Double Single-Crystal-to-Single-Crystal Transformation and Small-Molecule Activation in Rhodium NHC Complexes
Three gases, one crystal: Rhodium NHC complexes undergo back‐to‐back single‐crystal‐to‐single‐crystal transformations by selective nonreversible ligand exchange reactions (see picture). Slow diffusion of O2 converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O2....
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| Vydáno v: | Angewandte Chemie International Edition Ročník 50; číslo 35; s. 8100 - 8104 |
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Weinheim
WILEY-VCH Verlag
22.08.2011
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Vydání: | International ed. in English |
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| ISSN: | 1433-7851, 1521-3773, 1521-3773 |
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| Abstract | Three gases, one crystal: Rhodium NHC complexes undergo back‐to‐back single‐crystal‐to‐single‐crystal transformations by selective nonreversible ligand exchange reactions (see picture). Slow diffusion of O2 converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O2. |
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| AbstractList | Three gases, one crystal: Rhodium NHC complexes undergo back‐to‐back single‐crystal‐to‐single‐crystal transformations by selective nonreversible ligand exchange reactions (see picture). Slow diffusion of O2 converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O2. Three gases, one crystal: rhodium NHC complexes undergo back-to-back single-crystal-to-single-crystal transformations by selective nonreversible ligand exchange reactions. Slow diffusion of O(2) converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O(2).Three gases, one crystal: rhodium NHC complexes undergo back-to-back single-crystal-to-single-crystal transformations by selective nonreversible ligand exchange reactions. Slow diffusion of O(2) converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O(2). Three gases, one crystal: rhodium NHC complexes undergo back-to-back single-crystal-to-single-crystal transformations by selective nonreversible ligand exchange reactions. Slow diffusion of O(2) converts a dinitrogen complex into a dioxygen complex, and CO subsequently replaces O(2). |
| Author | Keske, Eric C. Wang, Ruiyao Crudden, Cathleen M. Zenkina, Olena V. |
| Author_xml | – sequence: 1 givenname: Olena V. surname: Zenkina fullname: Zenkina, Olena V. organization: Department of Chemistry, Queen's University, Chernoff Hall, 90 Bader Lane, Kingston, Ontario (Canada) http://www.cruddengroup.com – sequence: 2 givenname: Eric C. surname: Keske fullname: Keske, Eric C. organization: Department of Chemistry, Queen's University, Chernoff Hall, 90 Bader Lane, Kingston, Ontario (Canada) http://www.cruddengroup.com – sequence: 3 givenname: Ruiyao surname: Wang fullname: Wang, Ruiyao organization: Department of Chemistry, Queen's University, Chernoff Hall, 90 Bader Lane, Kingston, Ontario (Canada) http://www.cruddengroup.com – sequence: 4 givenname: Cathleen M. surname: Crudden fullname: Crudden, Cathleen M. email: cathleen.crudden@chem.queensu.ca organization: Department of Chemistry, Queen's University, Chernoff Hall, 90 Bader Lane, Kingston, Ontario (Canada) http://www.cruddengroup.com |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/21744453$$D View this record in MEDLINE/PubMed |
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| Notes | ark:/67375/WNG-VJ69K53W-2 The National Sciences and Engineering Research Council of Canada (NSERC) is gratefully acknowledged for support of this research, and Johnson Matthey is acknowledged for a gift of [{Rh(C2H4)2Cl}2]. NHC=N-heterocyclic carbene. National Sciences and Engineering Research Council of Canada (NSERC) ArticleID:ANIE201103316 istex:226BB9029FC69C5566A8B32B450CFC4E9E69B428 2 4 NHC=N‐heterocyclic carbene. H The National Sciences and Engineering Research Council of Canada (NSERC) is gratefully acknowledged for support of this research, and Johnson Matthey is acknowledged for a gift of [{Rh(C ) Cl ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 |
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| Snippet | Three gases, one crystal: Rhodium NHC complexes undergo back‐to‐back single‐crystal‐to‐single‐crystal transformations by selective nonreversible ligand... Three gases, one crystal: rhodium NHC complexes undergo back-to-back single-crystal-to-single-crystal transformations by selective nonreversible ligand... |
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| SubjectTerms | hydrides N-heterocyclic carbenes Rhodium single-crystal reactions X-ray diffraction |
| Title | Double Single-Crystal-to-Single-Crystal Transformation and Small-Molecule Activation in Rhodium NHC Complexes |
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