Isotope Shifts of Radium Monofluoride Molecules

Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2 ← X2Σ+. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the...

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Published in:Physical review letters Vol. 127; no. 3; p. 1
Main Authors: Udrescu, S. M., Brinson, A. J., Ruiz, R. F. Garcia, Gaul, K., Berger, R., Billowes, J., Binnersley, C. L., Bissell, M. L., Breier, A. A., Chrysalidis, K., Cocolios, T. E., Cooper, B. S., Flanagan, K. T., Giesen, T. F., de Groote, R. P., Franchoo, S., Gustafsson, F. P., Isaev, T. A., Koszorús, Á., Neyens, G., Perrett, H. A., Ricketts, C. M., Rothe, S., Vernon, A. R., Wendt, K. D. A., Wienholtz, F., Wilkins, S. G., Yang, X. F.
Format: Journal Article
Language:English
Published: College Park American Physical Society 16.07.2021
American Physical Society (APS)
Subjects:
ab initio calculations
atomic & molecular structure
fundamental symmetries
Hartree-Fock methods
molecular physics
molecular spectra
Molecular structure
molecule trapping & guiding
Nuclear Experiment
nuclear physics
Nuclear structure
optical absorption spectroscopy
Physics
Quantum chemistry
radioactive isotopes
radioactive molecules
Radium
relativistic & quantum electrodynamic effects in atoms, molecules,& ions
Size effects
ISSN:0031-9007, 1079-7114, 1079-7114
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Abstract Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2 ← X2Σ+. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.
AbstractList Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2 ← X2Σ+. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.
Isotope shifts of ^{223-226,228}Ra^{19}F were measured for different vibrational levels in the electronic transition A^{2}Π_{1/2}←X^{2}Σ^{+}. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.Isotope shifts of ^{223-226,228}Ra^{19}F were measured for different vibrational levels in the electronic transition A^{2}Π_{1/2}←X^{2}Σ^{+}. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.
Isotope shifts of $^{223-226,228}$ Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^2 \Pi_{1/2} \leftarrow X^2 \Sigma^+$. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies
Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2←X2Σ+. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.
ArticleNumber 033001
Author Breier, A. A.
Udrescu, S. M.
Billowes, J.
Yang, X. F.
Franchoo, S.
de Groote, R. P.
Gaul, K.
Ruiz, R. F. Garcia
Wienholtz, F.
Gustafsson, F. P.
Binnersley, C. L.
Cocolios, T. E.
Bissell, M. L.
Isaev, T. A.
Berger, R.
Ricketts, C. M.
Rothe, S.
Neyens, G.
Wilkins, S. G.
Perrett, H. A.
Vernon, A. R.
Chrysalidis, K.
Wendt, K. D. A.
Brinson, A. J.
Giesen, T. F.
Flanagan, K. T.
Cooper, B. S.
Koszorús, Á.
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Snippet Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2 ← X2Σ+. The observed isotope shifts...
Isotope shifts of ^{223-226,228}Ra^{19}F were measured for different vibrational levels in the electronic transition A^{2}Π_{1/2}←X^{2}Σ^{+}. The observed...
Isotope shifts of $^{223-226,228}$ Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^2 \Pi_{1/2} \leftarrow X^2...
Isotope shifts of 223–226,228Ra19F were measured for different vibrational levels in the electronic transition A2II1/2←X2Σ+. The observed isotope shifts...
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StartPage 1
SubjectTerms ab initio calculations
atomic & molecular structure
fundamental symmetries
Hartree-Fock methods
molecular physics
molecular spectra
Molecular structure
molecule trapping & guiding
Nuclear Experiment
nuclear physics
Nuclear structure
optical absorption spectroscopy
Physics
Quantum chemistry
radioactive isotopes
radioactive molecules
Radium
relativistic & quantum electrodynamic effects in atoms, molecules,& ions
Size effects
Title Isotope Shifts of Radium Monofluoride Molecules
URI https://www.proquest.com/docview/2557868001
https://www.proquest.com/docview/2557224147
https://hal.science/hal-03312599
https://www.osti.gov/servlets/purl/1797304
Volume 127
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