Biomass to olefins: Cracking of renewable naphtha
► Steam cracking of renewable naphtha was studied in a pilot plant. ► The naphtha was derived from waste fats and greases by catalytic hydrotreatment. ► The pilot plant experiments show that high light olefin yields can be obtained. ► Based on an experimental coking study, high run lengths can be ex...
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| Vydané v: | Chemical engineering journal (Lausanne, Switzerland : 1996) Ročník 176; s. 178 - 187 |
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| Hlavní autori: | , , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
| Vydavateľské údaje: |
Elsevier B.V
01.12.2011
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| ISSN: | 1385-8947, 1873-3212 |
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| Abstract | ► Steam cracking of renewable naphtha was studied in a pilot plant. ► The naphtha was derived from waste fats and greases by catalytic hydrotreatment. ► The pilot plant experiments show that high light olefin yields can be obtained. ► Based on an experimental coking study, high run lengths can be expected.
An alternative route for the production of light olefins is proposed starting from low value and waste fats, greases and other renewable fractions. The first step catalytically converts triglycerides and/or fatty acids from bio oils to a high quality paraffinic diesel or jet fuel and renewable naphtha. GC
×
GC–TOF-MS and GC
×
GC–FID characterization of the renewable naphtha showed that it mainly consists of n-paraffins (32.6
wt%) and iso-paraffins (60
wt%), with only small amounts of aromatics (0.8
wt%), naphthenics (6.3
wt%) and olefinics (0.3
wt%). No remaining oxygenates are measured, making it a potentially attractive feed for the production of ethylene. Steam cracking of this renewable naphtha in a pilot plant revealed that high light olefin yields can be obtained (ethylene yield of 31
wt% and a propylene yield of 17.5
wt%), while the amount of pyrolysis gasoline (15
wt%) and pyrolysis fuel oil (<1
wt%) produced remains small. An experimental coking study further confirmed the attractive character of this feed. Run length simulations show that higher run lengths can be expected in comparison with the typically used naphtha fractions from fossil resources. |
|---|---|
| AbstractList | An alternative route for the production of light olefins is proposed starting from low value and waste fats, greases and other renewable fractions. The first step catalytically converts triglycerides and/or fatty acids from bio oils to a high quality paraffinic diesel or jet fuel and renewable naphtha. GC×GC–TOF-MS and GC×GC–FID characterization of the renewable naphtha showed that it mainly consists of n-paraffins (32.6wt%) and iso-paraffins (60wt%), with only small amounts of aromatics (0.8wt%), naphthenics (6.3wt%) and olefinics (0.3wt%). No remaining oxygenates are measured, making it a potentially attractive feed for the production of ethylene. Steam cracking of this renewable naphtha in a pilot plant revealed that high light olefin yields can be obtained (ethylene yield of 31wt% and a propylene yield of 17.5wt%), while the amount of pyrolysis gasoline (15wt%) and pyrolysis fuel oil (<1wt%) produced remains small. An experimental coking study further confirmed the attractive character of this feed. Run length simulations show that higher run lengths can be expected in comparison with the typically used naphtha fractions from fossil resources. ► Steam cracking of renewable naphtha was studied in a pilot plant. ► The naphtha was derived from waste fats and greases by catalytic hydrotreatment. ► The pilot plant experiments show that high light olefin yields can be obtained. ► Based on an experimental coking study, high run lengths can be expected. An alternative route for the production of light olefins is proposed starting from low value and waste fats, greases and other renewable fractions. The first step catalytically converts triglycerides and/or fatty acids from bio oils to a high quality paraffinic diesel or jet fuel and renewable naphtha. GC × GC–TOF-MS and GC × GC–FID characterization of the renewable naphtha showed that it mainly consists of n-paraffins (32.6 wt%) and iso-paraffins (60 wt%), with only small amounts of aromatics (0.8 wt%), naphthenics (6.3 wt%) and olefinics (0.3 wt%). No remaining oxygenates are measured, making it a potentially attractive feed for the production of ethylene. Steam cracking of this renewable naphtha in a pilot plant revealed that high light olefin yields can be obtained (ethylene yield of 31 wt% and a propylene yield of 17.5 wt%), while the amount of pyrolysis gasoline (15 wt%) and pyrolysis fuel oil (<1 wt%) produced remains small. An experimental coking study further confirmed the attractive character of this feed. Run length simulations show that higher run lengths can be expected in comparison with the typically used naphtha fractions from fossil resources. An alternative route for the production of light olefins is proposed starting from low value and waste fats, greases and other renewable fractions. The first step catalytically converts triglycerides and/or fatty acids from bio oils to a high quality paraffinic diesel or jet fuel and renewable naphtha. GC x GC-TOF-MS and GC x GC-FID characterization of the renewable naphtha showed that it mainly consists of n-paraffins (32.6 wt%) and iso-paraffins (60 wt%), with only small amounts of aromatics (0.8 wt%), naphthenics (6.3 wt%) and olefinics (0.3 wt%). No remaining oxygenates are measured, making it a potentially attractive feed for the production of ethylene. Steam cracking of this renewable naphtha in a pilot plant revealed that high light olefin yields can be obtained (ethylene yield of 31 wt% and a propylene yield of 17.5 wt%), while the amount of pyrolysis gasoline (15 wt%) and pyrolysis fuel oil (<1 wt%) produced remains small. An experimental coking study further confirmed the attractive character of this feed. Run length simulations show that higher run lengths can be expected in comparison with the typically used naphtha fractions from fossil resources. |
| Author | Marin, Guy. B. Van Geem, Kevin M. Reyniers, Marie-Françoise Pyl, Steven P. Schietekat, Carl M. Abhari, Ramin |
| Author_xml | – sequence: 1 givenname: Steven P. surname: Pyl fullname: Pyl, Steven P. organization: Laboratory for Chemical Technology, Ghent Univeristy (LCT), Technologiepark 918, B-9052 Gent, Belgium – sequence: 2 givenname: Carl M. surname: Schietekat fullname: Schietekat, Carl M. organization: Laboratory for Chemical Technology, Ghent Univeristy (LCT), Technologiepark 918, B-9052 Gent, Belgium – sequence: 3 givenname: Marie-Françoise surname: Reyniers fullname: Reyniers, Marie-Françoise organization: Laboratory for Chemical Technology, Ghent Univeristy (LCT), Technologiepark 918, B-9052 Gent, Belgium – sequence: 4 givenname: Ramin surname: Abhari fullname: Abhari, Ramin organization: Syntroleum Corporation, Tulsa, OK, USA – sequence: 5 givenname: Guy. B. surname: Marin fullname: Marin, Guy. B. organization: Laboratory for Chemical Technology, Ghent Univeristy (LCT), Technologiepark 918, B-9052 Gent, Belgium – sequence: 6 givenname: Kevin M. surname: Van Geem fullname: Van Geem, Kevin M. email: kevin.vangeem@ugent.be organization: Laboratory for Chemical Technology, Ghent Univeristy (LCT), Technologiepark 918, B-9052 Gent, Belgium |
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| Snippet | ► Steam cracking of renewable naphtha was studied in a pilot plant. ► The naphtha was derived from waste fats and greases by catalytic hydrotreatment. ► The... An alternative route for the production of light olefins is proposed starting from low value and waste fats, greases and other renewable fractions. The first... |
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| SubjectTerms | aromatic compounds Biomass Biomass conversion chemical engineering Comprehensive 2D GC cracking Ethylene ethylene production Fats fatty acids Fossils Fracture mechanics fuel oils gasoline Naphtha olefin Olefin production Olefins propylene Pyrolysis steam Steam cracking triacylglycerols |
| Title | Biomass to olefins: Cracking of renewable naphtha |
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