Local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys investigated by EXAFS method

▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition. We report on extended X-ray absorption fine structure (EXAFS) study of...

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Published in:Journal of alloys and compounds Vol. 509; pp. S34 - S37
Main Authors: Antonowicz, J., Pietnoczka, A., Zalewski, W., Bacewicz, R., Stoica, M., Georgarakis, K., Yavari, A.R.
Format: Journal Article
Language:English
Published: Elsevier B.V 01.06.2011
Elsevier
Subjects:
Alloys
Amorphous alloys
Amorphous materials
AMORPHOUS STRUCTURE
Atomic scale structure
Atomic structure
Chemical Sciences
Deviation
EXAFS
FITTINGS
Material chemistry
Metallic glasses
MOLECULAR STRUCTURE
QUENCHING MECHANISMS
Zirconium
ZIRCONIUM ALLOYS (50 TO 99 ZR)
Zirconium base alloys
ZIRCONIUM COPPERS
Atomic scale structure
Metallic glasses
Amorphous materials
EXAFS
ISSN:0925-8388, 1873-4669
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Abstract ▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition. We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr–Cu and Zr–Cu–Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr–Cu alloys.
AbstractList We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr-Cu and Zr-Cu-Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr-Cu alloys.
▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition. We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr–Cu and Zr–Cu–Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr–Cu alloys.
We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr-Cu and Zr-Cu-Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr-Cu alloys. (C) 2010 Elsevier B.V. All rights reserved
Author Stoica, M.
Zalewski, W.
Georgarakis, K.
Pietnoczka, A.
Bacewicz, R.
Yavari, A.R.
Antonowicz, J.
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  surname: Antonowicz
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  surname: Zalewski
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  organization: Faculty of Physics, Warsaw University of Technology, Koszykowa 75, 00-662 Warsaw, Poland
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  surname: Georgarakis
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  organization: SIMAP-LTPCM, Institut National Polytechnique de Grenoble, BP 75, 38402 St-Martin-d’Heres Campus, France
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  givenname: A.R.
  surname: Yavari
  fullname: Yavari, A.R.
  organization: SIMAP-LTPCM, Institut National Polytechnique de Grenoble, BP 75, 38402 St-Martin-d’Heres Campus, France
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Keywords Atomic scale structure
Metallic glasses
Amorphous materials
EXAFS
Language English
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Snippet ▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic...
We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and...
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SubjectTerms Alloys
Amorphous alloys
Amorphous materials
AMORPHOUS STRUCTURE
Atomic scale structure
Atomic structure
Chemical Sciences
Deviation
EXAFS
FITTINGS
Material chemistry
Metallic glasses
MOLECULAR STRUCTURE
QUENCHING MECHANISMS
Zirconium
ZIRCONIUM ALLOYS (50 TO 99 ZR)
Zirconium base alloys
ZIRCONIUM COPPERS
Title Local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys investigated by EXAFS method
URI https://dx.doi.org/10.1016/j.jallcom.2010.10.105
https://www.proquest.com/docview/896230543
https://hal.science/hal-00640045
Volume 509
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