On the Determination of Uncertainty and Limit of Detection in Label-Free Biosensors

A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison among the different biosensors is limited by the procedure used of calculating the limit of detection and the measurement uncertainty. This a...

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Vydané v:Sensors (Basel, Switzerland) Ročník 18; číslo 7; s. 2038
Hlavní autori: Lavín, Álvaro, Vicente, Jesús de, Holgado, Miguel, Laguna, María F., Casquel, Rafael, Santamaría, Beatriz, Maigler, María Victoria, Hernández, Ana L., Ramírez, Yolanda
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: Switzerland MDPI 26.06.2018
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Abstract A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison among the different biosensors is limited by the procedure used of calculating the limit of detection and the measurement uncertainty. This article clarifies and establishes a simple procedure to determine the calibration function and the uncertainty of the concentration measured at any point of the measuring interval of a generic label-free biosensor. The value of the limit of detection arises naturally from this model as the limit at which uncertainty tends when the concentration tends to zero. The need to provide additional information, such as the measurement interval and its linearity, among others, on the analytical systems and biosensor in addition to the detection limit is pointed out. Finally, the model is applied to curves that are typically obtained in immunoassays and a discussion is made on the application validity of the model and its limitations.
AbstractList A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison among the different biosensors is limited by the procedure used of calculating the limit of detection and the measurement uncertainty. This article clarifies and establishes a simple procedure to determine the calibration function and the uncertainty of the concentration measured at any point of the measuring interval of a generic label-free biosensor. The value of the limit of detection arises naturally from this model as the limit at which uncertainty tends when the concentration tends to zero. The need to provide additional information, such as the measurement interval and its linearity, among others, on the analytical systems and biosensor in addition to the detection limit is pointed out. Finally, the model is applied to curves that are typically obtained in immunoassays and a discussion is made on the application validity of the model and its limitations.
A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison among the different biosensors is limited by the procedure used of calculating the limit of detection and the measurement uncertainty. This article clarifies and establishes a simple procedure to determine the calibration function and the uncertainty of the concentration measured at any point of the measuring interval of a generic label-free biosensor. The value of the limit of detection arises naturally from this model as the limit at which uncertainty tends when the concentration tends to zero. The need to provide additional information, such as the measurement interval and its linearity, among others, on the analytical systems and biosensor in addition to the detection limit is pointed out. Finally, the model is applied to curves that are typically obtained in immunoassays and a discussion is made on the application validity of the model and its limitations.A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison among the different biosensors is limited by the procedure used of calculating the limit of detection and the measurement uncertainty. This article clarifies and establishes a simple procedure to determine the calibration function and the uncertainty of the concentration measured at any point of the measuring interval of a generic label-free biosensor. The value of the limit of detection arises naturally from this model as the limit at which uncertainty tends when the concentration tends to zero. The need to provide additional information, such as the measurement interval and its linearity, among others, on the analytical systems and biosensor in addition to the detection limit is pointed out. Finally, the model is applied to curves that are typically obtained in immunoassays and a discussion is made on the application validity of the model and its limitations.
Author Laguna, María F.
Santamaría, Beatriz
Holgado, Miguel
Maigler, María Victoria
Lavín, Álvaro
Vicente, Jesús de
Hernández, Ana L.
Casquel, Rafael
Ramírez, Yolanda
AuthorAffiliation 4 BioOptical Detection, Centro de Tecnología Biomédica, Campus Montegancedo, 28223 Madrid, Spain
3 Laboratorio de Metrología y Metrotecnia, Escuela Técnica Superior de Ingenieros Industriales, Universidad Politécnica de Madrid, C/ José Gutiérrez Abascal, 2, 28006 Madrid, Spain
1 Centre for Biomedical Technology, Optics, Photonics and Biophotonics Laboratory, Campus Montegancedo, Universidad Politécnica de Madrid, 28223 Madrid, Spain; alvaro.lavin@upm.es (A.L.); mariafe.laguna@upm.es (M.F.L.); rafael.casquel@upm.es (R.C.); beatriz.santamaria@ctb.upm.es (B.S.); m.maigler@biod.es (M.V.M.); ana.lopez@upm.es (A.L.H.); y.ramirez@biod.es (Y.R.)
2 Department of Applied Physics, Escuela Técnica Superior de Ingenieros Industriales, Universidad Politécnica de Madrid, C/José Gutiérrez Abascal, 2, 28006 Madrid, Spain; jvo@etsii.upm.es
AuthorAffiliation_xml – name: 2 Department of Applied Physics, Escuela Técnica Superior de Ingenieros Industriales, Universidad Politécnica de Madrid, C/José Gutiérrez Abascal, 2, 28006 Madrid, Spain; jvo@etsii.upm.es
– name: 1 Centre for Biomedical Technology, Optics, Photonics and Biophotonics Laboratory, Campus Montegancedo, Universidad Politécnica de Madrid, 28223 Madrid, Spain; alvaro.lavin@upm.es (A.L.); mariafe.laguna@upm.es (M.F.L.); rafael.casquel@upm.es (R.C.); beatriz.santamaria@ctb.upm.es (B.S.); m.maigler@biod.es (M.V.M.); ana.lopez@upm.es (A.L.H.); y.ramirez@biod.es (Y.R.)
– name: 4 BioOptical Detection, Centro de Tecnología Biomédica, Campus Montegancedo, 28223 Madrid, Spain
– name: 3 Laboratorio de Metrología y Metrotecnia, Escuela Técnica Superior de Ingenieros Industriales, Universidad Politécnica de Madrid, C/ José Gutiérrez Abascal, 2, 28006 Madrid, Spain
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  givenname: María F.
  orcidid: 0000-0002-1580-4509
  surname: Laguna
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  surname: Casquel
  fullname: Casquel, Rafael
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  orcidid: 0000-0003-3714-7922
  surname: Santamaría
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Issue 7
Keywords label-free biosensing performance
measurement uncertainty
limit of quantification
calculation of the limit of detection
Language English
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Snippet A significant amount of noteworthy articles reviewing different label-free biosensors are being published in the last years. Most of the times, the comparison...
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SubjectTerms Biosensing Techniques - standards
calculation of the limit of detection
Calibration
label-free biosensing performance
Limit of Detection
limit of quantification
measurement uncertainty
Reproducibility of Results
Review
Uncertainty
Title On the Determination of Uncertainty and Limit of Detection in Label-Free Biosensors
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Volume 18
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