Designing Hydrogen‐Bonded Organic Frameworks (HOFs) with Permanent Porosity

Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self‐standing porous molecular crystals (PMCs). Particularly, a...

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Published in:	Angewandte Chemie International Edition Vol. 58; no. 33; pp. 11160 - 11170
Main Authors:	Hisaki, Ichiro, Xin, Chen, Takahashi, Kiyonori, Nakamura, Takayoshi
Format:	Journal Article
Language:	English
Published:	Germany Wiley Subscription Services, Inc 12.08.2019
Edition:	International ed. in English
Subjects:	Construction materials Crystals gas sorption Hydrogen Hydrogen bonding hydrogen bonds hydrogen-bonded organic frameworks (HOFs) Organic chemistry permanent porosity Porosity Porous materials permanent porosity porous materials gas sorption hydrogen bonds hydrogen-bonded organic frameworks (HOFs)
ISSN:	1433-7851, 1521-3773, 1521-3773
Online Access:	Get full text
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Abstract	Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self‐standing porous molecular crystals (PMCs). Particularly, a number of crystalline systems with permanent porosity that are formed by self‐assembly through hydrogen bonding (H‐bonding) have been developed. Such systems are called hydrogen‐bonded organic frameworks (HOFs). Herein we systematically describe H‐bonding patterns (supramolecular synthons) and molecular structures (tectons) that have been used to achieve thermal and chemical durability, a large surface area, and functions, such as selective gas sorption and separation, which can provide design principles for constructing HOFs with permanent porosity. HOF the shelf: Hydrogen‐bonded organic frameworks (HOFs) are described systematically based on hydrogen‐bonding patterns (supramolecular synthons) and molecular structures (tectons). HOFs can show thermal and chemical durability, a large surface area, and permanent porosity.
AbstractList	Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self‐standing porous molecular crystals (PMCs). Particularly, a number of crystalline systems with permanent porosity that are formed by self‐assembly through hydrogen bonding (H‐bonding) have been developed. Such systems are called hydrogen‐bonded organic frameworks (HOFs). Herein we systematically describe H‐bonding patterns (supramolecular synthons) and molecular structures (tectons) that have been used to achieve thermal and chemical durability, a large surface area, and functions, such as selective gas sorption and separation, which can provide design principles for constructing HOFs with permanent porosity. Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self-standing porous molecular crystals (PMCs). Particularly, a number of crystalline systems with permanent porosity that are formed by self-assembly through hydrogen bonding (H-bonding) have been developed. Such systems are called hydrogen-bonded organic frameworks (HOFs). Herein we systematically describe H-bonding patterns (supramolecular synthons) and molecular structures (tectons) that have been used to achieve thermal and chemical durability, a large surface area, and functions, such as selective gas sorption and separation, which can provide design principles for constructing HOFs with permanent porosity.Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self-standing porous molecular crystals (PMCs). Particularly, a number of crystalline systems with permanent porosity that are formed by self-assembly through hydrogen bonding (H-bonding) have been developed. Such systems are called hydrogen-bonded organic frameworks (HOFs). Herein we systematically describe H-bonding patterns (supramolecular synthons) and molecular structures (tectons) that have been used to achieve thermal and chemical durability, a large surface area, and functions, such as selective gas sorption and separation, which can provide design principles for constructing HOFs with permanent porosity. Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous materials has seen a resurgence in the past decade as a result of finding of self‐standing porous molecular crystals (PMCs). Particularly, a number of crystalline systems with permanent porosity that are formed by self‐assembly through hydrogen bonding (H‐bonding) have been developed. Such systems are called hydrogen‐bonded organic frameworks (HOFs). Herein we systematically describe H‐bonding patterns (supramolecular synthons) and molecular structures (tectons) that have been used to achieve thermal and chemical durability, a large surface area, and functions, such as selective gas sorption and separation, which can provide design principles for constructing HOFs with permanent porosity. HOF the shelf: Hydrogen‐bonded organic frameworks (HOFs) are described systematically based on hydrogen‐bonding patterns (supramolecular synthons) and molecular structures (tectons). HOFs can show thermal and chemical durability, a large surface area, and permanent porosity.
Author	Xin, Chen Hisaki, Ichiro Takahashi, Kiyonori Nakamura, Takayoshi
Author_xml	– sequence: 1 givenname: Ichiro orcidid: 0000-0002-8170-5605 surname: Hisaki fullname: Hisaki, Ichiro email: hisaki@es.hokudai.ac.jp organization: Hokkaido University, N10W5 – sequence: 2 givenname: Chen surname: Xin fullname: Xin, Chen organization: Hokkaido University, N10W5 – sequence: 3 givenname: Kiyonori surname: Takahashi fullname: Takahashi, Kiyonori organization: Hokkaido University, N10W5 – sequence: 4 givenname: Takayoshi surname: Nakamura fullname: Nakamura, Takayoshi organization: Hokkaido University, N10W5
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/30891889$$D View this record in MEDLINE/PubMed
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Snippet	Designing organic components that can be used to construct porous materials enables the preparation of tailored functionalized materials. Research into porous...
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SubjectTerms	Construction materials Crystals gas sorption Hydrogen Hydrogen bonding hydrogen bonds hydrogen-bonded organic frameworks (HOFs) Organic chemistry permanent porosity Porosity Porous materials
Title	Designing Hydrogen‐Bonded Organic Frameworks (HOFs) with Permanent Porosity
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