Physicochemical properties and heavy metals characteristics of building ceramsites with oil-based drilling cutting residues

Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were p...

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Veröffentlicht in:	Scientific reports Jg. 15; H. 1; S. 8473 - 16
Hauptverfasser:	Xiong, Deming, Wang, Chaoqiang
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	London Nature Publishing Group UK 12.03.2025 Nature Publishing Group Nature Portfolio
Schlagworte:	704/172/169/896 704/2151 Arsenic Barium Cadmium Carbonates Ceramsite Chemical properties Chromium Drilling Fly ash Foaming Heavy metal Heavy metals Humanities and Social Sciences Leaching Lead Mercury multidisciplinary Natural gas exploration Oil and gas exploration Oil based drilling cutting Organic matter Physicochemical characteristic Physicochemical properties Raw materials Science Science (multidisciplinary) Shale Solid wastes Toxicity Ceramsite Oil based drilling cutting Physicochemical characteristic Heavy metal
ISSN:	2045-2322, 2045-2322
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Abstract	Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were prepared with OBDCRs incorporating with fly ash (a byproduct of coal combustion) as raw materials. The aim was to comprehensively and systematically investigate physicochemical properties and characteristics of heavy metals (HMs) in the ceramsites. Research shows that building ceramsites can indeed be prepared using OBDCRs, which exhibit good comprehensive properties and strong resistance to acid/ alkali. The main HMs found in ceramsite are barium (Ba), chromium (Cr), nickel (Ni), lead (Pb), arsenic (As), cadmium (Cd), and mercury (Hg). During the calcination process, these OBDCRs, along with fly ash and foaming agent, underwent mutual melting, resulting in the formation of glass, anorthite and mullite. These newly formed phases effectively encapsulated HMs, resulting in varying degrees of enrichment of HMs such as As, Ba, Pb, Cr, and Ni, except for Cd and Hg. However, the leaching toxicity of these HMs in the ceramsite was significantly lower compared to that of the original OBDCRs. Further analysis revealed a significant increase in the proportion of Fe–Mn Oxides and Organic Matter in HMs such as Cr, Ni, As, Cd, and Pb, while the proportion of Exchangeable and Carbonates forms decreased markedly. This trend clearly demonstrated that the calcination process modified the physical and chemical properties of the ceramsite, and effectively stabilized HMs, i.e., migrated from an active state to a more stable form.
AbstractList	Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were prepared with OBDCRs incorporating with fly ash (a byproduct of coal combustion) as raw materials. The aim was to comprehensively and systematically investigate physicochemical properties and characteristics of heavy metals (HMs) in the ceramsites. Research shows that building ceramsites can indeed be prepared using OBDCRs, which exhibit good comprehensive properties and strong resistance to acid/ alkali. The main HMs found in ceramsite are barium (Ba), chromium (Cr), nickel (Ni), lead (Pb), arsenic (As), cadmium (Cd), and mercury (Hg). During the calcination process, these OBDCRs, along with fly ash and foaming agent, underwent mutual melting, resulting in the formation of glass, anorthite and mullite. These newly formed phases effectively encapsulated HMs, resulting in varying degrees of enrichment of HMs such as As, Ba, Pb, Cr, and Ni, except for Cd and Hg. However, the leaching toxicity of these HMs in the ceramsite was significantly lower compared to that of the original OBDCRs. Further analysis revealed a significant increase in the proportion of Fe–Mn Oxides and Organic Matter in HMs such as Cr, Ni, As, Cd, and Pb, while the proportion of Exchangeable and Carbonates forms decreased markedly. This trend clearly demonstrated that the calcination process modified the physical and chemical properties of the ceramsite, and effectively stabilized HMs, i.e., migrated from an active state to a more stable form. Abstract Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were prepared with OBDCRs incorporating with fly ash (a byproduct of coal combustion) as raw materials. The aim was to comprehensively and systematically investigate physicochemical properties and characteristics of heavy metals (HMs) in the ceramsites. Research shows that building ceramsites can indeed be prepared using OBDCRs, which exhibit good comprehensive properties and strong resistance to acid/ alkali. The main HMs found in ceramsite are barium (Ba), chromium (Cr), nickel (Ni), lead (Pb), arsenic (As), cadmium (Cd), and mercury (Hg). During the calcination process, these OBDCRs, along with fly ash and foaming agent, underwent mutual melting, resulting in the formation of glass, anorthite and mullite. These newly formed phases effectively encapsulated HMs, resulting in varying degrees of enrichment of HMs such as As, Ba, Pb, Cr, and Ni, except for Cd and Hg. However, the leaching toxicity of these HMs in the ceramsite was significantly lower compared to that of the original OBDCRs. Further analysis revealed a significant increase in the proportion of Fe–Mn Oxides and Organic Matter in HMs such as Cr, Ni, As, Cd, and Pb, while the proportion of Exchangeable and Carbonates forms decreased markedly. This trend clearly demonstrated that the calcination process modified the physical and chemical properties of the ceramsite, and effectively stabilized HMs, i.e., migrated from an active state to a more stable form. Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were prepared with OBDCRs incorporating with fly ash (a byproduct of coal combustion) as raw materials. The aim was to comprehensively and systematically investigate physicochemical properties and characteristics of heavy metals (HMs) in the ceramsites. Research shows that building ceramsites can indeed be prepared using OBDCRs, which exhibit good comprehensive properties and strong resistance to acid/ alkali. The main HMs found in ceramsite are barium (Ba), chromium (Cr), nickel (Ni), lead (Pb), arsenic (As), cadmium (Cd), and mercury (Hg). During the calcination process, these OBDCRs, along with fly ash and foaming agent, underwent mutual melting, resulting in the formation of glass, anorthite and mullite. These newly formed phases effectively encapsulated HMs, resulting in varying degrees of enrichment of HMs such as As, Ba, Pb, Cr, and Ni, except for Cd and Hg. However, the leaching toxicity of these HMs in the ceramsite was significantly lower compared to that of the original OBDCRs. Further analysis revealed a significant increase in the proportion of Fe-Mn Oxides and Organic Matter in HMs such as Cr, Ni, As, Cd, and Pb, while the proportion of Exchangeable and Carbonates forms decreased markedly. This trend clearly demonstrated that the calcination process modified the physical and chemical properties of the ceramsite, and effectively stabilized HMs, i.e., migrated from an active state to a more stable form.Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing equipment to transform OBDCRs into ceramsites appears to be a feasible and resource-efficient approach. In this study, building ceramsites were prepared with OBDCRs incorporating with fly ash (a byproduct of coal combustion) as raw materials. The aim was to comprehensively and systematically investigate physicochemical properties and characteristics of heavy metals (HMs) in the ceramsites. Research shows that building ceramsites can indeed be prepared using OBDCRs, which exhibit good comprehensive properties and strong resistance to acid/ alkali. The main HMs found in ceramsite are barium (Ba), chromium (Cr), nickel (Ni), lead (Pb), arsenic (As), cadmium (Cd), and mercury (Hg). During the calcination process, these OBDCRs, along with fly ash and foaming agent, underwent mutual melting, resulting in the formation of glass, anorthite and mullite. These newly formed phases effectively encapsulated HMs, resulting in varying degrees of enrichment of HMs such as As, Ba, Pb, Cr, and Ni, except for Cd and Hg. However, the leaching toxicity of these HMs in the ceramsite was significantly lower compared to that of the original OBDCRs. Further analysis revealed a significant increase in the proportion of Fe-Mn Oxides and Organic Matter in HMs such as Cr, Ni, As, Cd, and Pb, while the proportion of Exchangeable and Carbonates forms decreased markedly. This trend clearly demonstrated that the calcination process modified the physical and chemical properties of the ceramsite, and effectively stabilized HMs, i.e., migrated from an active state to a more stable form.
ArticleNumber	8473
Author	Wang, Chaoqiang Xiong, Deming
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Cites_doi	10.1016/j.biombioe.2022.106436 10.1016/j.jclepro.2018.10.134 10.1016/j.jhazmat.2008.12.023 10.1016/j.ecoenv.2019.03.081 10.1016/j.scitotenv.2021.146727 10.3389/fmats.2023.1245121 10.1038/s41401-019-0299-4 10.1038/s41598-023-50600-8 10.1007/s11356-021-16120-6 10.1016/j.ceramint.2023.07.107 10.1021/ac50043a017 10.1089/ees.2020.0490 10.1016/j.fuel.2022.125777
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Snippet	Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing existing... Abstract Oil-based drilling cutting residues (OBDCRs) are among the primary solid wastes generated during shale gas exploration and development. Utilizing...
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SubjectTerms	704/172/169/896 704/2151 Arsenic Barium Cadmium Carbonates Ceramsite Chemical properties Chromium Drilling Fly ash Foaming Heavy metal Heavy metals Humanities and Social Sciences Leaching Lead Mercury multidisciplinary Natural gas exploration Oil and gas exploration Oil based drilling cutting Organic matter Physicochemical characteristic Physicochemical properties Raw materials Science Science (multidisciplinary) Shale Solid wastes Toxicity
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Title	Physicochemical properties and heavy metals characteristics of building ceramsites with oil-based drilling cutting residues
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