de organization: Inorganic Chemistry II-Organometallics & Material Chemistry, Department of Chemistry and Biochemistry, Ruhr-University Bochum, Universitätsstrasse 150, 44801 Bochum (Germany)
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Snippet	Defect engineering in metal–organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in... Defect engineering in metal-organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in...
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SubjectTerms	Catalysis Classification Computer numerical control coordination chemistry Crystal defects Crystal structure Defects defects engineering Electrically conductive heterogeneity Metal-organic frameworks Networks Physical properties porous materials Review Zeolites
Title	Defect-Engineered Metal-Organic Frameworks
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