Ionic Conduction in Polymer‐Based Solid Electrolytes

Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, a...

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Vydané v:Advanced science Ročník 10; číslo 10; s. e2201718 - n/a
Hlavní autori: Li, Zhuo, Fu, Jialong, Zhou, Xiaoyan, Gui, Siwei, Wei, Lu, Yang, Hui, Li, Hong, Guo, Xin
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: Germany John Wiley & Sons, Inc 01.04.2023
John Wiley and Sons Inc
Wiley
Predmet:
composite polymer electrolyte
Conductivity
Electrolytes
Energy
interfacial interaction
ionic conduction
Ions
Lithium
Oxygen
polymer electrolyte
Polymers
Review
Reviews
solid‐state batteries
composite polymer electrolyte
interfacial interaction
solid-state batteries
ionic conduction
polymer electrolyte
ISSN:2198-3844, 2198-3844
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Shrnutí:Good safety, high interfacial compatibility, low cost, and facile processability make polymer‐based solid electrolytes promising materials for next‐generation batteries. Key issues related to polymer‐based solid electrolytes, such as synthesis methods, ionic conductivity, and battery architecture, are investigated in past decades. However, mechanistic understanding of the ionic conduction is still lacking, which impedes the design and optimization of polymer‐based solid electrolytes. In this review, the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, are summarized and evaluated. Challenges and strategies for enhancing the ionic conductivity are elaborated, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted. This comprehensive review is especially pertinent for the targeted enhancement of the Li‐ion conductivity of polymer‐based solid electrolytes. This article reviews the ionic conduction mechanisms and optimization strategies of polymer‐based solid electrolytes, including solvent‐free polymer electrolytes, composite polymer electrolytes, and quasi‐solid/gel polymer electrolytes, while the ion‐pair dissociation, ion mobility, polymer relaxation, and interactions at polymer/filler interfaces are highlighted.
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ISSN:2198-3844
2198-3844
DOI:10.1002/advs.202201718