Metal-decorated 3D tin oxide nanotubes in a monolithic sensor array chip for room-temperature gas identification
Inadequate limit of detection at room temperature and unsatisfactory selectivity remain challenge for wide applications of the chemiresistive gas sensors. Nanostructured gas sensors ensure the desirable activation energy for the gas adsorption and chemical reactions, favorable for room-temperature p...
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| Vydáno v: | Journal of alloys and compounds Ročník 976; s. 173075 |
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| Hlavní autoři: | , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Elsevier B.V
05.03.2024
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| ISSN: | 0925-8388 |
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| Abstract | Inadequate limit of detection at room temperature and unsatisfactory selectivity remain challenge for wide applications of the chemiresistive gas sensors. Nanostructured gas sensors ensure the desirable activation energy for the gas adsorption and chemical reactions, favorable for room-temperature parts-per-billion (ppb) level gas detection. In this work, we demonstrated a single-chip integrated gas sensor array (4 ×4 pixels) based on kinds of metal (Pt, Pd, Au, Ag) decorated 3D SnO2 nanotubes for ultrasensitive room-temperature gas-sensing. The nanostructured sensor array has a high surface area-to-volume ratio, enabling room temperature sensing with high detection response toward H2 (minimum 5 ppm), formaldehyde (minimum 50 ppb), toluene (minimum 50 ppb) and NO2 (minimum 100 ppb) with the detection accuracy within 5% range, respectively. In addition, the effect of metals decoration on the gas identification features were systematically conducted, and these specific response features can be mainly attributed to metal activation capability toward the gases, which enables demonstrating differentiable response patterns for the target gases identification employing a pattern recognition algorithm. These results demonstrate that the proposed strategy helps to provide an excellent route for the future low-power-consumption smart sensing devices design and fabrication.
•Metal-decorated 3D tin oxide nanotubes sensor array chip was realized.•The sensor array enables room temperature gas sensing with high detection accuracy.•The sensor array enables achieving gas identification in the specific circumstances. |
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| AbstractList | Inadequate limit of detection at room temperature and unsatisfactory selectivity remain challenge for wide applications of the chemiresistive gas sensors. Nanostructured gas sensors ensure the desirable activation energy for the gas adsorption and chemical reactions, favorable for room-temperature parts-per-billion (ppb) level gas detection. In this work, we demonstrated a single-chip integrated gas sensor array (4 ×4 pixels) based on kinds of metal (Pt, Pd, Au, Ag) decorated 3D SnO2 nanotubes for ultrasensitive room-temperature gas-sensing. The nanostructured sensor array has a high surface area-to-volume ratio, enabling room temperature sensing with high detection response toward H2 (minimum 5 ppm), formaldehyde (minimum 50 ppb), toluene (minimum 50 ppb) and NO2 (minimum 100 ppb) with the detection accuracy within 5% range, respectively. In addition, the effect of metals decoration on the gas identification features were systematically conducted, and these specific response features can be mainly attributed to metal activation capability toward the gases, which enables demonstrating differentiable response patterns for the target gases identification employing a pattern recognition algorithm. These results demonstrate that the proposed strategy helps to provide an excellent route for the future low-power-consumption smart sensing devices design and fabrication.
•Metal-decorated 3D tin oxide nanotubes sensor array chip was realized.•The sensor array enables room temperature gas sensing with high detection accuracy.•The sensor array enables achieving gas identification in the specific circumstances. |
| ArticleNumber | 173075 |
| Author | Song, Zhilong Yan, Jia |
| Author_xml | – sequence: 1 givenname: Jia surname: Yan fullname: Yan, Jia – sequence: 2 givenname: Zhilong surname: Song fullname: Song, Zhilong email: songzl@ujs.edu.cn |
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| CitedBy_id | crossref_primary_10_1016_j_jssc_2025_125251 crossref_primary_10_1016_j_vacuum_2025_114407 crossref_primary_10_1021_acsami_5c10408 crossref_primary_10_3390_s25154784 crossref_primary_10_1007_s00604_025_07234_6 crossref_primary_10_1016_j_mssp_2025_109448 crossref_primary_10_1021_acssensors_5c00045 crossref_primary_10_1016_j_ceramint_2025_03_074 crossref_primary_10_1039_D5NR02580J crossref_primary_10_1021_acssensors_5c01699 crossref_primary_10_1039_D5LC00570A |
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| Keywords | Gas identification Pattern recognition algorithm Metal decoration Gas sensor array Room temperature 3D nanostructured tin oxide |
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