Electric control of magnetic exchange in a molecular spin triangle

Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu 3 (saltag)(py) 6 ]ClO 4 spin triangle....

Full description

Saved in:
Bibliographic Details
Published in:Nature communications Vol. 16; no. 1; pp. 6564 - 9
Main Authors: Cini, Alberto, Böhme, Michael, Kintzel, Benjamin, Perfetti, Mauro, Plass, Winfried, Sessoli, Roberta, Fittipaldi, Maria
Format: Journal Article
Language:English
Published: London Nature Publishing Group UK 16.07.2025
Nature Publishing Group
Nature Portfolio
Subjects:
ISSN:2041-1723, 2041-1723
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
Abstract Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu 3 (saltag)(py) 6 ]ClO 4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin–orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin–electric coupling. Electric control of magnetic interactions in a molecular spin-frustrated triangle is demonstrated through experiments and supported by ab initio calculations. This result opens new pathways for scalability by local control of qubit–qubit coupling.
AbstractList Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu (saltag)(py) ]ClO spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin-orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin-electric coupling.
Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu 3 (saltag)(py) 6 ]ClO 4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin–orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin–electric coupling. Electric control of magnetic interactions in a molecular spin-frustrated triangle is demonstrated through experiments and supported by ab initio calculations. This result opens new pathways for scalability by local control of qubit–qubit coupling.
Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu3(saltag)(py)6]ClO4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin-orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin-electric coupling.Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu3(saltag)(py)6]ClO4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin-orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin-electric coupling.
Abstract Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu3(saltag)(py)6]ClO4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin–orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin–electric coupling.
Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism independent of spin-orbit interaction, here we report the detection of a spin-electric effect in the [Cu3(saltag)(py)6]ClO4 spin triangle. The effect is investigated by electron paramagnetic resonance under electric field modulation on single crystals. The anisotropy of the magnetic response to the electric field is addressed, and comprehensive ab initio calculations are performed to elucidate its origin. We demonstrate that when the electric field is applied in the plane of the triangle, the dominant contribution to the observed spin-electric signal arises from a variation of the isotropic exchange interaction. Our combined theoretical and experimental approach demonstrates that, in our system, there is no evidence of antisymmetric exchange (Dzyaloshinskii-Moriya) interaction, confirming that electric-field control of magnetic exchange is achievable in the absence of significant spin–orbit coupling. Moreover, we underscore the crucial role of the bridging ligand, which opens new avenues for chemically optimizing spin–electric coupling. Electric control of magnetic interactions in a molecular spin-frustrated triangle is demonstrated through experiments and supported by ab initio calculations. This result opens new pathways for scalability by local control of qubit–qubit coupling.
ArticleNumber 6564
Author Sessoli, Roberta
Plass, Winfried
Fittipaldi, Maria
Cini, Alberto
Böhme, Michael
Perfetti, Mauro
Kintzel, Benjamin
Author_xml – sequence: 1
  givenname: Alberto
  orcidid: 0000-0003-4040-5531
  surname: Cini
  fullname: Cini, Alberto
  organization: Department of Physics and Astronomy, University of Florence and INSTM UdR
– sequence: 2
  givenname: Michael
  surname: Böhme
  fullname: Böhme, Michael
  organization: Institut für Anorganische und Analytische Chemie, Friedrich-Schiller-Universität Jena, Humboldtstraße 8
– sequence: 3
  givenname: Benjamin
  orcidid: 0009-0005-9761-6390
  surname: Kintzel
  fullname: Kintzel, Benjamin
  organization: Institut für Anorganische und Analytische Chemie, Friedrich-Schiller-Universität Jena, Humboldtstraße 8
– sequence: 4
  givenname: Mauro
  orcidid: 0000-0001-5649-0449
  surname: Perfetti
  fullname: Perfetti, Mauro
  organization: Department of Chemistry “Ugo Schiff”, University of Florence and INSTM UdR
– sequence: 5
  givenname: Winfried
  orcidid: 0000-0003-3473-9682
  surname: Plass
  fullname: Plass, Winfried
  email: sekr.plass@uni-jena.de
  organization: Institut für Anorganische und Analytische Chemie, Friedrich-Schiller-Universität Jena, Humboldtstraße 8
– sequence: 6
  givenname: Roberta
  orcidid: 0000-0003-3783-2700
  surname: Sessoli
  fullname: Sessoli, Roberta
  email: roberta.sessoli@unifi.it
  organization: Department of Chemistry “Ugo Schiff”, University of Florence and INSTM UdR
– sequence: 7
  givenname: Maria
  orcidid: 0000-0002-6254-2003
  surname: Fittipaldi
  fullname: Fittipaldi, Maria
  email: maria.fittipaldi@unifi.it
  organization: Department of Physics and Astronomy, University of Florence and INSTM UdR
BackLink https://www.ncbi.nlm.nih.gov/pubmed/40670338$$D View this record in MEDLINE/PubMed
BookMark eNp9Uk1v1DAUtFARLaV_gAOKxIVLwF9x7BOCqkClSlzgbL3YL9usnHixkwr-Pd5NKW0P9cXWezPjsd-8JEdTnJCQ14y-Z1ToD1kyqdqa8qZWTLK2Vs_ICaeS1azl4uje-Zic5bylZQnDtJQvyLGkqqVC6BPy-SKgm9PgKhenOcVQxb4aYTPhXGr4213DtMFqmCqoxliwS4BU5V0pFFbpBXxFnvcQMp7d7qfk55eLH-ff6qvvXy_PP13VrpFirjV4o5lGbEBxzSkYBsJji33PPIpeK98Z3ntpwCjOQKPuNDaiK0fvGi9OyeWq6yNs7S4NI6Q_NsJgD4WYNhZScR3Qyla4zgvR6R5lrwVw8MhNbyiyTummaH1ctXZLN6J3WN4O4YHow840XNtNvLGMc9UquVd4d6uQ4q8F82zHITsMASaMS7aCC2qokpQV6NtH0G1c0lT-6oBSzMiGF9Sb-5buvPybVQHwFeBSzDlhfwdh1O4zYddM2JIJe8iEVYWkH5HcMMM87IcNQ3iaKlZqLveUEKT_tp9g_QVNyMrV
CitedBy_id crossref_primary_10_1021_jacs_5c10840
Cites_doi 10.1016/j.jmr.2005.08.013
10.1088/0022-3719/2/3/312
10.1002/anie.202017116
10.1038/nnano.2015.22
10.1103/Physics.2.20
10.1103/PhysRevLett.96.107202
10.1038/s41563-019-0314-7
10.1103/PhysRevLett.101.217201
10.1103/PhysRevB.85.085427
10.1103/PhysRevLett.108.247211
10.1038/natrevmats.2016.46
10.1021/ic503095t
10.1021/ic2020034
10.1063/1.449486
10.1038/s41563-018-0275-2
10.1103/PhysRevB.82.045429
10.1038/s41598-023-29840-1
10.1038/s41563-019-0310-y
10.1038/s41467-025-56453-1
10.1038/s41567-021-01355-4
10.1021/jp031064+
10.1103/PhysRevB.82.155446
10.1103/PhysRevB.78.024402
10.1088/0022-3719/1/4/307
10.1038/ncomms1904
10.1021/jp0581126
10.1038/s41563-019-0288-5
10.1021/acs.jctc.9b00532
10.1103/PhysRevB.74.165319
10.1088/0953-8984/22/16/164209
10.1002/chem.201803038
10.1088/0022-3719/9/4/014
10.1039/C8CC06741D
10.1103/PhysRevB.109.214407
10.1021/jacs.9b09101
10.1126/science.1113357
10.1016/0003-9861(74)90298-7
10.1093/nsr/nwaa148
10.1038/30156
10.1103/PhysRevLett.122.037202
10.1039/b508541a
ContentType Journal Article
Copyright The Author(s) 2025
2025. The Author(s).
The Author(s) 2025. This work is published under http://creativecommons.org/licenses/by-nc-nd/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.
The Author(s) 2025 2025
Copyright_xml – notice: The Author(s) 2025
– notice: 2025. The Author(s).
– notice: The Author(s) 2025. This work is published under http://creativecommons.org/licenses/by-nc-nd/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.
– notice: The Author(s) 2025 2025
DBID C6C
AAYXX
CITATION
NPM
3V.
7QL
7QP
7QR
7SN
7SS
7ST
7T5
7T7
7TM
7TO
7X7
7XB
88E
8AO
8FD
8FE
8FG
8FH
8FI
8FJ
8FK
ABUWG
AEUYN
AFKRA
ARAPS
AZQEC
BBNVY
BENPR
BGLVJ
BHPHI
C1K
CCPQU
DWQXO
FR3
FYUFA
GHDGH
GNUQQ
H94
HCIFZ
K9.
LK8
M0S
M1P
M7P
P5Z
P62
P64
PHGZM
PHGZT
PIMPY
PJZUB
PKEHL
PPXIY
PQEST
PQGLB
PQQKQ
PQUKI
PRINS
RC3
SOI
7X8
5PM
DOA
DOI 10.1038/s41467-025-61417-6
DatabaseName SpringerOpen Free (Free internet resource, activated by CARLI)
CrossRef
PubMed
ProQuest Central (Corporate)
Bacteriology Abstracts (Microbiology B)
Calcium & Calcified Tissue Abstracts
Chemoreception Abstracts
Ecology Abstracts
Entomology Abstracts (Full archive)
Environment Abstracts
Immunology Abstracts
Industrial and Applied Microbiology Abstracts (Microbiology A)
Nucleic Acids Abstracts
Oncogenes and Growth Factors Abstracts
Health & Medical Collection
ProQuest Central (purchase pre-March 2016)
Medical Database (Alumni Edition)
ProQuest Pharma Collection
Technology Research Database
ProQuest SciTech Collection
ProQuest Technology Collection
ProQuest Natural Science Journals
Hospital Premium Collection
Hospital Premium Collection (Alumni Edition)
ProQuest Central (Alumni) (purchase pre-March 2016)
ProQuest Central (Alumni)
One Sustainability
ProQuest Central UK/Ireland
Advanced Technologies & Computer Science Collection
ProQuest Central Essentials - QC
Biological Science Collection
ProQuest Central
ProQuest Technology Collection (LUT)
Natural Science Collection
Environmental Sciences and Pollution Management
ProQuest One Community College
ProQuest Central Korea
Engineering Research Database
Proquest Health Research Premium Collection
Health Research Premium Collection (Alumni)
ProQuest Central Student
AIDS and Cancer Research Abstracts
SciTech Premium Collection
ProQuest Health & Medical Complete (Alumni)
Biological Sciences
ProQuest Health & Medical Collection
Medical Database
Biological Science Database
Advanced Technologies & Aerospace Database
ProQuest Advanced Technologies & Aerospace Collection
Biotechnology and BioEngineering Abstracts
Proquest Central Premium
ProQuest One Academic
Publicly Available Content Database
ProQuest Health & Medical Research Collection
ProQuest One Academic Middle East (New)
One Health & Nursing
ProQuest One Academic Eastern Edition (DO NOT USE)
One Applied & Life Sciences
ProQuest One Academic (retired)
ProQuest One Academic UKI Edition
ProQuest Central China
Genetics Abstracts
Environment Abstracts
MEDLINE - Academic
PubMed Central (Full Participant titles)
DOAJ Directory of Open Access Journals
DatabaseTitle CrossRef
PubMed
Publicly Available Content Database
ProQuest Central Student
Oncogenes and Growth Factors Abstracts
ProQuest Advanced Technologies & Aerospace Collection
ProQuest Central Essentials
Nucleic Acids Abstracts
SciTech Premium Collection
ProQuest Central China
Environmental Sciences and Pollution Management
ProQuest One Applied & Life Sciences
ProQuest One Sustainability
Health Research Premium Collection
Natural Science Collection
Health & Medical Research Collection
Biological Science Collection
Chemoreception Abstracts
Industrial and Applied Microbiology Abstracts (Microbiology A)
ProQuest Central (New)
ProQuest Medical Library (Alumni)
Advanced Technologies & Aerospace Collection
ProQuest Biological Science Collection
ProQuest One Academic Eastern Edition
ProQuest Hospital Collection
ProQuest Technology Collection
Health Research Premium Collection (Alumni)
Biological Science Database
Ecology Abstracts
ProQuest Hospital Collection (Alumni)
Biotechnology and BioEngineering Abstracts
Entomology Abstracts
ProQuest Health & Medical Complete
ProQuest One Academic UKI Edition
Engineering Research Database
ProQuest One Academic
Calcium & Calcified Tissue Abstracts
ProQuest One Academic (New)
Technology Collection
Technology Research Database
ProQuest One Academic Middle East (New)
ProQuest Health & Medical Complete (Alumni)
ProQuest Central (Alumni Edition)
ProQuest One Community College
ProQuest One Health & Nursing
ProQuest Natural Science Collection
ProQuest Pharma Collection
ProQuest Central
ProQuest Health & Medical Research Collection
Genetics Abstracts
Health and Medicine Complete (Alumni Edition)
ProQuest Central Korea
Bacteriology Abstracts (Microbiology B)
AIDS and Cancer Research Abstracts
ProQuest SciTech Collection
Advanced Technologies & Aerospace Database
ProQuest Medical Library
Immunology Abstracts
Environment Abstracts
ProQuest Central (Alumni)
MEDLINE - Academic
DatabaseTitleList PubMed

MEDLINE - Academic


Publicly Available Content Database
Database_xml – sequence: 1
  dbid: DOA
  name: DOAJ Directory of Open Access Journals
  url: https://www.doaj.org/
  sourceTypes: Open Website
– sequence: 2
  dbid: NPM
  name: PubMed
  url: http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?db=PubMed
  sourceTypes: Index Database
– sequence: 3
  dbid: PIMPY
  name: Publicly Available Content Database
  url: http://search.proquest.com/publiccontent
  sourceTypes: Aggregation Database
DeliveryMethod fulltext_linktorsrc
Discipline Biology
EISSN 2041-1723
EndPage 9
ExternalDocumentID oai_doaj_org_article_473cbd33b8fe4f83a2ade29f90e1b685
PMC12267645
40670338
10_1038_s41467_025_61417_6
Genre Journal Article
GrantInformation_xml – fundername: Ministero dell'Università e Ricerca - Fondo Italiano per la Scienza (Proj. n. FIS00001045) Ministero dell'Università e Ricerca Dipartimenti di Eccellenza 2023-2027 (DICUS 2.0)
– fundername: EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020)
  grantid: 862893
  funderid: https://doi.org/10.13039/100010661
– fundername: European Cooperation in Science and Technology (COST)
  grantid: 15128
  funderid: https://doi.org/10.13039/501100000921
– fundername: EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 European Research Council (H2020 Excellent Science - European Research Council)
  grantid: 101039890
  funderid: https://doi.org/10.13039/100010663
– fundername: Banca d'Italia (Bank of Italy)
  grantid: NAMASSTE-UNIFI
  funderid: https://doi.org/10.13039/501100003770
– fundername: Istituto Nazionale di Fisica Nucleare Grant NAMASSTE
– fundername: Banca d'Italia (Bank of Italy)
  grantid: NAMASSTE-UNIFI
– fundername: EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020)
  grantid: 862893
– fundername: EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 European Research Council (H2020 Excellent Science - European Research Council)
  grantid: 101039890
– fundername: European Cooperation in Science and Technology (COST)
  grantid: 15128
GroupedDBID ---
0R~
39C
53G
5VS
70F
7X7
88E
8AO
8FE
8FG
8FH
8FI
8FJ
AAHBH
AAJSJ
AASML
ABUWG
ACGFO
ACGFS
ACIWK
ACMJI
ACPRK
ADBBV
ADFRT
ADMLS
ADRAZ
AENEX
AEUYN
AFKRA
AFRAH
AHMBA
ALIPV
ALMA_UNASSIGNED_HOLDINGS
AMTXH
AOIJS
ARAPS
ASPBG
AVWKF
AZFZN
BBNVY
BCNDV
BENPR
BGLVJ
BHPHI
BPHCQ
BVXVI
C6C
CCPQU
DIK
EBLON
EBS
EE.
EMOBN
F5P
FEDTE
FYUFA
GROUPED_DOAJ
HCIFZ
HMCUK
HVGLF
HYE
HZ~
KQ8
LGEZI
LK8
LOTEE
M1P
M7P
M~E
NADUK
NAO
NXXTH
O9-
OK1
P2P
P62
PHGZM
PHGZT
PIMPY
PPXIY
PQGLB
PQQKQ
PROAC
PSQYO
RNS
RNT
RNTTT
RPM
SNYQT
SV3
TSG
UKHRP
AAYXX
AFFHD
CITATION
PJZUB
NPM
3V.
7QL
7QP
7QR
7SN
7SS
7ST
7T5
7T7
7TM
7TO
7XB
8FD
8FK
AZQEC
C1K
DWQXO
FR3
GNUQQ
H94
K9.
M48
P64
PKEHL
PQEST
PQUKI
PRINS
RC3
SOI
7X8
PUEGO
5PM
ID FETCH-LOGICAL-c543t-8ad9818ee5a62820a91a3de7eff1de3f86db92fd49a9621a8e8b8e53b1a8dc5d3
IEDL.DBID DOA
ISICitedReferencesCount 1
ISICitedReferencesURI http://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestLinkType=CitingArticles&DestApp=WOS_CPL&KeyUT=001530788700013&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D
ISSN 2041-1723
IngestDate Fri Oct 03 12:53:44 EDT 2025
Tue Nov 04 02:03:58 EST 2025
Tue Aug 26 09:01:09 EDT 2025
Tue Oct 07 07:24:01 EDT 2025
Wed Jul 23 01:41:27 EDT 2025
Sat Nov 29 07:35:14 EST 2025
Tue Nov 18 21:08:58 EST 2025
Thu Jul 17 02:06:27 EDT 2025
IsDoiOpenAccess true
IsOpenAccess true
IsPeerReviewed true
IsScholarly true
Issue 1
Language English
License 2025. The Author(s).
Open Access This article is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License, which permits any non-commercial use, sharing, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if you modified the licensed material. You do not have permission under this licence to share adapted material derived from this article or parts of it. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by-nc-nd/4.0/.
LinkModel DirectLink
MergedId FETCHMERGED-LOGICAL-c543t-8ad9818ee5a62820a91a3de7eff1de3f86db92fd49a9621a8e8b8e53b1a8dc5d3
Notes ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 14
content type line 23
ORCID 0000-0003-3473-9682
0000-0001-5649-0449
0000-0002-6254-2003
0000-0003-4040-5531
0009-0005-9761-6390
0000-0003-3783-2700
OpenAccessLink https://doaj.org/article/473cbd33b8fe4f83a2ade29f90e1b685
PMID 40670338
PQID 3230619452
PQPubID 546298
PageCount 9
ParticipantIDs doaj_primary_oai_doaj_org_article_473cbd33b8fe4f83a2ade29f90e1b685
pubmedcentral_primary_oai_pubmedcentral_nih_gov_12267645
proquest_miscellaneous_3230906401
proquest_journals_3230619452
pubmed_primary_40670338
crossref_primary_10_1038_s41467_025_61417_6
crossref_citationtrail_10_1038_s41467_025_61417_6
springer_journals_10_1038_s41467_025_61417_6
PublicationCentury 2000
PublicationDate 2025-07-16
PublicationDateYYYYMMDD 2025-07-16
PublicationDate_xml – month: 07
  year: 2025
  text: 2025-07-16
  day: 16
PublicationDecade 2020
PublicationPlace London
PublicationPlace_xml – name: London
– name: England
PublicationTitle Nature communications
PublicationTitleAbbrev Nat Commun
PublicationTitleAlternate Nat Commun
PublicationYear 2025
Publisher Nature Publishing Group UK
Nature Publishing Group
Nature Portfolio
Publisher_xml – name: Nature Publishing Group UK
– name: Nature Publishing Group
– name: Nature Portfolio
References B Kintzel (61417_CR31) 2021; 60
CA Bates (61417_CR36) 1969; 2
MF Islam (61417_CR14) 2010; 82
BO Roos (61417_CR43) 2004; 108
NA Spaldin (61417_CR1) 2005; 309
LN Bulaevskii (61417_CR15) 2008; 78
61417_CR37
J Van Slageren (61417_CR7) 2019; 18
S Ferrer (61417_CR21) 2012; 51
B Kintzel (61417_CR32) 2018; 54
AE Reed (61417_CR41) 1985; 83
M Fittipaldi (61417_CR30) 2019; 18
61417_CR39
KY Choi (61417_CR22) 2006; 96
D Khomskii (61417_CR2) 2009; 2
M Fiebig (61417_CR4) 2016; 1
NA Spaldin (61417_CR6) 2019; 18
F le Mardelé (61417_CR19) 2025; 16
AK Boudalis (61417_CR25) 2018; 24
A Maisuradze (61417_CR29) 2012; 108
JF Nossa (61417_CR20) 2012; 85
CA Bates (61417_CR35) 1968; 1
M Trif (61417_CR13) 2010; 82
S Stoll (61417_CR34) 2006; 178
DI Khomskii (61417_CR16) 2010; 22
F Matsukura (61417_CR3) 2015; 10
VN Golovach (61417_CR8) 2006; 74
MF Islam (61417_CR18) 2024; 109
61417_CR23
61417_CR45
M Trif (61417_CR12) 2008; 101
BO Roos (61417_CR44) 2005; 109
J Robert (61417_CR26) 2020; 141
F Weigend (61417_CR40) 2005; 7
M Lewkowitz (61417_CR27) 2023; 13
J Peisach (61417_CR38) 1974; 165
J Liu (61417_CR24) 2019; 122
Z Liu (61417_CR9) 2020; 7
BE Kane (61417_CR11) 1998; 393
P Wysling (61417_CR28) 1975; 9
J Liu (61417_CR10) 2021; 17
DI Khomskii (61417_CR17) 2012; 3
I Fdez. Galván (61417_CR42) 2019; 15
61417_CR5
ET Spielberg (61417_CR33) 2015; 54
References_xml – volume: 178
  start-page: 42
  year: 2006
  ident: 61417_CR34
  publication-title: J. Magn. Reson.
  doi: 10.1016/j.jmr.2005.08.013
– volume: 2
  start-page: 476
  year: 1969
  ident: 61417_CR36
  publication-title: J. Phys. C: Solid State Phys.
  doi: 10.1088/0022-3719/2/3/312
– volume: 60
  start-page: 8832
  year: 2021
  ident: 61417_CR31
  publication-title: Angew. Chem. Int. Ed.
  doi: 10.1002/anie.202017116
– volume: 10
  start-page: 209
  year: 2015
  ident: 61417_CR3
  publication-title: Nat. Nanotechnol.
  doi: 10.1038/nnano.2015.22
– volume: 2
  start-page: 20
  year: 2009
  ident: 61417_CR2
  publication-title: Physics
  doi: 10.1103/Physics.2.20
– volume: 96
  start-page: 107202
  year: 2006
  ident: 61417_CR22
  publication-title: Phys. Rev. Lett.
  doi: 10.1103/PhysRevLett.96.107202
– volume: 18
  start-page: 300
  year: 2019
  ident: 61417_CR7
  publication-title: Nat. Mater.
  doi: 10.1038/s41563-019-0314-7
– ident: 61417_CR45
– volume: 101
  start-page: 217201
  year: 2008
  ident: 61417_CR12
  publication-title: Phys. Rev. Lett.
  doi: 10.1103/PhysRevLett.101.217201
– ident: 61417_CR39
– volume: 85
  start-page: 085427
  year: 2012
  ident: 61417_CR20
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.85.085427
– volume: 108
  start-page: 247211
  year: 2012
  ident: 61417_CR29
  publication-title: Phys. Rev. Lett.
  doi: 10.1103/PhysRevLett.108.247211
– volume: 1
  start-page: 16046
  year: 2016
  ident: 61417_CR4
  publication-title: Nat. Rev. Mater.
  doi: 10.1038/natrevmats.2016.46
– volume: 54
  start-page: 3432
  year: 2015
  ident: 61417_CR33
  publication-title: Inorg. Chem.
  doi: 10.1021/ic503095t
– volume: 51
  start-page: 985
  year: 2012
  ident: 61417_CR21
  publication-title: Inorg. Chem.
  doi: 10.1021/ic2020034
– volume: 83
  start-page: 735
  year: 1985
  ident: 61417_CR41
  publication-title: J. Chem. Phys.
  doi: 10.1063/1.449486
– volume: 18
  start-page: 203
  year: 2019
  ident: 61417_CR6
  publication-title: Nat. Mater.
  doi: 10.1038/s41563-018-0275-2
– volume: 82
  start-page: 045429
  year: 2010
  ident: 61417_CR13
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.82.045429
– volume: 13
  start-page: 2769
  year: 2023
  ident: 61417_CR27
  publication-title: Sci. Rep.
  doi: 10.1038/s41598-023-29840-1
– ident: 61417_CR5
  doi: 10.1038/s41563-019-0310-y
– volume: 16
  start-page: 1198
  year: 2025
  ident: 61417_CR19
  publication-title: Nat. Commun.
  doi: 10.1038/s41467-025-56453-1
– ident: 61417_CR37
– volume: 17
  start-page: 1205
  year: 2021
  ident: 61417_CR10
  publication-title: Nat. Phys.
  doi: 10.1038/s41567-021-01355-4
– volume: 108
  start-page: 2851
  year: 2004
  ident: 61417_CR43
  publication-title: J. Phys. Chem. A
  doi: 10.1021/jp031064+
– volume: 82
  start-page: 155446
  year: 2010
  ident: 61417_CR14
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.82.155446
– volume: 78
  start-page: 024402
  year: 2008
  ident: 61417_CR15
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.78.024402
– volume: 1
  start-page: 877
  year: 1968
  ident: 61417_CR35
  publication-title: J. Phys. C: Solid State Phys.
  doi: 10.1088/0022-3719/1/4/307
– volume: 3
  year: 2012
  ident: 61417_CR17
  publication-title: Nat. Commun.
  doi: 10.1038/ncomms1904
– volume: 109
  start-page: 6575
  year: 2005
  ident: 61417_CR44
  publication-title: J. Phys. Chem. A
  doi: 10.1021/jp0581126
– volume: 18
  start-page: 329
  year: 2019
  ident: 61417_CR30
  publication-title: Nat. Mater.
  doi: 10.1038/s41563-019-0288-5
– volume: 15
  start-page: 5925
  year: 2019
  ident: 61417_CR42
  publication-title: J. Chem. Theory Comput
  doi: 10.1021/acs.jctc.9b00532
– ident: 61417_CR23
– volume: 74
  start-page: 165319
  year: 2006
  ident: 61417_CR8
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.74.165319
– volume: 22
  start-page: 164209
  year: 2010
  ident: 61417_CR16
  publication-title: J. Phys. Cond. Matter
  doi: 10.1088/0953-8984/22/16/164209
– volume: 24
  start-page: 14896
  year: 2018
  ident: 61417_CR25
  publication-title: Chem. Eur. J.
  doi: 10.1002/chem.201803038
– volume: 9
  start-page: 635
  year: 1975
  ident: 61417_CR28
  publication-title: J. Phys. C: Solid State Phys.
  doi: 10.1088/0022-3719/9/4/014
– volume: 54
  start-page: 12934
  year: 2018
  ident: 61417_CR32
  publication-title: Chem. Commun.
  doi: 10.1039/C8CC06741D
– volume: 109
  start-page: 214407
  year: 2024
  ident: 61417_CR18
  publication-title: Phys. Rev. B
  doi: 10.1103/PhysRevB.109.214407
– volume: 141
  start-page: 19765
  year: 2020
  ident: 61417_CR26
  publication-title: J. Am. Chem. Soc.
  doi: 10.1021/jacs.9b09101
– volume: 309
  start-page: 391
  year: 2005
  ident: 61417_CR1
  publication-title: Science
  doi: 10.1126/science.1113357
– volume: 165
  start-page: 691
  year: 1974
  ident: 61417_CR38
  publication-title: Arch. Biochem. Biophys.
  doi: 10.1016/0003-9861(74)90298-7
– volume: 7
  start-page: 1557
  year: 2020
  ident: 61417_CR9
  publication-title: Natl Sci. Rev.
  doi: 10.1093/nsr/nwaa148
– volume: 393
  start-page: 133
  year: 1998
  ident: 61417_CR11
  publication-title: Nature
  doi: 10.1038/30156
– volume: 122
  start-page: 37202
  year: 2019
  ident: 61417_CR24
  publication-title: Phys. Rev. Lett.
  doi: 10.1103/PhysRevLett.122.037202
– volume: 7
  start-page: 3297
  year: 2005
  ident: 61417_CR40
  publication-title: Phys. Chem. Chem. Phys.
  doi: 10.1039/b508541a
SSID ssj0000391844
Score 2.4833505
Snippet Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a mechanism...
Abstract Spin-electric effects are crucial for quantum technologies, offering several advantages over standard magnetic field-based spin control. Seeking a...
SourceID doaj
pubmedcentral
proquest
pubmed
crossref
springer
SourceType Open Website
Open Access Repository
Aggregation Database
Index Database
Enrichment Source
Publisher
StartPage 6564
SubjectTerms 119/118
639/638/263
639/638/911
639/766/119/997
Anisotropy
Copper
Crystals
Electric control
Electric fields
Electron paramagnetic resonance
Electron spin resonance
Electrons
Exchanging
Humanities and Social Sciences
Investigations
Ligands
Magnetic fields
multidisciplinary
Qubits (quantum computing)
Science
Science (multidisciplinary)
Single crystals
Spectrum analysis
Spin-orbit interactions
Symmetry
SummonAdditionalLinks – databaseName: Biological Science Database
  dbid: M7P
  link: http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwpV1Jb9QwFH6CAlIv7IVAQUbiBlHj2HHsE6KoFaeqB5B6s7wOI7XJMJlW8O-xHSfVsPTC1Xak57zFz37LB_C20Rp7QVVJsaElJUyV2ghRBtGxGqum0p4nsIn25ISfnYnT_OA25LTKySYmQ217E9_ID0j0lcONu6k_rL6XETUqRlczhMZtuBO7JJCUunc6v7HE7uec0lwrUxF-MNBkGSKGaziXgoFmW-dRatv_N1_zz5TJ3-Km6Tg6fvC_G3kI97Mjij6OkvMIbrnuMdwboSl_PoHDo4SPszQoJ7Oj3qMLtehi0SNyP8aCYbTskEIXE8QuGlZhIAKBdItz9xS-Hh99-fS5zHgLpWko2ZRcWRHOb-caxcJNrFICK2Jd67zH1hHPmdWi9pYKJViNFXdcc9eQwFNuTWPJHux0feeeA-IRwKP2Yb4NLqEioqE6XASpUtap1lQF4OmvS5ObkUdMjHOZguKEy5FTMnBKJk5JVsC7-ZvV2IrjxtWHkZnzythGOw3064XMWilpS4y2hGjuHfWcqDrQVwsvKoc1400B-xMPZdbtQV4zsIA383TQyhhqUZ3rL8c1IgZJcQHPRsmZKaGxNIoQXgDfkqktUrdnuuW31PkbB2e5ZTTQ9X4Sv2u6_v0vXty8jZewW0eNiO1C2T7sbNaX7hXcNVeb5bB-nVTqF7O9J-k
  priority: 102
  providerName: ProQuest
Title Electric control of magnetic exchange in a molecular spin triangle
URI https://link.springer.com/article/10.1038/s41467-025-61417-6
https://www.ncbi.nlm.nih.gov/pubmed/40670338
https://www.proquest.com/docview/3230619452
https://www.proquest.com/docview/3230906401
https://pubmed.ncbi.nlm.nih.gov/PMC12267645
https://doaj.org/article/473cbd33b8fe4f83a2ade29f90e1b685
Volume 16
WOSCitedRecordID wos001530788700013&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D
hasFullText 1
inHoldings 1
isFullTextHit
isPrint
journalDatabaseRights – providerCode: PRVAON
  databaseName: DOAJ Directory of Open Access Journals
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: DOA
  dateStart: 20150101
  isFulltext: true
  titleUrlDefault: https://www.doaj.org/
  providerName: Directory of Open Access Journals
– providerCode: PRVHPJ
  databaseName: ROAD: Directory of Open Access Scholarly Resources
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: M~E
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: https://road.issn.org
  providerName: ISSN International Centre
– providerCode: PRVPQU
  databaseName: Advanced Technologies & Aerospace Database
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: P5Z
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: https://search.proquest.com/hightechjournals
  providerName: ProQuest
– providerCode: PRVPQU
  databaseName: Biological Science Database
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: M7P
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: http://search.proquest.com/biologicalscijournals
  providerName: ProQuest
– providerCode: PRVPQU
  databaseName: Health & Medical Collection
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: 7X7
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: https://search.proquest.com/healthcomplete
  providerName: ProQuest
– providerCode: PRVPQU
  databaseName: ProQuest Central
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: BENPR
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: https://www.proquest.com/central
  providerName: ProQuest
– providerCode: PRVPQU
  databaseName: Publicly Available Content Database
  customDbUrl:
  eissn: 2041-1723
  dateEnd: 99991231
  omitProxy: false
  ssIdentifier: ssj0000391844
  issn: 2041-1723
  databaseCode: PIMPY
  dateStart: 20100101
  isFulltext: true
  titleUrlDefault: http://search.proquest.com/publiccontent
  providerName: ProQuest
link http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwrV1Lb9QwEB5BAYkL4k1KuzISN4gax3ZiH1m0FRxYRQikhYtlx3a7UputulsE_75jJ7t0KY8LlxxsRxrNjD0zmscH8FJYS4PiJue05Tlnlcltq1SOquMsNaKwQSawiXo6lbOZaq5AfcWasH48cM-4A16z1jrGrAyeB8lMaZwvVVCFp7aSaXopej1Xgqn0BjOFoQsfumQKJg-WPL0JEb0VLRI-zdWWJUoD-3_nZV4vlvwlY5oM0eF9uDd4kORNT_kDuOG7h3Cnx5T88QjGkwRsM2_JUIVOFoGcmqMudisS_73v9CXzjhhyusbGJcszXIgIHt3RiX8Mnw8nn96-yweghLwVnK1yaZxCw-u9MBWGUIVR1DDnax8CdZ4FWTmryuC4MqoqqZFeWukFQ2FI1wrHnsBOt-j8MyAyIm-UAfdr9OUMU4JbjOC4Qa6bui0yoGum6XaYIh7BLE50ymYzqXtGa2S0TozWVQavNv-c9TM0_np6HGWxORnnX6cF1Ao9aIX-l1ZksLeWpB4u5VKzGG5RxUWZwYvNNl6nmCMxnV9c9GdUzG7SDJ72gt9QwmNPE4b0GcgtldgidXunmx-nkd0Uvdy64kjX67X2_KTrz7zY_R-8eA53y6j2cRpotQc7q_MLvw-322-r-fJ8BDfrWZ2-cgS3xpNp83GU7tIolsE2-G3EV9xp3n9ovlwCZY4h2w
linkProvider Directory of Open Access Journals
linkToHtml http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMw1V1Jb9QwFH4qBQQX9iVQwEhwgqiJ7ST2ASEKrVq1jHooUm_G6zBSmwwzU6B_it-I7SzVsPTWA9fYiV6Sz2_x83sfwItCqdxxKlOaa5pSUspUac5TDx2jcllkyrFINlGNRuzwkO-vwM--FiYcq-x1YlTUptFhj3ydBF_ZR9wFfjv9mgbWqJBd7Sk0Wljs2tPvPmSbv9n54P_vS4y3Ng_eb6cdq0CqC0oWKZOGeytlbSFLH29kkueSGFtZ53JjiWOlURw7Q7nkJc4ls0wxWxAvOTO6MMQ_9xJc9m4EZvGo4P6wpxO6rTNKu9qcjLD1OY2aKHDGejvoDUK5ZP8iTcDffNs_j2j-lqeN5m_r5v_24W7Bjc7RRu_alXEbVmx9B6621Jund2FjM_L_TDTqDuujxqFjOa5DUSeyP9qCaDSpkUTHPYUwmk_9hUB0Uo-P7D34dCEvcB9W66a2DwGxQFCCnR-vvMsrCS-o8oEuldJYWeksgbz_y0J3zdYD58eRiEl_wkSLDOGRISIyRJnAq-Geadtq5NzZGwE8w8zQJjxeaGZj0WkdQSuilSFEMWepY0RiLx_mjmc2VyUrEljrMSM63TUXZ4BJ4Pkw7LVOSCXJ2jYn7RweksB5Ag9apA6S0FD6RQhLgC1heEnU5ZF68iV2Ns99MFCV1Mv1uof7mVz__haPzn-NZ3Bt--DjntjbGe0-hus4rMbQGrVcg9XF7MQ-gSv622Iynz2NyxnB54teBr8AWvSHpA
linkToPdf http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMw1V1Lb9QwEB6V8hAX3o9AASPBiUYbx05iHxCitCuqotUeQOrN2LG9rNQmy2YL9K_x67CdR7U8euuBq-1E4_jzjCeemQ_gRaYUtpzKmOKSxpTkMlYl57GDjlZYZomyLJBNFJMJOzzk0w342efC-LDKXicGRa3r0v8jHxF_VnYed5aObBcWMd0dv1l8jT2DlL9p7ek0WogcmNPvzn1rXu_vurV-mabjvY_v3scdw0BcZpSsYiY1dxbLmEzmzvdIJMeSaFMYa7E2xLJcK55aTbnkeYolM0wxkxE3C6bLTBP33ktwufBFy0PY4HT4v-MrrzNKuzydhLBRQ4NW8vyxziY645Cv2cJAGfC3c-6f4Zq_3dkGUzi--T9_xFtwozuAo7ftjrkNG6a6A1dbSs7Tu7CzF3iB5iXqgvhRbdGxnFU-2ROZH22iNJpXSKLjnloYNQvX4AlQqtmRuQefLmQC92GzqivzEBDzxCWpdf2FOwpLwjOqnANMpdRGFmUSAe5XXJRdEXbPBXIkQjAAYaJFiXAoEQElIo_g1fDMoi1Bcu7oHQ-kYaQvHx4a6uVMdNpI0IKUShOimDXUMiJTJ1_KLU8MVjnLItjq8SM6ndaIM_BE8HzodtrIXzHJytQn7RjuL4dxBA9a1A6SUJ8SRgiLgK3heU3U9Z5q_iVUPMfOSShy6uTa7qF_Jte_v8Wj86fxDK459IsP-5ODx3A99RvTV0zNt2BztTwxT-BK-W01b5ZPw85G8Pmid8EvsBeQYQ
openUrl ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Electric+control+of+magnetic+exchange+in+a+molecular+spin+triangle&rft.jtitle=Nature+communications&rft.au=Alberto+Cini&rft.au=Michael+B%C3%B6hme&rft.au=Benjamin+Kintzel&rft.au=Mauro+Perfetti&rft.date=2025-07-16&rft.pub=Nature+Portfolio&rft.eissn=2041-1723&rft.volume=16&rft.issue=1&rft.spage=1&rft.epage=9&rft_id=info:doi/10.1038%2Fs41467-025-61417-6&rft.externalDBID=DOA&rft.externalDocID=oai_doaj_org_article_473cbd33b8fe4f83a2ade29f90e1b685
thumbnail_l http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=2041-1723&client=summon
thumbnail_m http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=2041-1723&client=summon
thumbnail_s http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=2041-1723&client=summon