Hydrogen Bond-Assisted Ultra-Stable and Fast Aqueous NH4+ Storage

Highlights Zero capacity fading after over 3000 cycles at 1 C. Only 6.4% capacity is lost when rate is increased by 50 times. Diffusion mechanism of formation and fracture of hydrogen bonds is proposed. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage system...

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Vydáno v:	Nano-micro letters Ročník 13; číslo 1; s. 139 - 16
Hlavní autoři:	Zhang, Xikun, Xia, Maoting, Yu, Haoxiang, Zhang, Junwei, Yang, Zhengwei, Zhang, Liyuan, Shu, Jie
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Singapore Springer Nature Singapore 01.12.2021 Springer Nature B.V SpringerOpen
Témata:	Aqueous ammonium ion batteries Aqueous batteries Aqueous solutions Bonded joints Charge transfer Copper hexacyanoferrate Density functional theory Diffusion rate Energy storage Engineering Excellent rate performance Fading Hydrogen bonds Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Pigments Polyanilines Redox reactions Renewable energy Storage batteries Storage systems Ultra-long cycling performance Copper hexacyanoferrate Ultra-long cycling performance Hydrogen bonds Excellent rate performance Aqueous ammonium ion batteries
ISSN:	2311-6706, 2150-5551, 2150-5551
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Abstract	Highlights Zero capacity fading after over 3000 cycles at 1 C. Only 6.4% capacity is lost when rate is increased by 50 times. Diffusion mechanism of formation and fracture of hydrogen bonds is proposed. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH 4 + in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH 4 + insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH 4 + diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH 4 + storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH 4 + storage in cubic PBAs creates a blueprint for fast and sustainable energy storage.
AbstractList	Abstract Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4 + in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH4 + insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH4 + diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH4 + storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH4 + storage in cubic PBAs creates a blueprint for fast and sustainable energy storage. Highlights Zero capacity fading after over 3000 cycles at 1 C. Only 6.4% capacity is lost when rate is increased by 50 times. Diffusion mechanism of formation and fracture of hydrogen bonds is proposed. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH 4 + in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH 4 + insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH 4 + diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH 4 + storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH 4 + storage in cubic PBAs creates a blueprint for fast and sustainable energy storage. Zero capacity fading after over 3000 cycles at 1 C.Only 6.4% capacity is lost when rate is increased by 50 times.Diffusion mechanism of formation and fracture of hydrogen bonds is proposed. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4+ in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH4+ insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH4+ diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH4+ storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH4+ storage in cubic PBAs creates a blueprint for fast and sustainable energy storage. HighlightsZero capacity fading after over 3000 cycles at 1 C.Only 6.4% capacity is lost when rate is increased by 50 times.Diffusion mechanism of formation and fracture of hydrogen bonds is proposed.Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4+ in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH4+ insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH4+ diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH4+ storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH4+ storage in cubic PBAs creates a blueprint for fast and sustainable energy storage. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH 4 + in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH 4 + insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH 4 + diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH 4 + storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH 4 + storage in cubic PBAs creates a blueprint for fast and sustainable energy storage. Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4+ in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH4+ insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH4+ diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH4+ storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH4+ storage in cubic PBAs creates a blueprint for fast and sustainable energy storage.Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4+ in aqueous solution is always in the process of development. On the basis of density functional theory calculations, the excellent performance of NH4+ insertion in Prussian blue analogues (PBAs) is proposed, especially for copper hexacyanoferrate (CuHCF). In this work, we prove the outstanding cycling and rate performance of CuHCF via electrochemical analyses, delivering no capacity fading during ultra-long cycles of 3000 times and high capacity retention of 93.6% at 50 C. One of main contributions to superior performance from highly reversible redox reaction and structural change is verified during the ammoniation/de-ammoniation progresses. More importantly, we propose the NH4+ diffusion mechanism in CuHCF based on continuous formation and fracture of hydrogen bonds from a joint theoretical and experimental study, which is another essential reason for rapid charge transfer and superior NH4+ storage. Lastly, a full cell by coupling CuHCF cathode and polyaniline anode is constructed to explore the practical application of CuHCF. In brief, the outstanding aqueous NH4+ storage in cubic PBAs creates a blueprint for fast and sustainable energy storage.
ArticleNumber	139
Author	Yang, Zhengwei Zhang, Liyuan Xia, Maoting Zhang, Junwei Zhang, Xikun Shu, Jie Yu, Haoxiang
Author_xml	– sequence: 1 givenname: Xikun surname: Zhang fullname: Zhang, Xikun organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 2 givenname: Maoting surname: Xia fullname: Xia, Maoting organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 3 givenname: Haoxiang surname: Yu fullname: Yu, Haoxiang organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 4 givenname: Junwei surname: Zhang fullname: Zhang, Junwei organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 5 givenname: Zhengwei surname: Yang fullname: Yang, Zhengwei organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 6 givenname: Liyuan surname: Zhang fullname: Zhang, Liyuan organization: School of Materials Science and Chemical Engineering, Ningbo University – sequence: 7 givenname: Jie surname: Shu fullname: Shu, Jie email: shujie@nbu.edu.cn organization: School of Materials Science and Chemical Engineering, Ningbo University
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Keywords	Copper hexacyanoferrate Ultra-long cycling performance Hydrogen bonds Excellent rate performance Aqueous ammonium ion batteries
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PublicationDate	2021-12-01
PublicationDateYYYYMMDD	2021-12-01
PublicationDate_xml	– month: 12 year: 2021 text: 2021-12-01 day: 01
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Snippet	Highlights Zero capacity fading after over 3000 cycles at 1 C. Only 6.4% capacity is lost when rate is increased by 50 times. Diffusion mechanism of formation... Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH 4 + in aqueous solution is... HighlightsZero capacity fading after over 3000 cycles at 1 C.Only 6.4% capacity is lost when rate is increased by 50 times.Diffusion mechanism of formation and... Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4+ in aqueous solution is always... Zero capacity fading after over 3000 cycles at 1 C.Only 6.4% capacity is lost when rate is increased by 50 times.Diffusion mechanism of formation and fracture... Abstract Aqueous ammonium ion batteries are regarded as eco-friendly and sustainable energy storage systems. And applicable host for NH4 + in aqueous solution...
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SubjectTerms	Aqueous ammonium ion batteries Aqueous batteries Aqueous solutions Bonded joints Charge transfer Copper hexacyanoferrate Density functional theory Diffusion rate Energy storage Engineering Excellent rate performance Fading Hydrogen bonds Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Pigments Polyanilines Redox reactions Renewable energy Storage batteries Storage systems Ultra-long cycling performance
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Title	Hydrogen Bond-Assisted Ultra-Stable and Fast Aqueous NH4+ Storage
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