Metal–Organic Gel Leading to Customized Magnetic-Coupling Engineering in Carbon Aerogels for Excellent Radar Stealth and Thermal Insulation Performances

Highlights Fe 3+ , Co 2+ , H 3 BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity. By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnet...

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Vydané v:	Nano-micro letters Ročník 16; číslo 1; s. 42 - 17
Hlavní autori:	Li, Xin, Hu, Ruizhe, Xiong, Zhiqiang, Wang, Dan, Zhang, Zhixia, Liu, Chongbo, Zeng, Xiaojun, Chen, Dezhi, Che, Renchao, Nie, Xuliang
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Singapore Springer Nature Singapore 01.12.2024 Springer Nature B.V SpringerOpen
Predmet:	Aerogels Aircraft performance Carbon Chemical composition Cobalt Collagen Complexation Computer simulation Computer simulation technology Coupling Electromagnetic radiation Engineering Heterometallic magnetic coupling Homogeneity Insulation Iron oxides Kirkendall effect Magnetic properties Metal–organic gels Microwave absorption Multifunctional materials Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Nitrogen Peptides Physical properties Polarity Pyrolysis Radar Radar stealth Stealth technology Thermal insulation Thermal treatment materials Viruses Metal–organic gels Computer simulation technology Radar stealth Thermal insulation Heterometallic magnetic coupling
ISSN:	2311-6706, 2150-5551, 2150-5551
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Abstract	Highlights Fe 3+ , Co 2+ , H 3 BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity. By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnetic particles are obtained. FeCo/Fe 3 O 4 /NC and FeCo/NC aerogels exhibit excellent electromagnetic wave absorbing and radar stealth performances. Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal–organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of − 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe 3 O 4 /NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings.
AbstractList	Metal-organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal-organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of - 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe3O4/NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings.Metal-organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal-organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of - 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe3O4/NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings. Metal-organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal-organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of - 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe O /NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings. Highlights Fe 3+ , Co 2+ , H 3 BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity. By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnetic particles are obtained. FeCo/Fe 3 O 4 /NC and FeCo/NC aerogels exhibit excellent electromagnetic wave absorbing and radar stealth performances. Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal–organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of − 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe 3 O 4 /NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings. Fe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity.By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnetic particles are obtained.FeCo/Fe3O4/NC and FeCo/NC aerogels exhibit excellent electromagnetic wave absorbing and radar stealth performances. Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal–organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of − 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe3O4/NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings. Highlights Fe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity. By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnetic particles are obtained. FeCo/Fe3O4/NC and FeCo/NC aerogels exhibit excellent electromagnetic wave absorbing and radar stealth performances. HighlightsFe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution polarity.By optimizing pyrolysis, two kinds of nitrogen-doped carbon aerogels loaded with virus-shaped and nanospherical magnetic particles are obtained.FeCo/Fe3O4/NC and FeCo/NC aerogels exhibit excellent electromagnetic wave absorbing and radar stealth performances.Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal–organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of − 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe3O4/NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings. Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity, tunable shape, and porous structure. Herein, stable metal–organic hydrogels are prepared by regulating the complexation effect, solution polarity and curing speed. Meanwhile, collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination. Subsequently, two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect. FeCo/nitrogen-doped carbon (NC) aerogel demonstrates an ultra-strong microwave absorption of − 85 dB at an ultra-low loading of 5%. After reducing the time taken by atom shifting, a FeCo/Fe 3 O 4 /NC aerogel containing virus-shaped particles is obtained, which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles. Furthermore, both aerogels show excellent thermal insulation property, and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology. The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels, which will enable the development and application of novel and lightweight stealth coatings.
ArticleNumber	42
Author	Xiong, Zhiqiang Zeng, Xiaojun Zhang, Zhixia Che, Renchao Wang, Dan Chen, Dezhi Liu, Chongbo Hu, Ruizhe Nie, Xuliang Li, Xin
Author_xml	– sequence: 1 givenname: Xin surname: Li fullname: Li, Xin organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 2 givenname: Ruizhe surname: Hu fullname: Hu, Ruizhe organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 3 givenname: Zhiqiang surname: Xiong fullname: Xiong, Zhiqiang organization: School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 4 givenname: Dan surname: Wang fullname: Wang, Dan organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 5 givenname: Zhixia surname: Zhang fullname: Zhang, Zhixia organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 6 givenname: Chongbo surname: Liu fullname: Liu, Chongbo email: cbliu2002@163.com organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 7 givenname: Xiaojun surname: Zeng fullname: Zeng, Xiaojun organization: School of Materials Science and Engineering, Jingdezhen Ceramic University – sequence: 8 givenname: Dezhi surname: Chen fullname: Chen, Dezhi organization: Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, School of Environmental and Chemical Engineering, Nanchang Hangkong University – sequence: 9 givenname: Renchao surname: Che fullname: Che, Renchao email: rcche@fudan.edu.cn organization: Laboratory of Advanced Materials, Department of Materials Science and Collaborative Innovation Center of Chemistry for Energy Materials and Collaborative Innovation Center of Chemistry for Energy Materials, Fudan University – sequence: 10 givenname: Xuliang surname: Nie fullname: Nie, Xuliang email: xuliangnie123@163.com organization: College of Chemistry and Materials, Jiangxi Agricultural University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/38047957$$D View this record in MEDLINE/PubMed
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Keywords	Metal–organic gels Computer simulation technology Radar stealth Thermal insulation Heterometallic magnetic coupling
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Snippet	Highlights Fe 3+ , Co 2+ , H 3 BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect... Metal–organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity,... Metal-organic gel (MOG) derived composites are promising multi-functional materials due to their alterable composition, identifiable chemical homogeneity,... HighlightsFe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and... Fe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and solution... Highlights Fe3+, Co2+, H3BTC, and collagen peptide are used to achieve a one-step assembly of stable FeCo-MOG/CP by manipulating the complexation effect and...
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SubjectTerms	Aerogels Aircraft performance Carbon Chemical composition Cobalt Collagen Complexation Computer simulation Computer simulation technology Coupling Electromagnetic radiation Engineering Heterometallic magnetic coupling Homogeneity Insulation Iron oxides Kirkendall effect Magnetic properties Metal–organic gels Microwave absorption Multifunctional materials Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Nitrogen Peptides Physical properties Polarity Pyrolysis Radar Radar stealth Stealth technology Thermal insulation Thermal treatment materials Viruses
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Title	Metal–Organic Gel Leading to Customized Magnetic-Coupling Engineering in Carbon Aerogels for Excellent Radar Stealth and Thermal Insulation Performances
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