SHAKE, rattle, and roll: Efficient constraint algorithms for linked rigid bodies

We present an iterative constraint algorithm, QSHAKE, for use with semirigid molecules in molecular dynamics simulations. The algorithm is based on “SHAKE‐ing” bond constraints between rigid bodies, whose equations of motion are solved in the quaternion framework. The algorithm is derived and its pe...

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Vydáno v:Journal of computational chemistry Ročník 19; číslo 1; s. 102 - 111
Hlavní autoři: Forester, Timothy R., Smith, William
Médium: Journal Article
Jazyk:angličtina
Vydáno: New York John Wiley & Sons, Inc 15.01.1998
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ISSN:0192-8651, 1096-987X
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Abstract We present an iterative constraint algorithm, QSHAKE, for use with semirigid molecules in molecular dynamics simulations. The algorithm is based on “SHAKE‐ing” bond constraints between rigid bodies, whose equations of motion are solved in the quaternion framework. The algorithm is derived and its performance compared with SHAKE for liquid octane. QSHAKE is significantly more efficient whenever SHAKE requires triangles (or tetrahedra) of constraints to maintain molecular shape. Efficiencies are gained because QSHAKE reduces the number of holonomic constraints that must be solved iteratively and requires fewer iterations to obtain convergence. The gains in efficiency are most noticeable when a high degree of precision is imposed on the constraint criteria. QSHAKE is also stable at larger time steps than SHAKE, thus allowing for even more efficient exploration of phase space for semirigid molecules. © 1998 John Wiley & Sons, Inc. J Comput Chem 19: 102–111, 1998
AbstractList We present an iterative constraint algorithm, QSHAKE, for use with semirigid molecules in molecular dynamics simulations. The algorithm is based on “SHAKE‐ing” bond constraints between rigid bodies, whose equations of motion are solved in the quaternion framework. The algorithm is derived and its performance compared with SHAKE for liquid octane. QSHAKE is significantly more efficient whenever SHAKE requires triangles (or tetrahedra) of constraints to maintain molecular shape. Efficiencies are gained because QSHAKE reduces the number of holonomic constraints that must be solved iteratively and requires fewer iterations to obtain convergence. The gains in efficiency are most noticeable when a high degree of precision is imposed on the constraint criteria. QSHAKE is also stable at larger time steps than SHAKE, thus allowing for even more efficient exploration of phase space for semirigid molecules. © 1998 John Wiley & Sons, Inc. J Comput Chem 19: 102–111, 1998
Author Forester, Timothy R.
Smith, William
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Cites_doi 10.1103/PhysRevA.7.1092
10.1016/0021-9991(83)90014-1
10.1103/PhysRevE.50.1559
10.1016/0021-9991(77)90098-5
10.1016/S0263-7855(96)00043-4
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SubjectTerms bond constraints
molecular dynamics simulations
QSHAKE
semirigid molecules
Title SHAKE, rattle, and roll: Efficient constraint algorithms for linked rigid bodies
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