Carrier dynamics in Landau-quantized graphene featuring strong Auger scattering

The energy spectrum of common two-dimensional electron gases consists of a harmonic (that is, equidistant) ladder of Landau levels, thus preventing the possibility of optically addressing individual transitions. In graphene, however, owing to its non-harmonic spectrum, individual levels can be addre...

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Veröffentlicht in:	Nature physics Jg. 11; H. 1; S. 75 - 81
Hauptverfasser:	Mittendorff, Martin, Wendler, Florian, Malic, Ermin, Knorr, Andreas, Orlita, Milan, Potemski, Marek, Berger, Claire, de Heer, Walter A., Schneider, Harald, Helm, Manfred, Winnerl, Stephan
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	London Nature Publishing Group UK 01.01.2015 Nature Publishing Group Nature Publishing Group [2005-....]
Schlagworte:	140/125 639/624/399/918 639/766/119/995 639/766/119/997 Atomic Augers Carriers Classical and Continuum Physics Complex Systems Condensed Matter Condensed Matter Physics Depletion Dynamics Graphene Ladders Magnetic fields Materials science Mathematical and Computational Physics Mesoscopic Systems and Quantum Hall Effect Molecular Optical and Plasma Physics Optical pumping Physics Quantum physics Scattering Theoretical Two dimensional
ISSN:	1745-2473, 1745-2481
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Abstract	The energy spectrum of common two-dimensional electron gases consists of a harmonic (that is, equidistant) ladder of Landau levels, thus preventing the possibility of optically addressing individual transitions. In graphene, however, owing to its non-harmonic spectrum, individual levels can be addressed selectively. Here, we report a time-resolved experiment directly pumping discrete Landau levels in graphene. Energetically degenerate Landau-level transitions from n = −1 to n = 0 and from n = 0 to n = 1 are distinguished by applying circularly polarized THz light. An analysis based on a microscopic theory shows that the zeroth Landau level is actually depleted by strong Auger scattering, even though it is optically pumped at the same time. The surprisingly strong electron–electron interaction responsible for this effect is directly evidenced through a sign reversal of the pump–probe signal. Landau levels in graphene are not equidistant so that transitions between them can be individually probed. Time-resolved optical pumping experiments reveal strong electron–electron scattering resulting in an Auger-depleted zeroth order Landau level.
AbstractList	The energy spectrum of common two-dimensional electron gases consists of a harmonic (that is, equidistant) ladder of Landau levels, thus preventing the possibility of optically addressing individual transitions. In graphene, however, owing to its non-harmonic spectrum, individual levels can be addressed selectively. Here, we report a time-resolved experiment directly pumping discrete Landau levels in graphene. Energetically degenerate Landau-level transitions from n = -1 to n = 0 and from n = 0 to n = 1 are distinguished by applying circularly polarized THz light. An analysis based on a microscopic theory shows that the zeroth Landau level is actually depleted by strong Auger scattering, even though it is optically pumped at the same time. The surprisingly strong electron-electron interaction responsible for this effect is directly evidenced through a sign reversal of the pump-probe signal. The energy spectrum of common two-dimensional electron gases consists of a harmonic (that is, equidistant) ladder of Landau levels, thus preventing the possibility of optically addressing individual transitions. In graphene, however, owing to its non-harmonic spectrum, individual levels can be addressed selectively. Here, we report a time-resolved experiment directly pumping discrete Landau levels in graphene. Energetically degenerate Landau-level transitions from n = −1 to n = 0 and from n = 0 to n = 1 are distinguished by applying circularly polarized THz light. An analysis based on a microscopic theory shows that the zeroth Landau level is actually depleted by strong Auger scattering, even though it is optically pumped at the same time. The surprisingly strong electron–electron interaction responsible for this effect is directly evidenced through a sign reversal of the pump–probe signal. Landau levels in graphene are not equidistant so that transitions between them can be individually probed. Time-resolved optical pumping experiments reveal strong electron–electron scattering resulting in an Auger-depleted zeroth order Landau level. The energy spectrum of common two-dimensional electron gases consists of a harmonic, i.e. equidistant ladder of Landau levels, thus preventing the possibility to optically address individual transitions. In graphene, however, due to its non-harmonic spectrum, individual levels can be addressed selectively. We report here the first time-resolved experiment directly pumping discrete Landau levels in graphene. Energetically degenerate Landau-level transitions from n =-1 to n = 0 and from n = 0 to n = 1 are distinguished by applying circularly polarized THz light. In agreement with our experimental results, an analysis based on microscopic theory shows that the zeroth Landau level is actually depleted by strong Auger scattering, even though it is optically pumped at the same time. Such a phenomenon has never been observed before in any system to our knowledge. The surprisingly strong electron-electron interaction responsible for this effect is directly evidenced through a sign reversal of the pump-probe signal.
Author	Potemski, Marek Mittendorff, Martin de Heer, Walter A. Malic, Ermin Orlita, Milan Berger, Claire Schneider, Harald Wendler, Florian Knorr, Andreas Helm, Manfred Winnerl, Stephan
Author_xml	– sequence: 1 givenname: Martin surname: Mittendorff fullname: Mittendorff, Martin email: mhm@umd.edu organization: Helmholtz-Zentrum Dresden-Rossendorf, PO Box 510119 01314 Dresden, Germany, Technische Universität Dresden, Present address: University of Maryland, College Park, Maryland 20742, USA – sequence: 2 givenname: Florian surname: Wendler fullname: Wendler, Florian organization: Technische Universität Berlin, Hardenbergstraße 36 10623 Berlin, Germany – sequence: 3 givenname: Ermin surname: Malic fullname: Malic, Ermin organization: Technische Universität Berlin, Hardenbergstraße 36 10623 Berlin, Germany – sequence: 4 givenname: Andreas surname: Knorr fullname: Knorr, Andreas organization: Technische Universität Berlin, Hardenbergstraße 36 10623 Berlin, Germany – sequence: 5 givenname: Milan surname: Orlita fullname: Orlita, Milan organization: Laboratoire National des Champs Magnétiques Intenses, CNRS-UJF-UPS-INSA 38042 Grenoble, France, Charles University Faculty of Mathematics and Physics, Ke Karlovu 5 121 16 Praha, Czech Republic – sequence: 6 givenname: Marek surname: Potemski fullname: Potemski, Marek organization: Laboratoire National des Champs Magnétiques Intenses, CNRS-UJF-UPS-INSA 38042 Grenoble, France – sequence: 7 givenname: Claire surname: Berger fullname: Berger, Claire organization: Georgia Institute of Technology, CNRS — Institut Néel – sequence: 8 givenname: Walter A. surname: de Heer fullname: de Heer, Walter A. organization: Georgia Institute of Technology, Department of Physics, King Abdulaziz University – sequence: 9 givenname: Harald surname: Schneider fullname: Schneider, Harald organization: Helmholtz-Zentrum Dresden-Rossendorf, PO Box 510119 01314 Dresden, Germany – sequence: 10 givenname: Manfred surname: Helm fullname: Helm, Manfred organization: Helmholtz-Zentrum Dresden-Rossendorf, PO Box 510119 01314 Dresden, Germany, Technische Universität Dresden – sequence: 11 givenname: Stephan surname: Winnerl fullname: Winnerl, Stephan email: s.winnerl@hzdr.de organization: Helmholtz-Zentrum Dresden-Rossendorf, PO Box 510119 01314 Dresden, Germany
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Snippet	The energy spectrum of common two-dimensional electron gases consists of a harmonic (that is, equidistant) ladder of Landau levels, thus preventing the... The energy spectrum of common two-dimensional electron gases consists of a harmonic, i.e. equidistant ladder of Landau levels, thus preventing the possibility...
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SubjectTerms	140/125 639/624/399/918 639/766/119/995 639/766/119/997 Atomic Augers Carriers Classical and Continuum Physics Complex Systems Condensed Matter Condensed Matter Physics Depletion Dynamics Graphene Ladders Magnetic fields Materials science Mathematical and Computational Physics Mesoscopic Systems and Quantum Hall Effect Molecular Optical and Plasma Physics Optical pumping Physics Quantum physics Scattering Theoretical Two dimensional
Title	Carrier dynamics in Landau-quantized graphene featuring strong Auger scattering
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