Achieving high-energy-density and ultra-stable zinc-ion hybrid supercapacitors by engineering hierarchical porous carbon architecture

Zinc-ion hybrid supercapacitor emerges as a promising energy storage device in benefit of the merits from both battery and supercapacitor. However, the challenges induced by the low energy density and poor cycling stability of the cathodes hinder the practical applications of zinc-ion hybrid superca...

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Published in:	Electrochimica acta Vol. 327; p. 134999
Main Authors:	Yu, Peifeng, Zeng, Yuan, Zeng, Yinxiang, Dong, Hanwu, Hu, Hang, Liu, Yingliang, Zheng, Mingtao, Xiao, Yong, Lu, Xihong, Liang, Yeru
Format:	Journal Article
Language:	English
Published:	Oxford Elsevier Ltd 10.12.2019 Elsevier BV
Subjects:	Architecture Carbon Cathodes Cycles Cycling stability Electrical resistivity Energy storage Flux density Graphitization Hierarchical porous carbon High energy density Ion storage Molecular-scale mixing strategy Morphology Specific surface Stability Structural engineering Structural hierarchy Supercapacitors Surface area Zinc Zinc-ion hybrid supercapacitors Cycling stability Hierarchical porous carbon High energy density Molecular-scale mixing strategy Zinc-ion hybrid supercapacitors
ISSN:	0013-4686, 1873-3859
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Abstract	Zinc-ion hybrid supercapacitor emerges as a promising energy storage device in benefit of the merits from both battery and supercapacitor. However, the challenges induced by the low energy density and poor cycling stability of the cathodes hinder the practical applications of zinc-ion hybrid supercapacitors. To address these issues, a structural engineering of carbonaceous cathode into a hierarchical porous architecture based on a hydrothermal-assisted molecular-scale mixing strategy is proposed. The key structures of the as-fabricated hierarchical porous carbon consist of high specific surface area, well-interconnected hierarchical porous morphology and favorable graphitization degree with good conductivity, which promises great conceptual and technological potential for high-performance zinc-ion storage. It is demonstrated that the high specific surface area supply sufficient active sites for zinc-ion storage, and collectively, the valuable hierarchical porous structure and high electric conductivity are beneficial for rapid transfer/diffusion of zinc ion. An ultrahigh capacity of 305 mAh g−1, a high energy density of 118 Wh kg−1, good rate capability, and excellent cycling stability of over 94.9% after 20000 cycles at a high current density of 2 A g−1 can be achieved when hierarchical porous carbon is used as the cathode of a zinc-ion hybrid supercapacitor. [Display omitted] •High-energy-density and ultra-stable zinc-ion hybrid supercapacitors are realized.•Hierarchical porous carbon is obtained based on a purposeful hydrothermal-assisted molecular-scale mixing strategy.•High surface area, hierarchical porous architecture and favorable graphitization degree is favorable to zinc-ion storage.
AbstractList	Zinc-ion hybrid supercapacitor emerges as a promising energy storage device in benefit of the merits from both battery and supercapacitor. However, the challenges induced by the low energy density and poor cycling stability of the cathodes hinder the practical applications of zinc-ion hybrid supercapacitors. To address these issues, a structural engineering of carbonaceous cathode into a hierarchical porous architecture based on a hydrothermal-assisted molecular-scale mixing strategy is proposed. The key structures of the as-fabricated hierarchical porous carbon consist of high specific surface area, well-interconnected hierarchical porous morphology and favorable graphitization degree with good conductivity, which promises great conceptual and technological potential for high-performance zinc-ion storage. It is demonstrated that the high specific surface area supply sufficient active sites for zinc-ion storage, and collectively, the valuable hierarchical porous structure and high electric conductivity are beneficial for rapid transfer/diffusion of zinc ion. An ultrahigh capacity of 305 mAh g−1, a high energy density of 118 Wh kg−1, good rate capability, and excellent cycling stability of over 94.9% after 20000 cycles at a high current density of 2 A g−1 can be achieved when hierarchical porous carbon is used as the cathode of a zinc-ion hybrid supercapacitor. Zinc-ion hybrid supercapacitor emerges as a promising energy storage device in benefit of the merits from both battery and supercapacitor. However, the challenges induced by the low energy density and poor cycling stability of the cathodes hinder the practical applications of zinc-ion hybrid supercapacitors. To address these issues, a structural engineering of carbonaceous cathode into a hierarchical porous architecture based on a hydrothermal-assisted molecular-scale mixing strategy is proposed. The key structures of the as-fabricated hierarchical porous carbon consist of high specific surface area, well-interconnected hierarchical porous morphology and favorable graphitization degree with good conductivity, which promises great conceptual and technological potential for high-performance zinc-ion storage. It is demonstrated that the high specific surface area supply sufficient active sites for zinc-ion storage, and collectively, the valuable hierarchical porous structure and high electric conductivity are beneficial for rapid transfer/diffusion of zinc ion. An ultrahigh capacity of 305 mAh g−1, a high energy density of 118 Wh kg−1, good rate capability, and excellent cycling stability of over 94.9% after 20000 cycles at a high current density of 2 A g−1 can be achieved when hierarchical porous carbon is used as the cathode of a zinc-ion hybrid supercapacitor. [Display omitted] •High-energy-density and ultra-stable zinc-ion hybrid supercapacitors are realized.•Hierarchical porous carbon is obtained based on a purposeful hydrothermal-assisted molecular-scale mixing strategy.•High surface area, hierarchical porous architecture and favorable graphitization degree is favorable to zinc-ion storage.
ArticleNumber	134999
Author	Dong, Hanwu Yu, Peifeng Liu, Yingliang Zeng, Yuan Zheng, Mingtao Liang, Yeru Xiao, Yong Zeng, Yinxiang Hu, Hang Lu, Xihong
Author_xml	– sequence: 1 givenname: Peifeng surname: Yu fullname: Yu, Peifeng organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 2 givenname: Yuan surname: Zeng fullname: Zeng, Yuan organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 3 givenname: Yinxiang surname: Zeng fullname: Zeng, Yinxiang organization: MOE of the Key Laboratory of Bioinorganic and Synthetic Chemistry, KLGHEI of Environment and Energy Chemistry, School of Chemistry, Sun Yat-sen University, Guangzhou, 510275, PR China – sequence: 4 givenname: Hanwu surname: Dong fullname: Dong, Hanwu organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 5 givenname: Hang surname: Hu fullname: Hu, Hang organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 6 givenname: Yingliang surname: Liu fullname: Liu, Yingliang email: tliuyl@scau.edu.cn organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 7 givenname: Mingtao surname: Zheng fullname: Zheng, Mingtao organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 8 givenname: Yong surname: Xiao fullname: Xiao, Yong organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China – sequence: 9 givenname: Xihong surname: Lu fullname: Lu, Xihong email: luxh6@mail.sysu.edu.cn organization: MOE of the Key Laboratory of Bioinorganic and Synthetic Chemistry, KLGHEI of Environment and Energy Chemistry, School of Chemistry, Sun Yat-sen University, Guangzhou, 510275, PR China – sequence: 10 givenname: Yeru surname: Liang fullname: Liang, Yeru email: liangyr@scau.edu.cn organization: College of Materials and Energy, South China Agricultural University, Guangzhou, 510642, PR China
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Snippet	Zinc-ion hybrid supercapacitor emerges as a promising energy storage device in benefit of the merits from both battery and supercapacitor. However, the...
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SubjectTerms	Architecture Carbon Cathodes Cycles Cycling stability Electrical resistivity Energy storage Flux density Graphitization Hierarchical porous carbon High energy density Ion storage Molecular-scale mixing strategy Morphology Specific surface Stability Structural engineering Structural hierarchy Supercapacitors Surface area Zinc Zinc-ion hybrid supercapacitors
Title	Achieving high-energy-density and ultra-stable zinc-ion hybrid supercapacitors by engineering hierarchical porous carbon architecture
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