Super-Resolution Reactivity Mapping of Nanostructured Catalyst Particles

Its a small world: Nanoscale reactivity maps of working heterogeneous catalysts are recorded under in situ conditions by localizing single fluorescent reaction products (see picture). This approach allows quantification of the reactivity of catalytic nanodomains.

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Bibliographic Details
Published in:Angewandte Chemie (International ed.) Vol. 48; no. 49; pp. 9285 - 9289
Main Authors: Roeffaers, Maarten B.J, De Cremer, Gert, Libeert, Julien, Ameloot, Rob, Dedecker, Peter, Bons, Anton-Jan, Bückins, Matthias, Martens, Johan A, Sels, Bert F, De Vos, Dirk E, Hofkens, Johan
Format: Journal Article
Language:English
Published: Weinheim Wiley-VCH Verlag 23.11.2009
WILEY-VCH Verlag
WILEY‐VCH Verlag
Subjects:
fluorescence
heterogeneous catalysis
kinetics
single-molecule studies
zeolites
ISSN:1433-7851, 1521-3773, 1521-3773
Online Access:Get full text
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Summary:Its a small world: Nanoscale reactivity maps of working heterogeneous catalysts are recorded under in situ conditions by localizing single fluorescent reaction products (see picture). This approach allows quantification of the reactivity of catalytic nanodomains.
Bibliography:http://dx.doi.org/10.1002/anie.200904944
EC 6th Framework Program - No. ERAS-CT-2003-980409
FWO Flanders - No. G.0366.06; No. G.0402.09
M.B.J.R., G.D.C., R.A., and P.D. thank the FWO (Fonds voor Wetenschappelijk Onderzoek)-Flanders for PhD or postdoctoral fellowships. This work was performed within the framework of the IAP-VI program Functional Supramolecular Systems of the Belgian Federal Government. The authors acknowledge financial support from the FWO Flanders (Grants G.0366.06 and G.0402.09), the K. U. Leuven Research Fund (GOA 2006/2, Center of Excellence CECAT, CREA2007), the Flemish Ministry of Education (ZWAP 04/007), long-term structural funding "Methusalem" by the K. U. Leuven, and the European Network of Excellence (IDECAT). This work was supported by the EC 6th Framework Program (ERAS-CT-2003-980409).
European Network of Excellence (IDECAT)
ark:/67375/WNG-HBR2SHJK-2
K. U. Leuven Research Fund - No. GOA 2006/2
Flemish Ministry of Education - No. ZWAP 04/007
istex:36DB091371698C95F11ED10246F085FF098EEA47
ArticleID:ANIE200904944
M.B.J.R., G.D.C., R.A., and P.D. thank the FWO (Fonds voor Wetenschappelijk Onderzoek)‐Flanders for PhD or postdoctoral fellowships. This work was performed within the framework of the IAP‐VI program Functional Supramolecular Systems of the Belgian Federal Government. The authors acknowledge financial support from the FWO Flanders (Grants G.0366.06 and G.0402.09), the K. U. Leuven Research Fund (GOA 2006/2, Center of Excellence CECAT, CREA2007), the Flemish Ministry of Education (ZWAP 04/007), long‐term structural funding “Methusalem” by the K. U. Leuven, and the European Network of Excellence (IDECAT). This work was supported by the EC 6th Framework Program (ERAS‐CT‐2003‐980409).
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ISSN:1433-7851
1521-3773
1521-3773
DOI:10.1002/anie.200904944