Ionic Conduction in Polymer‐Based Solid Electrolytes

Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, a...

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Vydané v:Advanced science Ročník 10; číslo 10; s. e2201718 - n/a
Hlavní autori: Li, Zhuo, Fu, Jialong, Zhou, Xiaoyan, Gui, Siwei, Wei, Lu, Yang, Hui, Li, Hong, Guo, Xin
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: Germany John Wiley & Sons, Inc 01.04.2023
John Wiley and Sons Inc
Wiley
Predmet:
composite polymer electrolyte
Conductivity
Electrolytes
Energy
interfacial interaction
ionic conduction
Ions
Lithium
Oxygen
polymer electrolyte
Polymers
Review
Reviews
solid‐state batteries
composite polymer electrolyte
interfacial interaction
solid-state batteries
ionic conduction
polymer electrolyte
ISSN:2198-3844, 2198-3844
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Abstract Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer‐based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li‐ion conductivity of polymer‐based solid electrolytes. This article reviews the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted.
AbstractList Good safety, high interfacial compatibility, low cost, and facile processability make polymer-based solid electrolytes promising materials for next-generation batteries. Key issues related to polymer-based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer-based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer-based solid electrolytes, including solvent-free polymer electrolytes, composite polymer electrolytes, and quasi-solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion-pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li-ion conductivity of polymer-based solid electrolytes.Good safety, high interfacial compatibility, low cost, and facile processability make polymer-based solid electrolytes promising materials for next-generation batteries. Key issues related to polymer-based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer-based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer-based solid electrolytes, including solvent-free polymer electrolytes, composite polymer electrolytes, and quasi-solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion-pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li-ion conductivity of polymer-based solid electrolytes.
Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer‐based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li‐ion conductivity of polymer‐based solid electrolytes. This article reviews the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted.
Good safety, high interfacial compatibility, low cost, and facile processability make polymer-based solid electrolytes promising materials for next-generation batteries. Key issues related to polymer-based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer-based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer-based solid electrolytes, including solvent-free polymer electrolytes, composite polymer electrolytes, and quasi-solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion-pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li-ion conductivity of polymer-based solid electrolytes.
Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer‐based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li‐ion conductivity of polymer‐based solid electrolytes. This article reviews the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted.
Abstract Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer‐based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li‐ion conductivity of polymer‐based solid electrolytes.
Author Li, Zhuo
Li, Hong
Zhou, Xiaoyan
Gui, Siwei
Guo, Xin
Wei, Lu
Fu, Jialong
Yang, Hui
AuthorAffiliation 2 Department of Mechanics School of Aerospace Engineering Huazhong University of Science and Technology Wuhan 430074 P.R. China
3 Institute of Physics Chinese Academy of Sciences Beijing 100190 P.R. China
1 School of Materials Science and Engineering State Key Laboratory of Material Processing and Die & Mould Technology Huazhong University of Science and Technology Wuhan 430074 P.R. China
AuthorAffiliation_xml – name: 1 School of Materials Science and Engineering State Key Laboratory of Material Processing and Die & Mould Technology Huazhong University of Science and Technology Wuhan 430074 P.R. China
– name: 2 Department of Mechanics School of Aerospace Engineering Huazhong University of Science and Technology Wuhan 430074 P.R. China
– name: 3 Institute of Physics Chinese Academy of Sciences Beijing 100190 P.R. China
Author_xml – sequence: 1
  givenname: Zhuo
  surname: Li
  fullname: Li, Zhuo
  organization: Huazhong University of Science and Technology
– sequence: 2
  givenname: Jialong
  surname: Fu
  fullname: Fu, Jialong
  organization: Huazhong University of Science and Technology
– sequence: 3
  givenname: Xiaoyan
  surname: Zhou
  fullname: Zhou, Xiaoyan
  organization: Huazhong University of Science and Technology
– sequence: 4
  givenname: Siwei
  surname: Gui
  fullname: Gui, Siwei
  organization: Huazhong University of Science and Technology
– sequence: 5
  givenname: Lu
  surname: Wei
  fullname: Wei, Lu
  organization: Huazhong University of Science and Technology
– sequence: 6
  givenname: Hui
  surname: Yang
  fullname: Yang, Hui
  organization: Huazhong University of Science and Technology
– sequence: 7
  givenname: Hong
  surname: Li
  fullname: Li, Hong
  organization: Chinese Academy of Sciences
– sequence: 8
  givenname: Xin
  orcidid: 0000-0003-1546-8119
  surname: Guo
  fullname: Guo, Xin
  email: xguo@hust.edu.cn
  organization: Huazhong University of Science and Technology
BackLink https://www.ncbi.nlm.nih.gov/pubmed/36698303$$D View this record in MEDLINE/PubMed
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Keywords composite polymer electrolyte
interfacial interaction
solid-state batteries
ionic conduction
polymer electrolyte
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Snippet Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation...
Good safety, high interfacial compatibility, low cost, and facile processability make polymer-based solid electrolytes promising materials for next-generation...
Abstract Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for...
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SubjectTerms composite polymer electrolyte
Conductivity
Electrolytes
Energy
interfacial interaction
ionic conduction
Ions
Lithium
Oxygen
polymer electrolyte
Polymers
Review
Reviews
solid‐state batteries
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Title Ionic Conduction in Polymer‐Based Solid Electrolytes
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