Strain engineering induced interfacial self-assembly and intrinsic exchange bias in a manganite perovskite film

The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimi...

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Published in:	Scientific reports Vol. 3; no. 1; p. 2542
Main Authors:	Cui, B., Song, C., Wang, G. Y., Mao, H. J., Zeng, F., Pan, F.
Format:	Journal Article
Language:	English
Published:	London Nature Publishing Group UK 29.08.2013 Nature Publishing Group
Subjects:	639/301/119/544 639/301/119/997 639/766/25 639/925/357/1018 Bias Engineering Humanities and Social Sciences Interfaces multidisciplinary Science Self-assembly Spectrum analysis
ISSN:	2045-2322, 2045-2322
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Abstract	The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimical to their device applications, could also flourish in tailored functionalities in return. Here we prove that the exchange bias (EB) effect can unexpectedly emerge in a (La,Sr)MnO 3 (LSMO) “single” film when large compressive stress imposed through a lattice mismatched substrate. The intrinsic EB behavior is directly demonstrated to be originating from the exchange coupling between ferromagnetic LSMO and an unprecedented LaSrMnO 4 -based spin glass, formed under a large interfacial strain and subsequent self-assembly. The present results not only provide a strategy for producing a new class of delicately functional interface by strain engineering, but also shed promising light on fabricating the EB part of spintronic devices in a single step.
AbstractList	The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimical to their device applications, could also flourish in tailored functionalities in return. Here we prove that the exchange bias (EB) effect can unexpectedly emerge in a (La,Sr)MnO3 (LSMO) “single” film when large compressive stress imposed through a lattice mismatched substrate. The intrinsic EB behavior is directly demonstrated to be originating from the exchange coupling between ferromagnetic LSMO and an unprecedented LaSrMnO4-based spin glass, formed under a large interfacial strain and subsequent self-assembly. The present results not only provide a strategy for producing a new class of delicately functional interface by strain engineering, but also shed promising light on fabricating the EB part of spintronic devices in a single step. The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimical to their device applications, could also flourish in tailored functionalities in return. Here we prove that the exchange bias (EB) effect can unexpectedly emerge in a (La,Sr)MnO 3 (LSMO) “single” film when large compressive stress imposed through a lattice mismatched substrate. The intrinsic EB behavior is directly demonstrated to be originating from the exchange coupling between ferromagnetic LSMO and an unprecedented LaSrMnO 4 -based spin glass, formed under a large interfacial strain and subsequent self-assembly. The present results not only provide a strategy for producing a new class of delicately functional interface by strain engineering, but also shed promising light on fabricating the EB part of spintronic devices in a single step. The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimical to their device applications, could also flourish in tailored functionalities in return. Here we prove that the exchange bias (EB) effect can unexpectedly emerge in a (La,Sr)MnO3 (LSMO) "single" film when large compressive stress imposed through a lattice mismatched substrate. The intrinsic EB behavior is directly demonstrated to be originating from the exchange coupling between ferromagnetic LSMO and an unprecedented LaSrMnO4-based spin glass, formed under a large interfacial strain and subsequent self-assembly. The present results not only provide a strategy for producing a new class of delicately functional interface by strain engineering, but also shed promising light on fabricating the EB part of spintronic devices in a single step.The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two separately prepared materials. The frustration of magnetization and conductivity of manganite perovskite at surface/interface which is inimical to their device applications, could also flourish in tailored functionalities in return. Here we prove that the exchange bias (EB) effect can unexpectedly emerge in a (La,Sr)MnO3 (LSMO) "single" film when large compressive stress imposed through a lattice mismatched substrate. The intrinsic EB behavior is directly demonstrated to be originating from the exchange coupling between ferromagnetic LSMO and an unprecedented LaSrMnO4-based spin glass, formed under a large interfacial strain and subsequent self-assembly. The present results not only provide a strategy for producing a new class of delicately functional interface by strain engineering, but also shed promising light on fabricating the EB part of spintronic devices in a single step.
ArticleNumber	2542
Author	Pan, F. Cui, B. Zeng, F. Song, C. Wang, G. Y. Mao, H. J.
Author_xml	– sequence: 1 givenname: B. surname: Cui fullname: Cui, B. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University – sequence: 2 givenname: C. surname: Song fullname: Song, C. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University – sequence: 3 givenname: G. Y. surname: Wang fullname: Wang, G. Y. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University – sequence: 4 givenname: H. J. surname: Mao fullname: Mao, H. J. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University – sequence: 5 givenname: F. surname: Zeng fullname: Zeng, F. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University – sequence: 6 givenname: F. surname: Pan fullname: Pan, F. organization: Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/23985971$$D View this record in MEDLINE/PubMed
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Snippet	The control of complex oxide heterostructures at atomic level generates a rich spectrum of exotic properties and unexpected states at the interface between two...
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Title	Strain engineering induced interfacial self-assembly and intrinsic exchange bias in a manganite perovskite film
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