Multi-level parallelization of quantum-chemical calculations

Strategies for multiple-level parallelizations of quantum-mechanical calculations are discussed, with an emphasis on using groups of workers for performing parallel tasks. These parallel programming models can be used for a variety ab initio quantum chemistry approaches, including the fragment molec...

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Vydané v:The Journal of chemical physics Ročník 158; číslo 16
Hlavní autori: Fedorov, Dmitri G, Pham, Buu Q
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: United States 28.04.2023
ISSN:1089-7690, 1089-7690
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Shrnutí:Strategies for multiple-level parallelizations of quantum-mechanical calculations are discussed, with an emphasis on using groups of workers for performing parallel tasks. These parallel programming models can be used for a variety ab initio quantum chemistry approaches, including the fragment molecular orbital method and replica-exchange molecular dynamics. Strategies for efficient load balancing on problems of increasing granularity are introduced and discussed. A four-level parallelization is developed based on a multi-level hierarchical grouping, and a high parallel efficiency is achieved on the Theta supercomputer using 131 072 OpenMP threads.
Bibliografia:ObjectType-Article-1
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ISSN:1089-7690
1089-7690
DOI:10.1063/5.0144917