A four-coordinate cobalt(II) single-ion magnet with coercivity and a very high energy barrier
Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistabili...
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| Veröffentlicht in: | Nature communications Jg. 7; H. 1; S. 10467 - 8 |
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| Hauptverfasser: | , , , , , , , , , |
| Format: | Journal Article |
| Sprache: | Englisch |
| Veröffentlicht: |
London
Nature Publishing Group UK
17.02.2016
Nature Publishing Group Nature Portfolio |
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| ISSN: | 2041-1723, 2041-1723 |
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| Abstract | Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistability. Attention has thus increasingly focussed on ions with large magnetic anisotropies, especially lanthanides. In spite of large effective energy barriers towards relaxation of the magnetic moment, this has so far not led to a big increase in magnetic bistability. Here we present a comprehensive study of a mononuclear, tetrahedrally coordinated cobalt(II) single-molecule magnet, which has a very high effective energy barrier and displays pronounced magnetic bistability. The combined experimental-theoretical approach enables an in-depth understanding of the origin of these favourable properties, which are shown to arise from a strong ligand field in combination with axial distortion. Our findings allow formulation of clear design principles for improved materials.
Bistable single-molecule magnets potentially allow information storage at extremely high densities. Here, the authors study an air- and moisture-stable mononuclear tetrahedral cobalt(II) complex, elucidating the origin of its pronounced magnetic bistability. |
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| AbstractList | Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistability. Attention has thus increasingly focussed on ions with large magnetic anisotropies, especially lanthanides. In spite of large effective energy barriers towards relaxation of the magnetic moment, this has so far not led to a big increase in magnetic bistability. Here we present a comprehensive study of a mononuclear, tetrahedrally coordinated cobalt(II) single-molecule magnet, which has a very high effective energy barrier and displays pronounced magnetic bistability. The combined experimental-theoretical approach enables an in-depth understanding of the origin of these favourable properties, which are shown to arise from a strong ligand field in combination with axial distortion. Our findings allow formulation of clear design principles for improved materials. Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistability. Attention has thus increasingly focussed on ions with large magnetic anisotropies, especially lanthanides. In spite of large effective energy barriers towards relaxation of the magnetic moment, this has so far not led to a big increase in magnetic bistability. Here we present a comprehensive study of a mononuclear, tetrahedrally coordinated cobalt(II) single-molecule magnet, which has a very high effective energy barrier and displays pronounced magnetic bistability. The combined experimental-theoretical approach enables an in-depth understanding of the origin of these favourable properties, which are shown to arise from a strong ligand field in combination with axial distortion. Our findings allow formulation of clear design principles for improved materials. Bistable single-molecule magnets potentially allow information storage at extremely high densities. Here, the authors study an air- and moisture-stable mononuclear tetrahedral cobalt(II) complex, elucidating the origin of its pronounced magnetic bistability. Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistability. Attention has thus increasingly focussed on ions with large magnetic anisotropies, especially lanthanides. In spite of large effective energy barriers towards relaxation of the magnetic moment, this has so far not led to a big increase in magnetic bistability. Here we present a comprehensive study of a mononuclear, tetrahedrally coordinated cobalt(II) single-molecule magnet, which has a very high effective energy barrier and displays pronounced magnetic bistability. The combined experimental-theoretical approach enables an in-depth understanding of the origin of these favourable properties, which are shown to arise from a strong ligand field in combination with axial distortion. Our findings allow formulation of clear design principles for improved materials.Single-molecule magnets display magnetic bistability of molecular origin, which may one day be exploited in magnetic data storage devices. Recently it was realised that increasing the magnetic moment of polynuclear molecules does not automatically lead to a substantial increase in magnetic bistability. Attention has thus increasingly focussed on ions with large magnetic anisotropies, especially lanthanides. In spite of large effective energy barriers towards relaxation of the magnetic moment, this has so far not led to a big increase in magnetic bistability. Here we present a comprehensive study of a mononuclear, tetrahedrally coordinated cobalt(II) single-molecule magnet, which has a very high effective energy barrier and displays pronounced magnetic bistability. The combined experimental-theoretical approach enables an in-depth understanding of the origin of these favourable properties, which are shown to arise from a strong ligand field in combination with axial distortion. Our findings allow formulation of clear design principles for improved materials. Bistable single-molecule magnets potentially allow information storage at extremely high densities. Here, the authors study an air- and moisture-stable mononuclear tetrahedral cobalt(II) complex, elucidating the origin of its pronounced magnetic bistability. |
| ArticleNumber | 10467 |
| Author | Sarkar, Biprajit Neugebauer, Petr van Slageren, Joris Rechkemmer, Yvonne Atanasov, Mihail van der Meer, Margarethe Neese, Frank Orlita, Milan Hakl, Michael Breitgoff, Frauke D. |
| Author_xml | – sequence: 1 givenname: Yvonne surname: Rechkemmer fullname: Rechkemmer, Yvonne organization: Institut für Physikalische Chemie, Universität Stuttgart – sequence: 2 givenname: Frauke D. surname: Breitgoff fullname: Breitgoff, Frauke D. organization: Institut für Physikalische Chemie, Universität Stuttgart, Present address: Laboratorium für Physikalische Chemie, ETH Zürich, Vladimir-Prelog-Weg 2, 8093 Zürich, Switzerland – sequence: 3 givenname: Margarethe surname: van der Meer fullname: van der Meer, Margarethe organization: Institut für Chemie und Biochemie, Anorganische Chemie, Freie Universität Berlin – sequence: 4 givenname: Mihail surname: Atanasov fullname: Atanasov, Mihail email: mihail.atanasov@cec.mpg.de organization: Max Planck Institute for Chemical Energy Conversion, Institute of General and Inorganic Chemistry, Bulgarian Academy of Sciences – sequence: 5 givenname: Michael surname: Hakl fullname: Hakl, Michael organization: Laboratoire national des champs magnétiques intenses, CNRS-UJF-UPS-INS – sequence: 6 givenname: Milan surname: Orlita fullname: Orlita, Milan organization: Laboratoire national des champs magnétiques intenses, CNRS-UJF-UPS-INS, Institute of Physics, Charles University in Prague – sequence: 7 givenname: Petr surname: Neugebauer fullname: Neugebauer, Petr organization: Institut für Physikalische Chemie, Universität Stuttgart – sequence: 8 givenname: Frank surname: Neese fullname: Neese, Frank organization: Max Planck Institute for Chemical Energy Conversion – sequence: 9 givenname: Biprajit surname: Sarkar fullname: Sarkar, Biprajit email: biprajit.sarkar@fu-berlin.de organization: Institut für Chemie und Biochemie, Anorganische Chemie, Freie Universität Berlin – sequence: 10 givenname: Joris surname: van Slageren fullname: van Slageren, Joris email: slageren@ipc.uni-stuttgart.de organization: Institut für Physikalische Chemie, Universität Stuttgart |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26883902$$D View this record in MEDLINE/PubMed https://hal.science/hal-01992694$$DView record in HAL |
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| ContentType | Journal Article |
| Copyright | The Author(s) 2016 Copyright Nature Publishing Group Feb 2016 Distributed under a Creative Commons Attribution 4.0 International License Copyright © 2016, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. 2016 Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. |
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| Title | A four-coordinate cobalt(II) single-ion magnet with coercivity and a very high energy barrier |
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