Complete Photocatalytic Mineralization of Microplastic on TiO2 Nanoparticle Film
Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degra...
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| Published in: | iScience Vol. 23; no. 7; p. 101326 |
|---|---|
| Main Authors: | , , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
| Published: |
Elsevier Inc
24.07.2020
Elsevier |
| Subjects: | |
| ISSN: | 2589-0042, 2589-0042 |
| Online Access: | Get full text |
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| Abstract | Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment.
[Display omitted]
•Efficient degradation of microplastics under UV light by TiO2 film•Triton-based TiO2 film showed higher photocatalytic performance•The role of radical species during microplastics degradation was elucidated•Degradation mechanism and reaction intermediates were explored
Catalysis; Environmental Chemistry; Nanomaterials |
|---|---|
| AbstractList | Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment.
[Display omitted]
•Efficient degradation of microplastics under UV light by TiO2 film•Triton-based TiO2 film showed higher photocatalytic performance•The role of radical species during microplastics degradation was elucidated•Degradation mechanism and reaction intermediates were explored
Catalysis; Environmental Chemistry; Nanomaterials Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment. • Efficient degradation of microplastics under UV light by TiO2 film • Triton-based TiO2 film showed higher photocatalytic performance • The role of radical species during microplastics degradation was elucidated • Degradation mechanism and reaction intermediates were explored Catalysis; Environmental Chemistry; Nanomaterials Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment. Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment.Recently, the environmental impacts of microplastics have received extensive attention owing to their accumulation in the environment. However, developing efficient technology for the control and purification of microplastics is still a big challenge. Herein, we investigated the photocatalytic degradation of typical microplastics such as polystyrene (PS) microspheres and polyethylene (PE) over TiO2 nanoparticle films under UV light irradiation. TiO2 nanoparticle film made with Triton X-100 showed complete mineralization (98.40%) of 400-nm PS in 12 h, while degradation for varying sizes of PS was also studied. PE degradation experiment presented a high photodegradation rate after 36 h. CO2 was found as the main end product. The degradation mechanism and intermediates were studied by in situ DRIFTS and HPPI-TOFMS, showing the generation of hydroxyl, carbonyl, and carbon-hydrogen groups during the photodegradation of PS. This study provides a green and cost-efficient strategy for the control of microplastics contamination in the environment. |
| ArticleNumber | 101326 |
| Author | Cheng, Hanyun Li, Kejian Feng, Yiqing Zhang, Liwu Wang, Tao Ajmal, Saira Liu, Yangyang Yang, Yang Nabi, Iqra Bacha, Aziz-Ur-Rahim |
| Author_xml | – sequence: 1 givenname: Iqra surname: Nabi fullname: Nabi, Iqra organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 2 givenname: Aziz-Ur-Rahim surname: Bacha fullname: Bacha, Aziz-Ur-Rahim organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 3 givenname: Kejian surname: Li fullname: Li, Kejian organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 4 givenname: Hanyun surname: Cheng fullname: Cheng, Hanyun organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 5 givenname: Tao surname: Wang fullname: Wang, Tao organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 6 givenname: Yangyang surname: Liu fullname: Liu, Yangyang organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 7 givenname: Saira surname: Ajmal fullname: Ajmal, Saira organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 8 givenname: Yang surname: Yang fullname: Yang, Yang organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 9 givenname: Yiqing surname: Feng fullname: Feng, Yiqing organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China – sequence: 10 givenname: Liwu orcidid: 0000-0002-0765-8660 surname: Zhang fullname: Zhang, Liwu email: zhanglw@fudan.edu.cn organization: Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China |
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