Three-dimensional collective charge excitations in electron-doped copper oxide superconductors

High-temperature copper oxide superconductors consist of stacked CuO 2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional 1 , 2 , but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane ch...

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Vydáno v:Nature (London) Ročník 563; číslo 7731; s. 374 - 378
Hlavní autoři: Hepting, M., Chaix, L., Huang, E. W., Fumagalli, R., Peng, Y. Y., Moritz, B., Kummer, K., Brookes, N. B., Lee, W. C., Hashimoto, M., Sarkar, T., He, J.-F., Rotundu, C. R., Lee, Y. S., Greene, R. L., Braicovich, L., Ghiringhelli, G., Shen, Z. X., Devereaux, T. P., Lee, W. S.
Médium: Journal Article
Jazyk:angličtina
Vydáno: London Nature Publishing Group UK 01.11.2018
Nature Publishing Group
Témata:
639/301/119/995
639/301/119/999
639/766/119/1003
639/766/930/12
Acoustic properties
Acoustics
Aircraft
Brillouin zones
Condensed Matter
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Copper
Copper compounds
Copper oxides
Crystallography
Dispersion
Electric properties
Electrons
Energy
High temperature
High temperature superconductors
Humanities and Social Sciences
Inelastic scattering
Lattice parameters
Lattice vibration
Letter
multidisciplinary
Optics
Periodicity
Physics
Planes
Properties
Resveratrol
Science
Science (multidisciplinary)
Spectrum analysis
Superconductors
X-ray scattering
Resonant Inelastic X-ray Scattering (RIXS)
Charge Dynamics
CuO2 Planes
Acoustic Plasmons
RIXS Spectra
ISSN:0028-0836, 1476-4687, 1476-4687
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Abstract High-temperature copper oxide superconductors consist of stacked CuO 2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional 1 , 2 , but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state 3 , 4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides 5 – 7 reveals their charge origin, that is, without mixing with magnetic components 5 – 7 . The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO 2 planes rather than to the crystallographic c -axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought ‘acoustic plasmon’, which is a branch of distinct charge collective modes predicted for layered systems 8 – 12 and argued to play a substantial part in mediating high-temperature superconductivity 10 – 12 . Resonant inelastic X-ray scattering on electron-doped copper oxide superconductors reveals a three-dimensional charge collective mode, which has properties suggestive of the long-sought acoustic plasmon.
AbstractList High-temperature copper oxide superconductors consist of stacked CuO.sub.2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional.sup.1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state.sup.3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides.sup.5-7 reveals their charge origin, that is, without mixing with magnetic components.sup.5-7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO.sub.2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems.sup.8-12 and argued to play a substantial part in mediating high-temperature superconductivity.sup.10-12.
High-temperature copper oxide superconductors consist of stacked CuO 2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional 1 , 2 , but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state 3 , 4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides 5 – 7 reveals their charge origin, that is, without mixing with magnetic components 5 – 7 . The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO 2 planes rather than to the crystallographic c -axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought ‘acoustic plasmon’, which is a branch of distinct charge collective modes predicted for layered systems 8 – 12 and argued to play a substantial part in mediating high-temperature superconductivity 10 – 12 . Resonant inelastic X-ray scattering on electron-doped copper oxide superconductors reveals a three-dimensional charge collective mode, which has properties suggestive of the long-sought acoustic plasmon.
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides5-7 reveals their charge origin, that is, without mixing with magnetic components5-7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems8-12 and argued to play a substantial part in mediating high-temperature superconductivity10-12.
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides5-7 reveals their charge origin, that is, without mixing with magnetic components5-7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems8-12 and argued to play a substantial part in mediating high-temperature superconductivity10-12.High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides5-7 reveals their charge origin, that is, without mixing with magnetic components5-7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems8-12 and argued to play a substantial part in mediating high-temperature superconductivity10-12.
High-temperature copper oxide superconductors consist of stacked CuO.sub.2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional.sup.1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state.sup.3,4 within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides.sup.5-7 reveals their charge origin, that is, without mixing with magnetic components.sup.5-7. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO.sub.2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems.sup.8-12 and argued to play a substantial part in mediating high-temperature superconductivity.sup.10-12.Resonant inelastic X-ray scattering on electron-doped copper oxide superconductors reveals a three-dimensional charge collective mode, which has properties suggestive of the long-sought acoustic plasmon.
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily two-dimensional1,2, but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state within the limited range of momenta accessible by optics. Here in this study, we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides reveals their charge origin, that is, without mixing with magnetic components. The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO2 planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought ‘acoustic plasmon’, which is a branch of distinct charge collective modes predicted for layered systems and argued to play a substantial part in mediating high-temperature superconductivity.
High-temperature copper oxide superconductors consist of stacked CuO planes, with electronic band structures and magnetic excitations that are primarily two-dimensional , but with superconducting coherence that is three-dimensional. This dichotomy highlights the importance of out-of-plane charge dynamics, which has been found to be incoherent in the normal state within the limited range of momenta accessible by optics. Here we use resonant inelastic X-ray scattering to explore the charge dynamics across all three dimensions of the Brillouin zone. Polarization analysis of recently discovered collective excitations (modes) in electron-doped copper oxides reveals their charge origin, that is, without mixing with magnetic components . The excitations disperse along both the in-plane and out-of-plane directions, revealing its three-dimensional nature. The periodicity of the out-of-plane dispersion corresponds to the distance between neighbouring CuO planes rather than to the crystallographic c-axis lattice constant, suggesting that the interplane Coulomb interaction is responsible for the coherent out-of-plane charge dynamics. The observed properties are hallmarks of the long-sought 'acoustic plasmon', which is a branch of distinct charge collective modes predicted for layered systems and argued to play a substantial part in mediating high-temperature superconductivity .
Audience Academic
Author Shen, Z. X.
Lee, W. C.
Peng, Y. Y.
Fumagalli, R.
Kummer, K.
Moritz, B.
Lee, Y. S.
He, J.-F.
Ghiringhelli, G.
Hashimoto, M.
Brookes, N. B.
Huang, E. W.
Devereaux, T. P.
Lee, W. S.
Sarkar, T.
Rotundu, C. R.
Greene, R. L.
Chaix, L.
Hepting, M.
Braicovich, L.
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  surname: Hepting
  fullname: Hepting, M.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
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  givenname: L.
  surname: Chaix
  fullname: Chaix, L.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University, Université Grenoble Alpes, CNRS, Institut Néel
– sequence: 3
  givenname: E. W.
  surname: Huang
  fullname: Huang, E. W.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University, Department of Physics, Stanford University
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  surname: Fumagalli
  fullname: Fumagalli, R.
  organization: Dipartimento di Fisica, Politecnico di Milano
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  givenname: Y. Y.
  surname: Peng
  fullname: Peng, Y. Y.
  organization: Dipartimento di Fisica, Politecnico di Milano, Department of Physics and Seitz Materials Research Lab, University of Illinois
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  surname: Moritz
  fullname: Moritz, B.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
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  surname: Kummer
  fullname: Kummer, K.
  organization: European Synchrotron Radiation Facility (ESRF)
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  surname: Brookes
  fullname: Brookes, N. B.
  organization: European Synchrotron Radiation Facility (ESRF)
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  surname: Lee
  fullname: Lee, W. C.
  organization: Department of Physics, Binghamton University
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  surname: Hashimoto
  fullname: Hashimoto, M.
  organization: Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
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  surname: Sarkar
  fullname: Sarkar, T.
  organization: Department of Physics, Center for Nanophysics and Advanced Materials, University of Maryland
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  givenname: J.-F.
  surname: He
  fullname: He, J.-F.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University, Department of Physics, University of Science and Technology of China
– sequence: 13
  givenname: C. R.
  surname: Rotundu
  fullname: Rotundu, C. R.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
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  givenname: Y. S.
  surname: Lee
  fullname: Lee, Y. S.
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
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  givenname: R. L.
  surname: Greene
  fullname: Greene, R. L.
  organization: Department of Physics, Center for Nanophysics and Advanced Materials, University of Maryland
– sequence: 16
  givenname: L.
  surname: Braicovich
  fullname: Braicovich, L.
  organization: Dipartimento di Fisica, Politecnico di Milano, European Synchrotron Radiation Facility (ESRF)
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  surname: Ghiringhelli
  fullname: Ghiringhelli, G.
  organization: Dipartimento di Fisica, Politecnico di Milano, CNR-SPIN, Politecnico di Milano
– sequence: 18
  givenname: Z. X.
  surname: Shen
  fullname: Shen, Z. X.
  email: zxshen@stanford.edu
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
– sequence: 19
  givenname: T. P.
  surname: Devereaux
  fullname: Devereaux, T. P.
  email: tpd@stanford.edu
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
– sequence: 20
  givenname: W. S.
  surname: Lee
  fullname: Lee, W. S.
  email: leews@stanford.edu
  organization: Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory and Stanford University
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ContentType Journal Article
Copyright Springer Nature Limited 2018
COPYRIGHT 2018 Nature Publishing Group
Copyright Nature Publishing Group Nov 15, 2018
Distributed under a Creative Commons Attribution 4.0 International License
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– notice: COPYRIGHT 2018 Nature Publishing Group
– notice: Copyright Nature Publishing Group Nov 15, 2018
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CorporateAuthor SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
CorporateAuthor_xml – name: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
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Issue 7731
Keywords Resonant Inelastic X-ray Scattering (RIXS)
Charge Dynamics
CuO2 Planes
Acoustic Plasmons
RIXS Spectra
Language English
License Distributed under a Creative Commons Attribution 4.0 International License: http://creativecommons.org/licenses/by/4.0
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Snippet High-temperature copper oxide superconductors consist of stacked CuO 2 planes, with electronic band structures and magnetic excitations that are primarily...
High-temperature copper oxide superconductors consist of stacked CuO planes, with electronic band structures and magnetic excitations that are primarily...
High-temperature copper oxide superconductors consist of stacked CuO.sub.2 planes, with electronic band structures and magnetic excitations that are primarily...
High-temperature copper oxide superconductors consist of stacked CuO2 planes, with electronic band structures and magnetic excitations that are primarily...
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SubjectTerms 639/301/119/995
639/301/119/999
639/766/119/1003
639/766/930/12
Acoustic properties
Acoustics
Aircraft
Brillouin zones
Condensed Matter
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Copper
Copper compounds
Copper oxides
Crystallography
Dispersion
Electric properties
Electrons
Energy
High temperature
High temperature superconductors
Humanities and Social Sciences
Inelastic scattering
Lattice parameters
Lattice vibration
Letter
multidisciplinary
Optics
Periodicity
Physics
Planes
Properties
Resveratrol
Science
Science (multidisciplinary)
Spectrum analysis
Superconductors
X-ray scattering
Title Three-dimensional collective charge excitations in electron-doped copper oxide superconductors
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Volume 563
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