Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance

Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh‐pe...

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Published in:Advanced materials (Weinheim) Vol. 31; no. 14; pp. e1807071 - n/a
Main Authors: Hong, Min, Zou, Jin, Chen, Zhi‐Gang
Format: Journal Article
Language:English
Published: Germany Wiley Subscription Services, Inc 05.04.2019
Subjects:
Banded structure
Carrier density
Cooling
Crystal structure
Degrees of freedom
GeTe thermoelectrics
Materials science
multiple valence bands
Phase transitions
phonon scatterings
Phonons
resonant bonding
Spacecraft
Thermal conductivity
Thermoelectric materials
Transport properties
phonon scatterings
phase transitions
GeTe thermoelectrics
resonant bonding
multiple valence bands
ISSN:0935-9648, 1521-4095, 1521-4095
Online Access:Get full text
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Abstract Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh‐performance GeTe‐based thermoelectric materials is reviewed with a focus on the crystal structures, phase transitions, resonant bondings, multiple valance bands, and phonon dispersions. These features diversify the degrees of freedom to tune the transport properties of electrons and phonons for GeTe. On the basis of the optimized carrier concentration, strategies of alignment of multiple valence bands and density‐of‐state resonant distortion are employed to further enhance the thermoelectric performance of GeTe‐based materials. To decrease the thermal conductivity, methods of strengthening intrinsic phonon–phonon interactions and introducing various lattice imperfections as scattering centers are highlighted. An overview of thermoelectric devices assembled from GeTe‐based thermoelectric materials is then presented. In conclusion, possible future directions for developing GeTe in thermoelectric applications are proposed. The achieved high thermoelectric performance in GeTe‐based thermoelectric materials with rationally established strategies can act as a reference for broader materials to tailor their thermoelectric performance. Recent progress in GeTe thermoelectrics is reviewed with a focus on the diverse degrees of freedom to tailor thermoelectric properties. The strategies for enhancing power factors include optimizing carrier concentration, aligning multiple valence bands, density‐of‐state resonant distortion, and increasing band degeneracy by slight symmetry reduction. Decreasing the thermal conductivity can be achieved by intrinsically strengthening the phonon–phonon interactions and introducing planar vacancies.
AbstractList Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh‐performance GeTe‐based thermoelectric materials is reviewed with a focus on the crystal structures, phase transitions, resonant bondings, multiple valance bands, and phonon dispersions. These features diversify the degrees of freedom to tune the transport properties of electrons and phonons for GeTe. On the basis of the optimized carrier concentration, strategies of alignment of multiple valence bands and density‐of‐state resonant distortion are employed to further enhance the thermoelectric performance of GeTe‐based materials. To decrease the thermal conductivity, methods of strengthening intrinsic phonon–phonon interactions and introducing various lattice imperfections as scattering centers are highlighted. An overview of thermoelectric devices assembled from GeTe‐based thermoelectric materials is then presented. In conclusion, possible future directions for developing GeTe in thermoelectric applications are proposed. The achieved high thermoelectric performance in GeTe‐based thermoelectric materials with rationally established strategies can act as a reference for broader materials to tailor their thermoelectric performance.
Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh‐performance GeTe‐based thermoelectric materials is reviewed with a focus on the crystal structures, phase transitions, resonant bondings, multiple valance bands, and phonon dispersions. These features diversify the degrees of freedom to tune the transport properties of electrons and phonons for GeTe. On the basis of the optimized carrier concentration, strategies of alignment of multiple valence bands and density‐of‐state resonant distortion are employed to further enhance the thermoelectric performance of GeTe‐based materials. To decrease the thermal conductivity, methods of strengthening intrinsic phonon–phonon interactions and introducing various lattice imperfections as scattering centers are highlighted. An overview of thermoelectric devices assembled from GeTe‐based thermoelectric materials is then presented. In conclusion, possible future directions for developing GeTe in thermoelectric applications are proposed. The achieved high thermoelectric performance in GeTe‐based thermoelectric materials with rationally established strategies can act as a reference for broader materials to tailor their thermoelectric performance. Recent progress in GeTe thermoelectrics is reviewed with a focus on the diverse degrees of freedom to tailor thermoelectric properties. The strategies for enhancing power factors include optimizing carrier concentration, aligning multiple valence bands, density‐of‐state resonant distortion, and increasing band degeneracy by slight symmetry reduction. Decreasing the thermal conductivity can be achieved by intrinsically strengthening the phonon–phonon interactions and introducing planar vacancies.
Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh-performance GeTe-based thermoelectric materials is reviewed with a focus on the crystal structures, phase transitions, resonant bondings, multiple valance bands, and phonon dispersions. These features diversify the degrees of freedom to tune the transport properties of electrons and phonons for GeTe. On the basis of the optimized carrier concentration, strategies of alignment of multiple valence bands and density-of-state resonant distortion are employed to further enhance the thermoelectric performance of GeTe-based materials. To decrease the thermal conductivity, methods of strengthening intrinsic phonon-phonon interactions and introducing various lattice imperfections as scattering centers are highlighted. An overview of thermoelectric devices assembled from GeTe-based thermoelectric materials is then presented. In conclusion, possible future directions for developing GeTe in thermoelectric applications are proposed. The achieved high thermoelectric performance in GeTe-based thermoelectric materials with rationally established strategies can act as a reference for broader materials to tailor their thermoelectric performance.Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive endeavors are dedicated to enhancing the thermoelectric performance of ecofriendly materials. Herein, the most recent progress in superhigh-performance GeTe-based thermoelectric materials is reviewed with a focus on the crystal structures, phase transitions, resonant bondings, multiple valance bands, and phonon dispersions. These features diversify the degrees of freedom to tune the transport properties of electrons and phonons for GeTe. On the basis of the optimized carrier concentration, strategies of alignment of multiple valence bands and density-of-state resonant distortion are employed to further enhance the thermoelectric performance of GeTe-based materials. To decrease the thermal conductivity, methods of strengthening intrinsic phonon-phonon interactions and introducing various lattice imperfections as scattering centers are highlighted. An overview of thermoelectric devices assembled from GeTe-based thermoelectric materials is then presented. In conclusion, possible future directions for developing GeTe in thermoelectric applications are proposed. The achieved high thermoelectric performance in GeTe-based thermoelectric materials with rationally established strategies can act as a reference for broader materials to tailor their thermoelectric performance.
Author Hong, Min
Chen, Zhi‐Gang
Zou, Jin
Author_xml – sequence: 1
  givenname: Min
  surname: Hong
  fullname: Hong, Min
  organization: University of Queensland
– sequence: 2
  givenname: Jin
  surname: Zou
  fullname: Zou, Jin
  email: j.zou@uq.edu.au
  organization: University of Queensland
– sequence: 3
  givenname: Zhi‐Gang
  orcidid: 0000-0002-9309-7993
  surname: Chen
  fullname: Chen, Zhi‐Gang
  email: zhigang.chen@usq.edu.au, zhigang.chen@uq.edu.au
  organization: University of Queensland
BackLink https://www.ncbi.nlm.nih.gov/pubmed/30756468$$D View this record in MEDLINE/PubMed
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Copyright 2019 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim
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Issue 14
Keywords phonon scatterings
phase transitions
GeTe thermoelectrics
resonant bonding
multiple valence bands
Language English
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Snippet Driven by the ability to harvest waste heat into reusable electricity and the exclusive role of serving as the power generator for deep spacecraft, intensive...
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SubjectTerms Banded structure
Carrier density
Cooling
Crystal structure
Degrees of freedom
GeTe thermoelectrics
Materials science
multiple valence bands
Phase transitions
phonon scatterings
Phonons
resonant bonding
Spacecraft
Thermal conductivity
Thermoelectric materials
Transport properties
Title Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201807071
https://www.ncbi.nlm.nih.gov/pubmed/30756468
https://www.proquest.com/docview/2201708245
https://www.proquest.com/docview/2202194322
Volume 31
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