A fast-charging/discharging and long-term stable artificial electrode enabled by space charge storage mechanism

Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electr...

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Vydáno v:Nature communications Ročník 15; číslo 1; s. 3778 - 12
Hlavní autoři: Zhao, Linyi, Wang, Tiansheng, Zuo, Fengkai, Ju, Zhengyu, Li, Yuhao, Li, Qiang, Zhu, Yue, Li, Hongsen, Yu, Guihua
Médium: Journal Article
Jazyk:angličtina
Vydáno: London Nature Publishing Group UK 06.05.2024
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ISSN:2041-1723, 2041-1723
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Abstract Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/Li x M, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li 2 O electrode is able to be charged/discharged to 126 mAh g −1 in 6 s at a high current density of up to 50 A g −1 , and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g −1 , with a mass-loading of ~2.5 mg cm −2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries. Lithium-ion batteries with fast-charging properties are urgently needed for wide adoption of electric vehicles. Here, the authors show a fast charging/discharging and long-term stable electrode made from a mixed electronic/ionic conductor material enabled by a space charge mechanism.
AbstractList Abstract Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/LixM, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li2O electrode is able to be charged/discharged to 126 mAh g−1 in 6 s at a high current density of up to 50 A g−1, and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g−1, with a mass-loading of ~2.5 mg cm−2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries.
Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/LixM, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li2O electrode is able to be charged/discharged to 126 mAh g−1 in 6 s at a high current density of up to 50 A g−1, and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g−1, with a mass-loading of ~2.5 mg cm−2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries. Lithium-ion batteries with fast-charging properties are urgently needed for wide adoption of electric vehicles. Here, the authors show a fast charging/discharging and long-term stable electrode made from a mixed electronic/ionic conductor material enabled by a space charge mechanism.
Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/Li x M, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li 2 O electrode is able to be charged/discharged to 126 mAh g −1 in 6 s at a high current density of up to 50 A g −1 , and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g −1 , with a mass-loading of ~2.5 mg cm −2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries. Lithium-ion batteries with fast-charging properties are urgently needed for wide adoption of electric vehicles. Here, the authors show a fast charging/discharging and long-term stable electrode made from a mixed electronic/ionic conductor material enabled by a space charge mechanism.
Lithium-ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/LixM, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li2O electrode is able to be charged/discharged to 126 mAh g-1 in 6 s at a high current density of up to 50 A g-1, and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g-1, with a mass-loading of ~2.5 mg cm-2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries.Lithium-ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/LixM, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li2O electrode is able to be charged/discharged to 126 mAh g-1 in 6 s at a high current density of up to 50 A g-1, and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g-1, with a mass-loading of ~2.5 mg cm-2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries.
Lithium-ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/Li M, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li O electrode is able to be charged/discharged to 126 mAh g in 6 s at a high current density of up to 50 A g , and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g , with a mass-loading of ~2.5 mg cm of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries.
Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast charging/discharging, long-term stable and high energy charge-storage properties can be realized in an artificial electrode made from a mixed electronic/ionic conductor material (Fe/Li x M, where M = O, F, S, N) enabled by a space charge principle. Particularly, the Fe/Li 2 O electrode is able to be charged/discharged to 126 mAh g −1 in 6 s at a high current density of up to 50 A g −1 , and it also shows stable cycling performance for 30,000 cycles at a current density of 10 A g −1 , with a mass-loading of ~2.5 mg cm −2 of the electrode materials. This study demonstrates the critical role of the space charge storage mechanism in advancing electrochemical energy storage and provides an unconventional perspective for designing high-performance anode materials for lithium-ion batteries.
ArticleNumber 3778
Author Li, Qiang
Wang, Tiansheng
Zuo, Fengkai
Zhu, Yue
Zhao, Linyi
Ju, Zhengyu
Li, Hongsen
Yu, Guihua
Li, Yuhao
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/38710689$$D View this record in MEDLINE/PubMed
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springer_journals_10_1038_s41467_024_48215_2
PublicationCentury 2000
PublicationDate 2024-05-06
PublicationDateYYYYMMDD 2024-05-06
PublicationDate_xml – month: 05
  year: 2024
  text: 2024-05-06
  day: 06
PublicationDecade 2020
PublicationPlace London
PublicationPlace_xml – name: London
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PublicationTitle Nature communications
PublicationTitleAbbrev Nat Commun
PublicationTitleAlternate Nat Commun
PublicationYear 2024
Publisher Nature Publishing Group UK
Nature Publishing Group
Nature Portfolio
Publisher_xml – name: Nature Publishing Group UK
– name: Nature Publishing Group
– name: Nature Portfolio
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Snippet Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast...
Lithium-ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that fast...
Abstract Lithium‐ion batteries with fast-charging/discharging properties are urgently needed for the mass adoption of electric vehicles. Here, we show that...
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SubjectTerms 639/301
639/925
Anodes
Charging
Conductors
Current density
Discharge
Electric vehicles
Electrochemistry
Electrode materials
Electrodes
Energy charge
Energy storage
Humanities and Social Sciences
Lithium
Lithium oxides
Lithium-ion batteries
multidisciplinary
Rechargeable batteries
Science
Science (multidisciplinary)
Space charge
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Title A fast-charging/discharging and long-term stable artificial electrode enabled by space charge storage mechanism
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