Recent Advances and Strategies toward Polysulfides Shuttle Inhibition for High‐Performance Li–S Batteries
Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and cost‐effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble l...
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| Vydané v: | Advanced science Ročník 9; číslo 12; s. e2106004 - n/a |
|---|---|
| Hlavní autori: | , , , , , , , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
| Vydavateľské údaje: |
Germany
John Wiley & Sons, Inc
01.04.2022
John Wiley and Sons Inc Wiley |
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| ISSN: | 2198-3844, 2198-3844 |
| On-line prístup: | Získať plný text |
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| Abstract | Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and cost‐effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li–S batteries is introduced first to give an in‐deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li–S batteries are proposed.
This review summarizes the recent advances and strategies to suppress the shuttle effect of lithium polysulfides (LiPSs) in lithium–sulfur batteries. These strategies are composed of using the modified sulfur hosts to immobilize LiPSs, electrolyte systems to alleviate shuttle behavior, functional separator to intercept LiPSs, and anode surface engineering to avoid the chemical reaction between LiPSs and Li. |
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| AbstractList | Lithium-sulfur (Li-S) batteries are regarded as the most promising next-generation energy storage systems due to their high energy density and cost-effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li-S batteries is introduced first to give an in-deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li-S batteries are proposed. Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and cost‐effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li–S batteries is introduced first to give an in‐deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li–S batteries are proposed. This review summarizes the recent advances and strategies to suppress the shuttle effect of lithium polysulfides (LiPSs) in lithium–sulfur batteries. These strategies are composed of using the modified sulfur hosts to immobilize LiPSs, electrolyte systems to alleviate shuttle behavior, functional separator to intercept LiPSs, and anode surface engineering to avoid the chemical reaction between LiPSs and Li. Lithium-sulfur (Li-S) batteries are regarded as the most promising next-generation energy storage systems due to their high energy density and cost-effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li-S batteries is introduced first to give an in-deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li-S batteries are proposed.Lithium-sulfur (Li-S) batteries are regarded as the most promising next-generation energy storage systems due to their high energy density and cost-effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li-S batteries is introduced first to give an in-deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li-S batteries are proposed. Abstract Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and cost‐effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li–S batteries is introduced first to give an in‐deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li–S batteries are proposed. Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and cost‐effectiveness. However, their practical applications are seriously hindered by several inevitable drawbacks, especially the shuttle effects of soluble lithium polysulfides (LiPSs) which lead to rapid capacity decay and short cycling lifespan. This review specifically concentrates on the shuttle path of LiPSs and their interaction with the corresponding cell components along the moving way, systematically retrospect the recent advances and strategies toward polysulfides diffusion suppression. Overall, the strategies for the shuttle effect inhibition can be classified into four parts, including capturing the LiPSs in the sulfur cathode, reducing the dissolution in electrolytes, blocking the shuttle channels by functional separators, and preventing the chemical reaction between LiPSs and Li metal anode. Herein, the fundamental aspect of Li–S batteries is introduced first to give an in‐deep understanding of the generation and shuttle effect of LiPSs. Then, the corresponding strategies toward LiPSs shuttle inhibition along the diffusion path are discussed step by step. Finally, general conclusions and perspectives for future research on shuttle issues and practical application of Li–S batteries are proposed. This review summarizes the recent advances and strategies to suppress the shuttle effect of lithium polysulfides (LiPSs) in lithium–sulfur batteries. These strategies are composed of using the modified sulfur hosts to immobilize LiPSs, electrolyte systems to alleviate shuttle behavior, functional separator to intercept LiPSs, and anode surface engineering to avoid the chemical reaction between LiPSs and Li. |
| Author | Wei, Qiulong Xie, Qingshui Li, Yikai Huang, Youzhang Lin, Liang Liu, Lie Qiao, Zhensong Lin, Jie Zhang, Chengkun Wang, Laisen Peng, Dong‐Liang |
| AuthorAffiliation | 1 State Key Lab for Physical Chemistry of Solid Surfaces Fujian Key Laboratory of Materials Genome Collaborative Innovation Center of Chemistry for Energy Materials College of Materials Xiamen University Xiamen 361005 P. R. China 2 Shenzhen Research Institute of Xiamen University Shenzhen 518000 P. R. China |
| AuthorAffiliation_xml | – name: 2 Shenzhen Research Institute of Xiamen University Shenzhen 518000 P. R. China – name: 1 State Key Lab for Physical Chemistry of Solid Surfaces Fujian Key Laboratory of Materials Genome Collaborative Innovation Center of Chemistry for Energy Materials College of Materials Xiamen University Xiamen 361005 P. R. China |
| Author_xml | – sequence: 1 givenname: Youzhang orcidid: 0000-0002-3581-2995 surname: Huang fullname: Huang, Youzhang organization: Xiamen University – sequence: 2 givenname: Liang surname: Lin fullname: Lin, Liang organization: Xiamen University – sequence: 3 givenname: Chengkun surname: Zhang fullname: Zhang, Chengkun organization: Xiamen University – sequence: 4 givenname: Lie surname: Liu fullname: Liu, Lie organization: Xiamen University – sequence: 5 givenname: Yikai surname: Li fullname: Li, Yikai organization: Xiamen University – sequence: 6 givenname: Zhensong surname: Qiao fullname: Qiao, Zhensong organization: Xiamen University – sequence: 7 givenname: Jie surname: Lin fullname: Lin, Jie organization: Xiamen University – sequence: 8 givenname: Qiulong surname: Wei fullname: Wei, Qiulong organization: Xiamen University – sequence: 9 givenname: Laisen surname: Wang fullname: Wang, Laisen organization: Xiamen University – sequence: 10 givenname: Qingshui surname: Xie fullname: Xie, Qingshui email: xieqsh@xmu.edu.cn organization: Shenzhen Research Institute of Xiamen University – sequence: 11 givenname: Dong‐Liang orcidid: 0000-0003-4155-4766 surname: Peng fullname: Peng, Dong‐Liang email: dlpeng@xmu.edu.cn organization: Xiamen University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35233996$$D View this record in MEDLINE/PubMed |
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| Snippet | Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and... Lithium-sulfur (Li-S) batteries are regarded as the most promising next-generation energy storage systems due to their high energy density and... Abstract Lithium–sulfur (Li–S) batteries are regarded as the most promising next‐generation energy storage systems due to their high energy density and... |
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| SubjectTerms | Carbon electrolyte systems Electrolytes Energy storage functional separators Lithium lithium anode Review Reviews shuttle effect sulfur hosts |
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| Title | Recent Advances and Strategies toward Polysulfides Shuttle Inhibition for High‐Performance Li–S Batteries |
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