Electronic structure of the parent compound of superconducting infinite-layer nickelates

The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors 1 – 10 . The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO 2 (refs. 11 , 12 ) has strengthened these efforts. Here, we use X-ray sp...

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Published in:	Nature materials Vol. 19; no. 4; pp. 381 - 385
Main Authors:	Hepting, M., Li, D., Jia, C. J., Lu, H., Paris, E., Tseng, Y., Feng, X., Osada, M., Been, E., Hikita, Y., Chuang, Y.-D., Hussain, Z., Zhou, K. J., Nag, A., Garcia-Fernandez, M., Rossi, M., Huang, H. Y., Huang, D. J., Shen, Z. X., Schmitt, T., Hwang, H. Y., Moritz, B., Zaanen, J., Devereaux, T. P., Lee, W. S.
Format:	Journal Article
Language:	English
Published:	London Nature Publishing Group UK 01.04.2020 Nature Publishing Group Springer Nature - Nature Publishing Group
Subjects:	639/301 639/766 Biomaterials Chemistry and Materials Science Condensed Matter Physics CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Copper compounds Cuprates Density functional theory Earth Electronic properties Electronic structure Electrons Fermions High temperature High temperature superconductors Letter Materials Science Nanotechnology Nickel Optical and Electronic Materials Physics Rare earth elements Spectrum analysis Superconductivity X-ray spectroscopy
ISSN:	1476-1122, 1476-4660, 1476-4660
Online Access:	Get full text
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Abstract	The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors 1 – 10 . The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO 2 (refs. 11 , 12 ) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO 2 and NdNiO 2 , while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5 d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with 3 d x 2 − y 2 symmetry in the NiO 2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics 13 – 15 , which are well known for heavy fermion behaviour, where the NiO 2 correlated layers play an analogous role to the 4 f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like ‘oxide-intermetallic’ replaces the Mott insulator as the reference state from which superconductivity emerges upon doping. X-ray spectroscopy and density functional theory are used to show that the electronic structure of the parent compound of superconducting infinite-layer nickelates, while similar to the copper-based high-temperature superconductors, has significant differences.
AbstractList	The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors . The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO (refs. ) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO and NdNiO , while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with [Formula: see text] symmetry in the NiO layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics , which are well known for heavy fermion behaviour, where the NiO correlated layers play an analogous role to the 4f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like 'oxide-intermetallic' replaces the Mott insulator as the reference state from which superconductivity emerges upon doping. The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1-10. The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO2 (refs. 11,12) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO2 and NdNiO2, while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with [Formula: see text] symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics13-15, which are well known for heavy fermion behaviour, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like 'oxide-intermetallic' replaces the Mott insulator as the reference state from which superconductivity emerges upon doping.The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1-10. The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO2 (refs. 11,12) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO2 and NdNiO2, while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with [Formula: see text] symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics13-15, which are well known for heavy fermion behaviour, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like 'oxide-intermetallic' replaces the Mott insulator as the reference state from which superconductivity emerges upon doping. The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1–10. The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO2 (refs. 11,12) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO2 and NdNiO2, while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with 3dx2−y2 symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics13–15, which are well known for heavy fermion behaviour, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like ‘oxide-intermetallic’ replaces the Mott insulator as the reference state from which superconductivity emerges upon doping.X-ray spectroscopy and density functional theory are used to show that the electronic structure of the parent compound of superconducting infinite-layer nickelates, while similar to the copper-based high-temperature superconductors, has significant differences. The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors 1 – 10 . The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO 2 (refs. 11 , 12 ) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO 2 and NdNiO 2 , while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5 d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with 3 d x 2 − y 2 symmetry in the NiO 2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics 13 – 15 , which are well known for heavy fermion behaviour, where the NiO 2 correlated layers play an analogous role to the 4 f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like ‘oxide-intermetallic’ replaces the Mott insulator as the reference state from which superconductivity emerges upon doping. X-ray spectroscopy and density functional theory are used to show that the electronic structure of the parent compound of superconducting infinite-layer nickelates, while similar to the copper-based high-temperature superconductors, has significant differences. The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1-10. The recent discovery of superconductivity in the doped infinite-layer nickelate NdNiO2 (refs. 11,12) has strengthened these efforts. Here, we use X-ray spectroscopy and density functional theory to show that the electronic structure of LaNiO2 and NdNiO2, while similar to the cuprates, includes significant distinctions. Unlike cuprates, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly interacting three-dimensional 5d metallic state, which hybridizes with a quasi-two-dimensional, strongly correlated state with [Formula: see text] symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare-earth intermetallics13-15, which are well known for heavy fermion behaviour, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy fermion compounds. This Kondo- or Anderson-lattice-like 'oxide-intermetallic' replaces the Mott insulator as the reference state from which superconductivity emerges upon doping.
Author	Hwang, H. Y. Huang, H. Y. Zhou, K. J. Zaanen, J. Jia, C. J. Lee, W. S. Rossi, M. Been, E. Nag, A. Garcia-Fernandez, M. Osada, M. Shen, Z. X. Huang, D. J. Moritz, B. Tseng, Y. Hussain, Z. Schmitt, T. Devereaux, T. P. Lu, H. Li, D. Hikita, Y. Paris, E. Chuang, Y.-D. Hepting, M. Feng, X.
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BackLink	https://www.ncbi.nlm.nih.gov/pubmed/31959951$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1605376$$D View this record in Osti.gov
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ContentType	Journal Article
Copyright	The Author(s), under exclusive licence to Springer Nature Limited 2020 The Author(s), under exclusive licence to Springer Nature Limited 2020.
Copyright_xml	– notice: The Author(s), under exclusive licence to Springer Nature Limited 2020 – notice: The Author(s), under exclusive licence to Springer Nature Limited 2020.
CorporateAuthor	SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States) Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
CorporateAuthor_xml	– name: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS) – name: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
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Snippet	The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors 1 – 10 . The recent... The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors . The recent discovery of... The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1–10. The recent discovery... The search continues for nickel oxide-based materials with electronic properties similar to cuprate high-temperature superconductors1-10. The recent discovery...
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SubjectTerms	639/301 639/766 Biomaterials Chemistry and Materials Science Condensed Matter Physics CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Copper compounds Cuprates Density functional theory Earth Electronic properties Electronic structure Electrons Fermions High temperature High temperature superconductors Letter Materials Science Nanotechnology Nickel Optical and Electronic Materials Physics Rare earth elements Spectrum analysis Superconductivity X-ray spectroscopy
Title	Electronic structure of the parent compound of superconducting infinite-layer nickelates
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