Local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys investigated by EXAFS method
▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition. We report on extended X-ray absorption fine structure (EXAFS) study of...
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| Published in: | Journal of alloys and compounds Vol. 509; pp. S34 - S37 |
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| Language: | English |
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Elsevier B.V
01.06.2011
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| ISSN: | 0925-8388, 1873-4669 |
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| Abstract | ▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition.
We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr–Cu and Zr–Cu–Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr–Cu alloys. |
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| AbstractList | ▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic structure. ▶ Deviation from random mixing behavior resulting from Al addition.
We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr–Cu and Zr–Cu–Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr–Cu alloys. We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr-Cu and Zr-Cu-Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr-Cu alloys. (C) 2010 Elsevier B.V. All rights reserved We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and Cu atoms was investigated. From the EXAFS data fitting the values of coordination number, interatomic distances and mean square atomic displacement were obtained for wide range of compositions. It was found that icosahedral symmetry rather than that of corresponding crystalline analogs dominates in the local atomic structure of Zr-Cu and Zr-Cu-Al amorphous alloys. Judging from bonding preferences we conclude that addition of Al as an alloying element results in considerable deviation from random mixing behavior observed in binary Zr-Cu alloys. |
| Author | Stoica, M. Zalewski, W. Georgarakis, K. Pietnoczka, A. Bacewicz, R. Yavari, A.R. Antonowicz, J. |
| Author_xml | – sequence: 1 givenname: J. surname: Antonowicz fullname: Antonowicz, J. email: antonowi@if.pw.edu.pl organization: Faculty of Physics, Warsaw University of Technology, Koszykowa 75, 00-662 Warsaw, Poland – sequence: 2 givenname: A. surname: Pietnoczka fullname: Pietnoczka, A. organization: Faculty of Physics, Warsaw University of Technology, Koszykowa 75, 00-662 Warsaw, Poland – sequence: 3 givenname: W. surname: Zalewski fullname: Zalewski, W. organization: Faculty of Physics, Warsaw University of Technology, Koszykowa 75, 00-662 Warsaw, Poland – sequence: 4 givenname: R. surname: Bacewicz fullname: Bacewicz, R. organization: Faculty of Physics, Warsaw University of Technology, Koszykowa 75, 00-662 Warsaw, Poland – sequence: 5 givenname: M. surname: Stoica fullname: Stoica, M. organization: IFW Dresden, Institute for Complex Materials, P.O. Box 270116, D-01171 Dresden, Germany – sequence: 6 givenname: K. surname: Georgarakis fullname: Georgarakis, K. organization: SIMAP-LTPCM, Institut National Polytechnique de Grenoble, BP 75, 38402 St-Martin-d’Heres Campus, France – sequence: 7 givenname: A.R. surname: Yavari fullname: Yavari, A.R. organization: SIMAP-LTPCM, Institut National Polytechnique de Grenoble, BP 75, 38402 St-Martin-d’Heres Campus, France |
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| Cites_doi | 10.1016/j.intermet.2006.01.006 10.1016/j.jallcom.2009.05.111 10.1103/PhysRevB.58.7565 10.4028/www.scientific.net/MSF.539-543.1959 10.1063/1.3136428 10.1016/j.jallcom.2008.03.092 10.1016/j.jnoncrysol.2005.03.012 10.1103/PhysRevB.71.224208 10.1016/j.msea.2006.02.334 10.1016/j.scriptamat.2007.02.013 10.1016/j.jallcom.2006.08.141 10.1063/1.1626266 10.1063/1.2009827 10.1103/PhysRevLett.102.245501 10.1063/1.2816912 10.1016/j.scriptamat.2009.09.019 10.2320/matertrans.45.584 10.1088/0022-3727/34/2/309 10.1016/j.jallcom.2008.07.211 10.1016/j.jallcom.2008.01.037 10.1063/1.2828694 10.1002/pssa.2210510235 10.1107/S0909049505012719 10.1016/0022-3093(84)90359-4 10.1016/j.scriptamat.2005.11.033 10.2320/matertrans.46.2893 10.1080/1478643031000098828 |
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| Keywords | Atomic scale structure Metallic glasses Amorphous materials EXAFS |
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| Snippet | ▶ Coordination number, interatomic distances and mean square atomic displacement in Zr–Cu and Zr–Cu–Al glasses. ▶ Icosahedral symmetry in local atomic... We report on extended X-ray absorption fine structure (EXAFS) study of rapidly quenched Zr-Cu and Zr-Cu-Al glassy alloys. The local atomic order around Zr and... |
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| SubjectTerms | Alloys Amorphous alloys Amorphous materials AMORPHOUS STRUCTURE Atomic scale structure Atomic structure Chemical Sciences Deviation EXAFS FITTINGS Material chemistry Metallic glasses MOLECULAR STRUCTURE QUENCHING MECHANISMS Zirconium ZIRCONIUM ALLOYS (50 TO 99 ZR) Zirconium base alloys ZIRCONIUM COPPERS |
| Title | Local atomic structure of Zr–Cu and Zr–Cu–Al amorphous alloys investigated by EXAFS method |
| URI | https://dx.doi.org/10.1016/j.jallcom.2010.10.105 https://www.proquest.com/docview/896230543 https://hal.science/hal-00640045 |
| Volume | 509 |
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