Synthesis of Chitosan–Ignosulfonate Composite as an Adsorbent for Dyes and Metal Ions Removal from Wastewater
Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic d...
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| Published in: | ACS omega Vol. 4; no. 25; pp. 21421 - 21430 |
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| Main Authors: | , , , , |
| Format: | Journal Article |
| Language: | English |
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United States
American Chemical Society
17.12.2019
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| ISSN: | 2470-1343, 2470-1343 |
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| Abstract | Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO3 –) and HCrO4 – groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO3 – of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B. |
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| AbstractList | Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO
) and HCrO
groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO
of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B. Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO3 –) and HCrO4 – groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO3 – of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B. Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO3–) and HCrO4– groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO3– of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B. Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO3 -) and HCrO4 - groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO3 - of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B.Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization. In this study, the adsorption material was prepared by blending sodium lignosulfonate and chitosan, which could adsorb anionic and cationic dyes and metal ions. The composite was characterized by Fourier transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), and thermogravimetry (TG). The results showed that the composite was cross-linked mainly by the strong electrostatic interaction between the protonated amino group in chitosan and the sulfonate group in sodium lignosulfonate. Moreover, the effects of initial concentration, adsorption time, initial pH, and mass ratio of chitosan to sodium lignosulfonate on the adsorption performance of the composite were investigated. Meanwhile, the adsorption processes were agreed well with the pseudo-second-order kinetic model and Langmuir isotherm model. The adsorption mechanism was that the electrostatic interaction between the protonated amino and hydroxyl groups of the composite with anionic (SO3 -) and HCrO4 - groups of Congo red and Cr(VI), respectively. In addition, the electrostatic interaction between SO3 - of the composite and positively charged group of Rhodamine B played an important role in the adsorption of Rhodamine B. |
| Author | Chang, Jianmin Cui, Yong Gu, Fei Li, Meiling Geng, Jing |
| AuthorAffiliation | College of Material Science and Technology Precision Manufacturing Engineering Department |
| AuthorAffiliation_xml | – name: College of Material Science and Technology – name: Precision Manufacturing Engineering Department |
| Author_xml | – sequence: 1 givenname: Fei surname: Gu fullname: Gu, Fei organization: College of Material Science and Technology – sequence: 2 givenname: Jing surname: Geng fullname: Geng, Jing organization: College of Material Science and Technology – sequence: 3 givenname: Meiling surname: Li fullname: Li, Meiling organization: College of Material Science and Technology – sequence: 4 givenname: Jianmin orcidid: 0000-0001-9622-0275 surname: Chang fullname: Chang, Jianmin email: cjianmin168@126.com organization: College of Material Science and Technology – sequence: 5 givenname: Yong surname: Cui fullname: Cui, Yong organization: Precision Manufacturing Engineering Department |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31867537$$D View this record in MEDLINE/PubMed |
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| Snippet | Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization.... Sodium lignosulfonate is a polymer with extensive sources and abundant functional groups. Therefore, it has potential value for research and wide utilization.... |
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| Title | Synthesis of Chitosan–Ignosulfonate Composite as an Adsorbent for Dyes and Metal Ions Removal from Wastewater |
| URI | http://dx.doi.org/10.1021/acsomega.9b03128 https://www.ncbi.nlm.nih.gov/pubmed/31867537 https://www.proquest.com/docview/2330062931 https://pubmed.ncbi.nlm.nih.gov/PMC6921639 https://doaj.org/article/4c2df7f477754053b93a42b537fec074 |
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