Exploring the High-Temperature Window of Operation for Organic Photovoltaics: A Combined Experimental and Simulations Study
Gespeichert in:
| Titel: | Exploring the High-Temperature Window of Operation for Organic Photovoltaics: A Combined Experimental and Simulations Study |
|---|---|
| Autoren: | Negash, Asfaw, Hustings, Jeroen, Robert, Allyson, Wolkeba, Zewdneh Genene, 1983, Yilma, Desalegn, Schreurs, Dieter, Mathijs, Michiel, Liesenborgs, Jori, Van Reeth, Frank, Vandewal, K., Mammo, Wendimagen, Admassie, Shimelis, Maes, Wouter, Manca, Jean |
| Quelle: | Advanced Materials for Optics and Electronics. 34(6) |
| Schlagwörter: | simulations, organic photovoltaics, high-temperature operation |
| Beschreibung: | The global climate change negatively affects the photovoltaic performance of traditional solar cell technologies. This article investigates the potential of organic photovoltaics (OPV) for high-temperature environments, ranging from urban hot summers (30—40 °C) and desert regions (65 °C) up to (aero) space conditions (130 °C), the thermal window in which OPV can operate. The approach is based on a combination of experiments and simulations up to 180 °C, moving significantly beyond the conventional temperature ranges reported in the literature. New 2H-benzo[d][1,2,3]triazole-5,6-dicarboxylic imide-based copolymers with decomposition onset temperatures above 340 °C are used for this study, in combination with non-fullerene acceptors. Contrary to their inorganic counterparts, OPV devices show a positive temperature coefficient up to ≈90 °C. At temperatures of 150 °C, they are still operational, retaining their room temperature efficiency. Complementary simulations are performed using an in-house developed software package that numerically solves the drift-diffusion equations to understand the general trends in the obtained current–voltage characteristics and the materials’ intrinsic behavior as a function of temperature. The presented methodology of combined high-temperature experiments and simulations can be further applied to investigate the thermal window of operation for other OPV material systems, opening novel high-temperature application routes. |
| Dateibeschreibung: | electronic |
| Zugangs-URL: | https://research.chalmers.se/publication/538125 https://research.chalmers.se/publication/538125/file/538125_Fulltext.pdf |
| Datenbank: | SwePub |
| FullText | Text: Availability: 0 CustomLinks: – Url: https://research.chalmers.se/publication/538125# Name: EDS - SwePub (s4221598) Category: fullText Text: View record in SwePub – Url: https://resolver.ebscohost.com/openurl?sid=EBSCO:edsswe&genre=article&issn=1616301x&ISBN=&volume=34&issue=6&date=20240101&spage=&pages=&title=Advanced Materials for Optics and Electronics&atitle=Exploring%20the%20High-Temperature%20Window%20of%20Operation%20for%20Organic%20Photovoltaics%3A%20A%20Combined%20Experimental%20and%20Simulations%20Study&aulast=Negash%2C%20Asfaw&id=DOI:10.1002/adfm.202308666 Name: Full Text Finder Category: fullText Text: Full Text Finder Icon: https://imageserver.ebscohost.com/branding/images/FTF.gif MouseOverText: Full Text Finder – Url: https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=EBSCO&SrcAuth=EBSCO&DestApp=WOS&ServiceName=TransferToWoS&DestLinkType=GeneralSearchSummary&Func=Links&author=Negash%20A Name: ISI Category: fullText Text: Nájsť tento článok vo Web of Science Icon: https://imagesrvr.epnet.com/ls/20docs.gif MouseOverText: Nájsť tento článok vo Web of Science |
|---|---|
| Header | DbId: edsswe DbLabel: SwePub An: edsswe.oai.research.chalmers.se.d18c9945.c467.4fa8.be9f.241bcf39a664 RelevancyScore: 1014 AccessLevel: 6 PubType: Academic Journal PubTypeId: academicJournal PreciseRelevancyScore: 1014.41540527344 |
| IllustrationInfo | |
| Items | – Name: Title Label: Title Group: Ti Data: Exploring the High-Temperature Window of Operation for Organic Photovoltaics: A Combined Experimental and Simulations Study – Name: Author Label: Authors Group: Au Data: <searchLink fieldCode="AR" term="%22Negash%2C+Asfaw%22">Negash, Asfaw</searchLink><br /><searchLink fieldCode="AR" term="%22Hustings%2C+Jeroen%22">Hustings, Jeroen</searchLink><br /><searchLink fieldCode="AR" term="%22Robert%2C+Allyson%22">Robert, Allyson</searchLink><br /><searchLink fieldCode="AR" term="%22Wolkeba%2C+Zewdneh+Genene%22">Wolkeba, Zewdneh Genene</searchLink>, 1983<br /><searchLink fieldCode="AR" term="%22Yilma%2C+Desalegn%22">Yilma, Desalegn</searchLink><br /><searchLink fieldCode="AR" term="%22Schreurs%2C+Dieter%22">Schreurs, Dieter</searchLink><br /><searchLink fieldCode="AR" term="%22Mathijs%2C+Michiel%22">Mathijs, Michiel</searchLink><br /><searchLink fieldCode="AR" term="%22Liesenborgs%2C+Jori%22">Liesenborgs, Jori</searchLink><br /><searchLink fieldCode="AR" term="%22Van+Reeth%2C+Frank%22">Van Reeth, Frank</searchLink><br /><searchLink fieldCode="AR" term="%22Vandewal%2C+K%2E%22">Vandewal, K.</searchLink><br /><searchLink fieldCode="AR" term="%22Mammo%2C+Wendimagen%22">Mammo, Wendimagen</searchLink><br /><searchLink fieldCode="AR" term="%22Admassie%2C+Shimelis%22">Admassie, Shimelis</searchLink><br /><searchLink fieldCode="AR" term="%22Maes%2C+Wouter%22">Maes, Wouter</searchLink><br /><searchLink fieldCode="AR" term="%22Manca%2C+Jean%22">Manca, Jean</searchLink> – Name: TitleSource Label: Source Group: Src Data: <i>Advanced Materials for Optics and Electronics</i>. 34(6) – Name: Subject Label: Subject Terms Group: Su Data: <searchLink fieldCode="DE" term="%22simulations%22">simulations</searchLink><br /><searchLink fieldCode="DE" term="%22organic+photovoltaics%22">organic photovoltaics</searchLink><br /><searchLink fieldCode="DE" term="%22high-temperature+operation%22">high-temperature operation</searchLink> – Name: Abstract Label: Description Group: Ab Data: The global climate change negatively affects the photovoltaic performance of traditional solar cell technologies. This article investigates the potential of organic photovoltaics (OPV) for high-temperature environments, ranging from urban hot summers (30—40 °C) and desert regions (65 °C) up to (aero) space conditions (130 °C), the thermal window in which OPV can operate. The approach is based on a combination of experiments and simulations up to 180 °C, moving significantly beyond the conventional temperature ranges reported in the literature. New 2H-benzo[d][1,2,3]triazole-5,6-dicarboxylic imide-based copolymers with decomposition onset temperatures above 340 °C are used for this study, in combination with non-fullerene acceptors. Contrary to their inorganic counterparts, OPV devices show a positive temperature coefficient up to ≈90 °C. At temperatures of 150 °C, they are still operational, retaining their room temperature efficiency. Complementary simulations are performed using an in-house developed software package that numerically solves the drift-diffusion equations to understand the general trends in the obtained current–voltage characteristics and the materials’ intrinsic behavior as a function of temperature. The presented methodology of combined high-temperature experiments and simulations can be further applied to investigate the thermal window of operation for other OPV material systems, opening novel high-temperature application routes. – Name: Format Label: File Description Group: SrcInfo Data: electronic – Name: URL Label: Access URL Group: URL Data: <link linkTarget="URL" linkTerm="https://research.chalmers.se/publication/538125" linkWindow="_blank">https://research.chalmers.se/publication/538125</link><br /><link linkTarget="URL" linkTerm="https://research.chalmers.se/publication/538125/file/538125_Fulltext.pdf" linkWindow="_blank">https://research.chalmers.se/publication/538125/file/538125_Fulltext.pdf</link> |
| PLink | https://erproxy.cvtisr.sk/sfx/access?url=https://search.ebscohost.com/login.aspx?direct=true&site=eds-live&db=edsswe&AN=edsswe.oai.research.chalmers.se.d18c9945.c467.4fa8.be9f.241bcf39a664 |
| RecordInfo | BibRecord: BibEntity: Identifiers: – Type: doi Value: 10.1002/adfm.202308666 Languages: – Text: English Subjects: – SubjectFull: simulations Type: general – SubjectFull: organic photovoltaics Type: general – SubjectFull: high-temperature operation Type: general Titles: – TitleFull: Exploring the High-Temperature Window of Operation for Organic Photovoltaics: A Combined Experimental and Simulations Study Type: main BibRelationships: HasContributorRelationships: – PersonEntity: Name: NameFull: Negash, Asfaw – PersonEntity: Name: NameFull: Hustings, Jeroen – PersonEntity: Name: NameFull: Robert, Allyson – PersonEntity: Name: NameFull: Wolkeba, Zewdneh Genene – PersonEntity: Name: NameFull: Yilma, Desalegn – PersonEntity: Name: NameFull: Schreurs, Dieter – PersonEntity: Name: NameFull: Mathijs, Michiel – PersonEntity: Name: NameFull: Liesenborgs, Jori – PersonEntity: Name: NameFull: Van Reeth, Frank – PersonEntity: Name: NameFull: Vandewal, K. – PersonEntity: Name: NameFull: Mammo, Wendimagen – PersonEntity: Name: NameFull: Admassie, Shimelis – PersonEntity: Name: NameFull: Maes, Wouter – PersonEntity: Name: NameFull: Manca, Jean IsPartOfRelationships: – BibEntity: Dates: – D: 01 M: 01 Type: published Y: 2024 Identifiers: – Type: issn-print Value: 1616301x – Type: issn-print Value: 16163028 – Type: issn-locals Value: SWEPUB_FREE – Type: issn-locals Value: CTH_SWEPUB Numbering: – Type: volume Value: 34 – Type: issue Value: 6 Titles: – TitleFull: Advanced Materials for Optics and Electronics Type: main |
| ResultId | 1 |
Full Text Finder
Nájsť tento článok vo Web of Science