Exploring the atmospheric chemistry of nitrous acid (HONO) at a rural site in Southern China

We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of inst...

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Published in:Atmospheric chemistry and physics Vol. 12; no. 3; pp. 1497 - 1513
Main Authors: Li, X., Brauers, T., Häseler, R., Bohn, B., Fuchs, H., Hofzumahaus, A., Holland, F., Lou, S., Lu, K. D., Rohrer, F., Hu, M., Zeng, L. M., Zhang, Y. H., Garland, R. M., Su, H., Nowak, A., Wiedensohler, A., Takegawa, N., Shao, M., Wahner, A.
Format: Journal Article
Language:English
Published: Katlenburg-Lindau Copernicus GmbH 08.02.2012
Copernicus Publications
Subjects:
Atmospheric chemistry
Instruments (Equipment)
China, People's Rep., Guangdong Prov., Guangzhou
China, People's Rep., Zhu R
ISSN:1680-7324, 1680-7316, 1680-7324
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Abstract We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1–5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO2 to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of ≈200 ppt indicate the existence of a daytime source higher than the OH + NO→HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO (PM) was calculated to be 0.77 ppb h−1 on average. This value compares well to previous measurements in other environments. Our analysis of PM provides evidence that the photolysis of HNO3 adsorbed on ground surfaces contributes to the HONO formation.
AbstractList We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1–5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO 2 to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of ≈200 ppt indicate the existence of a daytime source higher than the OH + NO→HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO ( P M ) was calculated to be 0.77 ppb h −1 on average. This value compares well to previous measurements in other environments. Our analysis of P M provides evidence that the photolysis of HNO 3 adsorbed on ground surfaces contributes to the HONO formation.
We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1-5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO sub(2) to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of approximately 200 ppt indicate the existence of a daytime source higher than the OH + NO arrow right HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO (P sub(M)) was calculated to be 0.77 ppb h super(-1) on average. This value compares well to previous measurements in other environments. Our analysis of P sub(M) provides evidence that the photolysis of HNO sub(3) adsorbed on ground surfaces contributes to the HONO formation.
We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1-5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO.sub.2 to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of ≈200 ppt indicate the existence of a daytime source higher than the OH + NO→HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO (P.sub.M) was calculated to be 0.77 ppb h.sup.-1 on average. This value compares well to previous measurements in other environments. Our analysis of P.sub.M provides evidence that the photolysis of HNO.sub.3 adsorbed on ground surfaces contributes to the HONO formation.
We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1-5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO2 to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of [approximate]200 ppt indicate the existence of a daytime source higher than the OH + NO->HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO (PM ) was calculated to be 0.77 ppb h-1 on average. This value compares well to previous measurements in other environments. Our analysis of PM provides evidence that the photolysis of HNO3 adsorbed on ground surfaces contributes to the HONO formation.
We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks in June 2006. HONO was measured by a LOPAP in-situ instrument which was setup in one of the campaign supersites along with a variety of instruments measuring hydroxyl radicals, trace gases, aerosols, and meteorological parameters. Maximum diurnal HONO mixing ratios of 1–5 ppb were observed during the nights. We found that the nighttime build-up of HONO can be attributed to the heterogeneous NO2 to HONO conversion on ground surfaces and the OH + NO reaction. In addition to elevated nighttime mixing ratios, measured noontime values of ≈200 ppt indicate the existence of a daytime source higher than the OH + NO→HONO reaction. Using the simultaneously recorded OH, NO, and HONO photolysis frequency, a daytime additional source strength of HONO (PM) was calculated to be 0.77 ppb h−1 on average. This value compares well to previous measurements in other environments. Our analysis of PM provides evidence that the photolysis of HNO3 adsorbed on ground surfaces contributes to the HONO formation.
Audience Academic
Author Hu, M.
Nowak, A.
Wahner, A.
Holland, F.
Bohn, B.
Lou, S.
Takegawa, N.
Li, X.
Zhang, Y. H.
Fuchs, H.
Lu, K. D.
Zeng, L. M.
Rohrer, F.
Brauers, T.
Garland, R. M.
Shao, M.
Hofzumahaus, A.
Su, H.
Wiedensohler, A.
Häseler, R.
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Copyright COPYRIGHT 2012 Copernicus GmbH
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Snippet We performed measurements of nitrous acid (HONO) during the PRIDE-PRD2006 campaign in the Pearl River Delta region 60 km north of Guangzhou, China, for 4 weeks...
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Instruments (Equipment)
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Title Exploring the atmospheric chemistry of nitrous acid (HONO) at a rural site in Southern China
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