Correlating the role of nanofillers with active layer properties and performance of thin-film nanocomposite membranes

Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties...

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Vydáno v:Desalination Ročník 550; číslo C; s. 116370
Hlavní autoři: Perry, Lamar A., Chew, Nick Guan Pin, Grzebyk, Kasia, Cay-Durgun, Pinar, Lind, Mary Laura, Sitaula, Paban, Soukri, Mustapha, Coronell, Orlando
Médium: Journal Article
Jazyk:angličtina
Vydáno: Netherlands Elsevier B.V 15.03.2023
Elsevier
Témata:
ENGINEERING
Membrane
MembraneZIF-8
Polyamide
Thin-film nanocomposite
Zeolite
Zeolitic imidazolate framework
ZIF-8
Polyamide
Thin-film nanocomposite
Zeolitic imidazolate framework
Membrane
Zeolite
ZIF-8
ISSN:0011-9164
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Abstract Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. The effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9–25.6 % and 26.1–48.3 % for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations. [Display omitted] •Nanofillers were embedded into TFN active layers at <1 at.%.•Physico-chemical characterizations of active layers were representative of polymer.•Salt rejection above nanofiller loading threshold of ~0.15 wt% was markedly lower.•Changes in membrane physico-chemical properties and performance were not correlated.•Flow through nanofiller/along nanofiller-polymer interface likely boosts permeance.
AbstractList Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. Throughout this work, the effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9–25.6 % and 26.1–48.3 % for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations.
Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. The effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9–25.6% and 26.1–48.3% for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations.
Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. The effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9-25.6% and 26.1-48.3% for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations.Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. The effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9-25.6% and 26.1-48.3% for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations.
Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over traditional thin-film composite (TFC) membranes. However, the effects of nanofiller incorporation on active layer physico-chemical properties have not been comprehensively studied. Accordingly, we aimed to understand the correlation between nanofillers, active layer physico-chemical properties, and membrane performance by investigating whether observed performance differences between TFN and control TFC membranes correlated with observed differences in physico-chemical properties. The effects of nanofiller loading, surface area, and size on membrane performance, along with active layer physico-chemical properties, were characterized in TFN membranes incorporated with Linde Type A (LTA) zeolite and zeolitic imidazole framework-8 (ZIF-8). Results show that nanofiller incorporation up to ~0.15 wt% resulted in higher water permeance and unchanged salt rejection, above which salt rejection decreased 0.9–25.6 % and 26.1–48.3 % for LTA-TFN and ZIF-8-TFN membranes, respectively. Observed changes in active layer physico-chemical properties were generally unsubstantial and did not explain observed changes in TFN membrane performance. Therefore, increased water permeance in TFN membranes could be due to preferential water transport through porous structures of nanofillers or along polymer-nanofiller interfaces. These findings offer new insights into the development of high-performance TFN membranes for water/ion separations. [Display omitted] •Nanofillers were embedded into TFN active layers at <1 at.%.•Physico-chemical characterizations of active layers were representative of polymer.•Salt rejection above nanofiller loading threshold of ~0.15 wt% was markedly lower.•Changes in membrane physico-chemical properties and performance were not correlated.•Flow through nanofiller/along nanofiller-polymer interface likely boosts permeance.
ArticleNumber 116370
Author Perry, Lamar A.
Sitaula, Paban
Coronell, Orlando
Soukri, Mustapha
Chew, Nick Guan Pin
Lind, Mary Laura
Grzebyk, Kasia
Cay-Durgun, Pinar
AuthorAffiliation c School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, AZ 85287, USA
a Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7431, USA
d RTI International, 3040 East Cornwallis Road, Research Triangle Park, Durham, NC 27709-2194, USA
b Curriculum in Applied Sciences and Engineering, The University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7431, USA
AuthorAffiliation_xml – name: d RTI International, 3040 East Cornwallis Road, Research Triangle Park, Durham, NC 27709-2194, USA
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– name: b Curriculum in Applied Sciences and Engineering, The University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7431, USA
– name: c School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, AZ 85287, USA
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  surname: Perry
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  givenname: Nick Guan Pin
  surname: Chew
  fullname: Chew, Nick Guan Pin
  organization: Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7431, USA
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  givenname: Kasia
  surname: Grzebyk
  fullname: Grzebyk, Kasia
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  givenname: Pinar
  surname: Cay-Durgun
  fullname: Cay-Durgun, Pinar
  organization: School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, AZ 85287, USA
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  givenname: Mary Laura
  surname: Lind
  fullname: Lind, Mary Laura
  organization: School for Engineering of Matter, Transport, and Energy, Arizona State University, Tempe, AZ 85287, USA
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  givenname: Paban
  surname: Sitaula
  fullname: Sitaula, Paban
  organization: RTI International, 3040 East Cornwallis Road, Research Triangle Park, Durham, NC 27709-2194, USA
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  givenname: Mustapha
  surname: Soukri
  fullname: Soukri, Mustapha
  organization: RTI International, 3040 East Cornwallis Road, Research Triangle Park, Durham, NC 27709-2194, USA
– sequence: 8
  givenname: Orlando
  surname: Coronell
  fullname: Coronell, Orlando
  email: coronell@unc.edu
  organization: Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC 27599-7431, USA
BackLink https://www.ncbi.nlm.nih.gov/pubmed/37274380$$D View this record in MEDLINE/PubMed
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ISSN 0011-9164
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Issue C
Keywords Polyamide
Thin-film nanocomposite
Zeolitic imidazolate framework
Membrane
Zeolite
ZIF-8
Language English
LinkModel OpenURL
MergedId FETCHMERGED-LOGICAL-c487t-83b07c08c2af69bbea1df6c222eb5198cb0f68536dd76f64b2ea6f86b5ac4a983
Notes ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
National Institute of Environmental Health Sciences (NIEHS)
FG02-97ER41033; FG02-97ER41041; 1264690; 1336532; ECCS-2025064; P42ES031007
National Science Foundation (NSF)
USDOE Office of Science (SC), Nuclear Physics (NP)
OpenAccessLink https://www.osti.gov/servlets/purl/2419506
PMID 37274380
PQID 2822706897
PQPubID 23479
ParticipantIDs pubmedcentral_primary_oai_pubmedcentral_nih_gov_10237506
osti_scitechconnect_2419506
proquest_miscellaneous_2822706897
pubmed_primary_37274380
crossref_primary_10_1016_j_desal_2023_116370
crossref_citationtrail_10_1016_j_desal_2023_116370
elsevier_sciencedirect_doi_10_1016_j_desal_2023_116370
PublicationCentury 2000
PublicationDate 2023-03-15
PublicationDateYYYYMMDD 2023-03-15
PublicationDate_xml – month: 03
  year: 2023
  text: 2023-03-15
  day: 15
PublicationDecade 2020
PublicationPlace Netherlands
PublicationPlace_xml – name: Netherlands
– name: United States
PublicationTitle Desalination
PublicationTitleAlternate Desalination
PublicationYear 2023
Publisher Elsevier B.V
Elsevier
Publisher_xml – name: Elsevier B.V
– name: Elsevier
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SSID ssj0012933
Score 2.4566371
Snippet Thin-film nanocomposite (TFN) membranes are emerging water-purification membranes that could provide enhanced water permeance with similar solute removal over...
SourceID pubmedcentral
osti
proquest
pubmed
crossref
elsevier
SourceType Open Access Repository
Aggregation Database
Index Database
Enrichment Source
Publisher
StartPage 116370
SubjectTerms ENGINEERING
Membrane
MembraneZIF-8
Polyamide
Thin-film nanocomposite
Zeolite
Zeolitic imidazolate framework
ZIF-8
Title Correlating the role of nanofillers with active layer properties and performance of thin-film nanocomposite membranes
URI https://dx.doi.org/10.1016/j.desal.2023.116370
https://www.ncbi.nlm.nih.gov/pubmed/37274380
https://www.proquest.com/docview/2822706897
https://www.osti.gov/servlets/purl/2419506
https://pubmed.ncbi.nlm.nih.gov/PMC10237506
Volume 550
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