Semiconductive Copper(I)–Organic Frameworks for Efficient Light‐Driven Hydrogen Generation Without Additional Photosensitizers and Cocatalysts

As the first example of a photocatalytic system for splitting water without additional cocatalysts and photosensitizers, the comparatively cost‐effective Cu2I2‐based MOF, Cu‐I‐bpy (bpy=4,4′‐bipyridine) exhibited highly efficient photocatalytic hydrogen production (7.09 mmol g−1 h−1). Density functio...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 56; H. 46; S. 14637 - 14641
Hauptverfasser:	Shi, Dongying, Zheng, Rui, Sun, Ming‐Jun, Cao, Xinrui, Sun, Chun‐Xiao, Cui, Chao‐Jie, Liu, Chun‐Sen, Zhao, Junwei, Du, Miao
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 13.11.2017
Ausgabe:	International ed. in English
Schlagworte:	Copper copper(I) halides Density functional theory Hydrogen Hydrogen evolution hydrogen generation Hydrogen production Hydrogen storage metal–organic frameworks Photocatalysis Redox reactions semiconductors Splitting photocatalysis semiconductors copper(I) halides hydrogen generation metal-organic frameworks
ISSN:	1433-7851, 1521-3773, 1521-3773
Online-Zugang:	Volltext
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