Solvents and Supporting Electrolytes in the Electrocatalytic Reduction of CO2

Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalys...

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Vydáno v:iScience Ročník 19; s. 135 - 160
Hlavní autoři: König, Maximilian, Vaes, Jan, Klemm, Elias, Pant, Deepak
Médium: Journal Article
Jazyk:angličtina
Vydáno: Elsevier Inc 27.09.2019
Elsevier
Témata:
Catalysis
Electrochemical Engineering
Organic Reaction
Review
Organic Reaction
Catalysis
Electrochemical Engineering
ISSN:2589-0042, 2589-0042
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Abstract Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed. [Display omitted] Catalysis; Organic Reaction; Electrochemical Engineering
AbstractList Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed. : Catalysis; Organic Reaction; Electrochemical Engineering Subject Areas: Catalysis, Organic Reaction, Electrochemical Engineering
Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed. [Display omitted] Catalysis; Organic Reaction; Electrochemical Engineering
Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed.Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed.
Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their concentration, species, buffer capacity, and pH value influence the local reaction conditions and impact the product distribution of the electrocatalyst. Relevant properties of prospective solvents include their basicity, CO2 solubility, conductivity, and toxicity, which affect the CO2RR and the applicability of the solvents. The complexity of an electrochemical system impedes the direct correlation between a single parameter and cell performance indicators such as the Faradaic efficiency; thus the effects of different electrolytes are often not fully comprehended. For an industrial application, a deeper understanding of the effects described in this review can help with the prediction of performance, as well as the development of scalable electrolyzers. In this review, the application of supporting electrolytes and different solvents in the CO2RR reported in the literature are summarized and discussed. Catalysis; Organic Reaction; Electrochemical Engineering
Author Klemm, Elias
Pant, Deepak
Vaes, Jan
König, Maximilian
AuthorAffiliation 1 Institute of Chemical Technology, University of Stuttgart, Pfaffenwaldring 55, 70569 Stuttgart, Germany
2 Separation & Conversion Technology, Flemish Institute for Technological Research (VITO), Boeretang 200, 2400 Mol, Belgium
AuthorAffiliation_xml – name: 1 Institute of Chemical Technology, University of Stuttgart, Pfaffenwaldring 55, 70569 Stuttgart, Germany
– name: 2 Separation & Conversion Technology, Flemish Institute for Technological Research (VITO), Boeretang 200, 2400 Mol, Belgium
Author_xml – sequence: 1
  givenname: Maximilian
  surname: König
  fullname: König, Maximilian
  organization: Institute of Chemical Technology, University of Stuttgart, Pfaffenwaldring 55, 70569 Stuttgart, Germany
– sequence: 2
  givenname: Jan
  surname: Vaes
  fullname: Vaes, Jan
  organization: Separation & Conversion Technology, Flemish Institute for Technological Research (VITO), Boeretang 200, 2400 Mol, Belgium
– sequence: 3
  givenname: Elias
  surname: Klemm
  fullname: Klemm, Elias
  organization: Institute of Chemical Technology, University of Stuttgart, Pfaffenwaldring 55, 70569 Stuttgart, Germany
– sequence: 4
  givenname: Deepak
  orcidid: 0000-0002-1425-9588
  surname: Pant
  fullname: Pant, Deepak
  email: deepak.pant@vito.be, pantonline@gmail.com
  organization: Separation & Conversion Technology, Flemish Institute for Technological Research (VITO), Boeretang 200, 2400 Mol, Belgium
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Snippet Different electrolytes applied in the aqueous electrocatalytic CO2 reduction reaction (CO2RR) considerably influence the catalyst performance. Their...
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SubjectTerms Catalysis
Electrochemical Engineering
Organic Reaction
Review
Title Solvents and Supporting Electrolytes in the Electrocatalytic Reduction of CO2
URI https://dx.doi.org/10.1016/j.isci.2019.07.014
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https://pubmed.ncbi.nlm.nih.gov/PMC6669325
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