Electron spin relaxation in CMR manganites: absence of critical acceleration
Using original modulation technique, the longitudinal electron spin-lattice relaxation time T 1 has been measured in a series of nearly cubic La 1− x Ca x MnO 3 ( x=0.1; 0.2; 0.25; 0.33) and layered La 2−2 x Sr 1+2 x Mn 2O 7 ( x=0.4 and 0.5) manganites both in paramagnetic state and around the tempe...
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| Published in: | Journal of Magnetism and Magnetic Materials Vol. 258; pp. 256 - 258 |
|---|---|
| Main Authors: | , , , , , , , |
| Format: | Journal Article |
| Language: | English Japanese |
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Elsevier B.V
01.03.2003
Elsevier BV |
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| ISSN: | 0304-8853 |
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| Abstract | Using original modulation technique, the longitudinal electron spin-lattice relaxation time
T
1 has been measured in a series of nearly cubic La
1−
x
Ca
x
MnO
3 (
x=0.1; 0.2; 0.25; 0.33) and layered La
2−2
x
Sr
1+2
x
Mn
2O
7 (
x=0.4 and 0.5) manganites both in paramagnetic state and around the temperature (
T
c) of the magnetic ordering. The data are compared with the evolution of the transverse relaxation time
T
2 as determined from the ESR linewidth. Well above
T
c, the
T
1=
T
2 equality is confirmed, whereas a pronounced slowing down of
T
1 is observed in all the materials as
T
c is approached. The temperature dependence of
T
1 is found to be consistent with that of
Tχ(
T), where
χ(
T) represents the temperature dependence of the electron-spin susceptibility determined from the ESR absorption area. The interpretation suggests freezing the local field fluctuations due to polarization of superparamagnetic clusters in the external magnetic field. |
|---|---|
| AbstractList | Using original modulation technique, the longitudinal electron spin-lattice relaxation time
T
1 has been measured in a series of nearly cubic La
1−
x
Ca
x
MnO
3 (
x=0.1; 0.2; 0.25; 0.33) and layered La
2−2
x
Sr
1+2
x
Mn
2O
7 (
x=0.4 and 0.5) manganites both in paramagnetic state and around the temperature (
T
c) of the magnetic ordering. The data are compared with the evolution of the transverse relaxation time
T
2 as determined from the ESR linewidth. Well above
T
c, the
T
1=
T
2 equality is confirmed, whereas a pronounced slowing down of
T
1 is observed in all the materials as
T
c is approached. The temperature dependence of
T
1 is found to be consistent with that of
Tχ(
T), where
χ(
T) represents the temperature dependence of the electron-spin susceptibility determined from the ESR absorption area. The interpretation suggests freezing the local field fluctuations due to polarization of superparamagnetic clusters in the external magnetic field. |
| Author | Demidov, V.V. Atsarkin, V.A. Moritomo, Y. Gaal, R. Jánossy, A. Forró, L. Simon, F. Conder, K. |
| Author_xml | – sequence: 1 givenname: V.A. surname: Atsarkin fullname: Atsarkin, V.A. email: atsarkin@mail.cplire.ru organization: Institute of Radio Engineering and Electronics, Russian Academy of Sciences, 101999 Moscow, Russia – sequence: 2 givenname: V.V. surname: Demidov fullname: Demidov, V.V. organization: Institute of Radio Engineering and Electronics, Russian Academy of Sciences, 101999 Moscow, Russia – sequence: 3 givenname: F. surname: Simon fullname: Simon, F. organization: Departement de Physique, EPFL, CH-1015 Lausanne, Switzerland – sequence: 4 givenname: R. surname: Gaal fullname: Gaal, R. organization: Departement de Physique, EPFL, CH-1015 Lausanne, Switzerland – sequence: 5 givenname: Y. surname: Moritomo fullname: Moritomo, Y. organization: Center for Integrated Research in Science and Engineering, Nagoya University, Nagoya 464-8601, Japan – sequence: 6 givenname: K. surname: Conder fullname: Conder, K. organization: Laboratory for Neutron Scattering, ETH Zurich and PSI, CH-5232 Villigen, Switzerland – sequence: 7 givenname: A. surname: Jánossy fullname: Jánossy, A. organization: Department of Physics, Technical University of Budapest, H-1111 Budapest, Hungary – sequence: 8 givenname: L. surname: Forró fullname: Forró, L. organization: Departement de Physique, EPFL, CH-1015 Lausanne, Switzerland |
| BackLink | https://cir.nii.ac.jp/crid/1871146592590599680$$DView record in CiNii |
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| Cites_doi | 10.1007/BF03162448 10.1103/PhysRevB.52.1290 10.1016/S0022-3697(71)80392-X 10.1103/PhysRevB.61.15269 10.1103/PhysRevB.58.3233 10.1007/BF03162374 10.1016/0038-1098(82)90271-X 10.1103/PhysRevB.9.197 10.1103/PhysRevB.61.5888 10.1103/PhysRevLett.81.1102 10.1103/PhysRevB.62.5313 10.1016/S0370-1573(00)00111-3 10.1103/PhysRevB.60.11922 10.1103/PhysRevB.61.6213 10.1103/PhysRevB.63.174413 10.1103/PhysRevB.60.12155 10.1103/PhysRevB.63.092405 10.1016/S0375-9601(99)00438-7 10.1016/S0921-4526(97)81596-7 10.1038/380141a0 10.1080/000187399243455 |
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| Keywords | Spin relaxation Critical phenomena Electron spin resonance Manganites |
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| Snippet | Using original modulation technique, the longitudinal electron spin-lattice relaxation time
T
1 has been measured in a series of nearly cubic La
1−
x
Ca
x
MnO... |
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| StartPage | 256 |
| SubjectTerms | Critical phenomena Electron spin resonance Manganites Spin relaxation |
| Title | Electron spin relaxation in CMR manganites: absence of critical acceleration |
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