Recovery of cathode copper and ternary precursors from CuS slag derived by waste lithium-ion batteries: Process analysis and evaluation
The efficient and environmentally friendly recycling technology of waste residue that including abundant heavy metal produced during the recovery of lithium batteries has become a research hotspot. Herein, a novelty process of acid leaching-selective electrodeposition-deep impurity removal-regenerat...
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| Abstract | The efficient and environmentally friendly recycling technology of waste residue that including abundant heavy metal produced during the recovery of lithium batteries has become a research hotspot. Herein, a novelty process of acid leaching-selective electrodeposition-deep impurity removal-regeneration was proposed to recovery of the CuS slag, which has been efficient transferred to high purity cathode copper and commercially available ternary precursors. Copper cathode with a purity of 99.67% was prepared under electrochemical reaction conditions at −0.55 V for 2 h. A novel impurity remover-Mn powder, which was used to remove the residual impurities and as a feedstock for the ternary precursor. Finally, NCM523 was regenerated by co-precipitation. The process is superior to the traditional process in economy, energy consumption, CO2 emissions, product purity and process duration. This study provides a new approach for solid waste recovery and precious metal enrichment.
For the resourceful recovery of secondary waste from retired lithium-ion batteries, a novel process of acid leaching-selective electrodeposition-deep decontamination-regeneration was proposed to recover CuS slag, and regenerate it efficiently with high-purity cathode copper and commercially available ternary precursors. A new pathway for solid waste recovery and precious metal enrichment is provided. [Display omitted] |
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| AbstractList | The efficient and environmentally friendly recycling technology of waste residue that including abundant heavy metal produced during the recovery of lithium batteries has become a research hotspot. Herein, a novelty process of acid leaching-selective electrodeposition-deep impurity removal-regeneration was proposed to recovery of the CuS slag, which has been efficient transferred to high purity cathode copper and commercially available ternary precursors. Copper cathode with a purity of 99.67% was prepared under electrochemical reaction conditions at −0.55 V for 2 h. A novel impurity remover-Mn powder, which was used to remove the residual impurities and as a feedstock for the ternary precursor. Finally, NCM523 was regenerated by co-precipitation. The process is superior to the traditional process in economy, energy consumption, CO2 emissions, product purity and process duration. This study provides a new approach for solid waste recovery and precious metal enrichment.
For the resourceful recovery of secondary waste from retired lithium-ion batteries, a novel process of acid leaching-selective electrodeposition-deep decontamination-regeneration was proposed to recover CuS slag, and regenerate it efficiently with high-purity cathode copper and commercially available ternary precursors. A new pathway for solid waste recovery and precious metal enrichment is provided. [Display omitted] The efficient and environmentally friendly recycling technology of waste residue that including abundant heavy metal produced during the recovery of lithium batteries has become a research hotspot.Herein,a novelty process of acid leaching-selective electrodeposition-deep impurity removal-regeneration was pro-posed to recovery of the CuS slag,which has been efficient transferred to high purity cathode copper and commercially available ternary precursors.Copper cathode with a purity of 99.67% was prepared under electrochemical reaction conditions at-0.55 V for 2h.A novel impurity remover-Mn powder,which was used to remove the residual impurities and as a feedstock for the ternary precursor.Finally,NCM523 was regenerated by co-precipitation.The process is superior to the traditional process in economy,energy consumption,CO2 emissions,product purity and process duration.This study provides a new approach for solid waste recovery and precious metal enrichment. |
| ArticleNumber | 109172 |
| Author | Yang, Liming Han, Fei Yang, Guang Ding, Xuan Shi, Hui Wei, Yun Zhou, Lei Wang, Chaoqiang Feng, Yufa Hu, Wenbin Luo, Xubiao Shao, Penghui |
| AuthorAffiliation | National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization,Nanchang Hangkong University,Nanchang 330063,China%CAS Key Laboratory of Green Process and Engineering,National Engineering Research Center of Green Recycling for Strategic Metal Resources,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China%Biomass Molecular Engineering Center and Anhui Provincial Key Laboratory of Microbial Pest Control,Anhui Agricultural University,Hefei 230036,China%Jiangxi Ganfeng Recycling Technology Co.LTD.,Xinyu 338004,China%National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization,Nanchang Hangkong University,Nanchang 330063,China;School of Life Science,Jinggangshan University,Ji'an 343009,China |
| AuthorAffiliation_xml | – name: National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization,Nanchang Hangkong University,Nanchang 330063,China%CAS Key Laboratory of Green Process and Engineering,National Engineering Research Center of Green Recycling for Strategic Metal Resources,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China%Biomass Molecular Engineering Center and Anhui Provincial Key Laboratory of Microbial Pest Control,Anhui Agricultural University,Hefei 230036,China%Jiangxi Ganfeng Recycling Technology Co.LTD.,Xinyu 338004,China%National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization,Nanchang Hangkong University,Nanchang 330063,China;School of Life Science,Jinggangshan University,Ji'an 343009,China |
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| Keywords | Cathode copper Ternary precursor Electrodeposition Solid waste recovery CuS slag |
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| SubjectTerms | Cathode copper CuS slag Electrodeposition Solid waste recovery Ternary precursor |
| Title | Recovery of cathode copper and ternary precursors from CuS slag derived by waste lithium-ion batteries: Process analysis and evaluation |
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