Laser spectroscopy of indium Rydberg atom bunches by electric field ionization
This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization tec...
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| Published in: | Scientific reports Vol. 10; no. 1; p. 12306 |
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| Main Authors: | , , , , , , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
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Nature Publishing Group UK
23.07.2020
Nature Publishing Group |
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| ISSN: | 2045-2322, 2045-2322 |
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| Abstract | This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the
5s
2
5d
2
D
5
/
2
and
5s
2
5d
2
D
3
/
2
states to
5s
2
n
p
2
P and
5s
2
n
f
2
F Rydberg states, up to a principal quantum number of
n
=
72
. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be
46
,
670.107
(
4
)
cm
-
1
. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the
5s
2
5d
2
D
5
/
2
and
5s
2
5d
2
D
3
/
2
states were determined for
113
,
115
In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. |
|---|---|
| AbstractList | This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the $$\text {5s}^2\text {5d}\,^2\text {D}_{5/2}$$ 5s25d2D5/2 and $$\text {5s}^2\text {5d}\,^2\text {D}_{3/2}$$ 5s25d2D3/2 states to $$\text {5s}^2n$$ 5s2np $$^2$$ 2P and $$\text {5s}^2n\text {f}\,^2$$ 5s2nf2F Rydberg states, up to a principal quantum number of $$n=72$$ n=72. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be $$46,670.107(4)\,\hbox {cm}^{-1}$$ 46,670.107(4)cm-1. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the $$\text {5s}^2\text {5d}\,^2\text {D}_{5/2}$$ 5s25d2D5/2 and $$\text {5s}^2\text {5d}\,^2\text {D}_{3/2}$$ 5s25d2D3/2 states were determined for $$^{113,115}$$ 113,115In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the 5s 2 5d 2 D 5 / 2 and 5s 2 5d 2 D 3 / 2 states to 5s 2 n p 2 P and 5s 2 n f 2 F Rydberg states, up to a principal quantum number of n = 72 . The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be 46 , 670.107 ( 4 ) cm - 1 . The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the 5s 2 5d 2 D 5 / 2 and 5s 2 5d 2 D 3 / 2 states were determined for 113 , 115 In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the $$\text {5s}^2\text {5d}\,^2\text {D}_{5/2}$$ 5s 2 5d 2 D 5 / 2 and $$\text {5s}^2\text {5d}\,^2\text {D}_{3/2}$$ 5s 2 5d 2 D 3 / 2 states to $$\text {5s}^2n$$ 5s 2 n p $$^2$$ 2 P and $$\text {5s}^2n\text {f}\,^2$$ 5s 2 n f 2 F Rydberg states, up to a principal quantum number of $$n=72$$ n = 72 . The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be $$46,670.107(4)\,\hbox {cm}^{-1}$$ 46 , 670.107 ( 4 ) cm - 1 . The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the $$\text {5s}^2\text {5d}\,^2\text {D}_{5/2}$$ 5s 2 5d 2 D 5 / 2 and $$\text {5s}^2\text {5d}\,^2\text {D}_{3/2}$$ 5s 2 5d 2 D 3 / 2 states were determined for $$^{113,115}$$ 113 , 115 In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the [Formula: see text] and [Formula: see text] states to [Formula: see text]p [Formula: see text]P and [Formula: see text]F Rydberg states, up to a principal quantum number of [Formula: see text]. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be [Formula: see text]. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the [Formula: see text] and [Formula: see text] states were determined for [Formula: see text]In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection.This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the [Formula: see text] and [Formula: see text] states to [Formula: see text]p [Formula: see text]P and [Formula: see text]F Rydberg states, up to a principal quantum number of [Formula: see text]. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be [Formula: see text]. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the [Formula: see text] and [Formula: see text] states were determined for [Formula: see text]In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the 5s25d2D5/2 and 5s25d2D3/2 states to 5s2np 2P and 5s2nf2F Rydberg states, up to a principal quantum number of n=72. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be 46,670.107(4)cm-1. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the 5s25d2D5/2 and 5s25d2D3/2 states were determined for 113,115In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over previous non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the 5s25d2D5/2 and 5s25d2D3/2 states to 5s2np 2P and 5s2nf2 F Rydberg states, up to a principal quantum number of n=72 . The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be 46,670.107(4)cm-1. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the 5s25d2D5/2 and 5s25d2D3/2 states were determined for 113,115In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed at the same time and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection. |
| ArticleNumber | 12306 |
| Author | Sahoo, B. K. Neyens, G. Wang, Q. Gustafsson, F. P. Cooper, B. S. Waso, F. J. Billowes, J. Garcia Ruiz, R. F. Flanagan, K. T. Yang, X. F. Perrett, H. A. Vernon, A. R. Cocolios, T. E. Ricketts, C. M. |
| Author_xml | – sequence: 1 givenname: A. R. surname: Vernon fullname: Vernon, A. R. email: adam.vernon@cern.ch organization: Instituut voor Kern- en Stralingsfysica, KU Leuven – sequence: 2 givenname: C. M. surname: Ricketts fullname: Ricketts, C. M. organization: School of Physics and Astronomy, The University of Manchester – sequence: 3 givenname: J. surname: Billowes fullname: Billowes, J. organization: School of Physics and Astronomy, The University of Manchester – sequence: 4 givenname: T. E. surname: Cocolios fullname: Cocolios, T. E. organization: Instituut voor Kern- en Stralingsfysica, KU Leuven – sequence: 5 givenname: B. S. surname: Cooper fullname: Cooper, B. S. organization: School of Physics and Astronomy, The University of Manchester, Photon Science Institute, Alan Turing Building, University of Manchester – sequence: 6 givenname: K. T. surname: Flanagan fullname: Flanagan, K. T. organization: School of Physics and Astronomy, The University of Manchester, Photon Science Institute, Alan Turing Building, University of Manchester – sequence: 7 givenname: R. F. surname: Garcia Ruiz fullname: Garcia Ruiz, R. F. organization: EP Department, CERN, Massachusetts Institute of Technology – sequence: 8 givenname: F. P. surname: Gustafsson fullname: Gustafsson, F. P. organization: Instituut voor Kern- en Stralingsfysica, KU Leuven – sequence: 9 givenname: G. surname: Neyens fullname: Neyens, G. organization: Instituut voor Kern- en Stralingsfysica, KU Leuven, EP Department, CERN – sequence: 10 givenname: H. A. surname: Perrett fullname: Perrett, H. A. organization: School of Physics and Astronomy, The University of Manchester – sequence: 11 givenname: B. K. surname: Sahoo fullname: Sahoo, B. K. organization: Atomic, Molecular and Optical Physics Division, Physical Research Laboratory – sequence: 12 givenname: Q. surname: Wang fullname: Wang, Q. organization: School of Nuclear Science and Technology, Lanzhou University – sequence: 13 givenname: F. J. surname: Waso fullname: Waso, F. J. organization: Stellenbosch University – sequence: 14 givenname: X. F. surname: Yang fullname: Yang, X. F. organization: School of Physics and State Key Laboratory of Nuclear Physics and Technology, Peking University |
| BackLink | https://www.osti.gov/servlets/purl/1817137$$D View this record in Osti.gov |
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| CitedBy_id | crossref_primary_10_1103_PhysRevC_111_064325 crossref_primary_10_1007_s11182_022_02535_2 crossref_primary_10_1103_nyn5_69s3 crossref_primary_10_1088_1572_9494_acb58b crossref_primary_10_1016_j_nimb_2023_04_054 crossref_primary_10_1016_j_nimb_2023_04_020 crossref_primary_10_1016_j_vacuum_2022_111640 crossref_primary_10_1007_s13538_024_01470_6 crossref_primary_10_1051_epjconf_202226104002 crossref_primary_10_1016_j_ppnp_2022_104005 crossref_primary_10_1088_1674_1137_ac501a crossref_primary_10_1140_epja_s10050_024_01230_9 crossref_primary_10_1103_PhysRevC_105_L031305 |
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| SubjectTerms | 639/766/36/1122 639/766/387/1126 639/766/930/527 ATOMIC AND MOLECULAR PHYSICS Electric fields electronic structure of atoms and molecules experimental nuclear physics Humanities and Social Sciences Indium Ionization Ions Isotopes Lasers multidisciplinary optical spectroscopy Science Science (multidisciplinary) Spectroscopy Spectrum analysis |
| Title | Laser spectroscopy of indium Rydberg atom bunches by electric field ionization |
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