Graphene Nanoarchitectonics: Recent Advances in Graphene‐Based Electrocatalysts for Hydrogen Evolution Reaction

Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy‐production and energy‐consumption systems. In this regard, the...

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Veröffentlicht in:Advanced materials (Weinheim) Jg. 31; H. 48; S. e1903415 - n/a
Hauptverfasser: Huang, Huajie, Yan, Minmin, Yang, Cuizhen, He, Haiyan, Jiang, Quanguo, Yang, Lu, Lu, Zhiyong, Sun, Ziqi, Xu, Xingtao, Bando, Yoshio, Yamauchi, Yusuke
Format: Journal Article
Sprache:Englisch
Veröffentlicht: Germany Wiley Subscription Services, Inc 01.11.2019
Schlagworte:
Electrical resistivity
Electrocatalysts
Graphene
hybrid structures
Hydrogen
hydrogen evolution reaction
Hydrogen evolution reactions
Hydrogen fuels
Hydrogen production
Mass production
Materials science
nanoparticles
Organic chemistry
Sustainable development
electrocatalysts
hybrid structures
nanoparticles
graphene
hydrogen evolution reaction
ISSN:0935-9648, 1521-4095, 1521-4095
Online-Zugang:Volltext
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Abstract Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy‐production and energy‐consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene‐based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene‐based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed. Electrode catalysts for the hydrogen evolution reaction are at the heart of electrochemical water splitting technology. Recent advances in the controllable synthesis, microstructural analysis, and electrocatalytic properties of graphene‐based hydrogen evolution electrocatalysts are presented, together with a discussion of the major challenges and opportunities in this emerging field.
AbstractList Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy-production and energy-consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene-based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene-based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed.
Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy‐production and energy‐consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene‐based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene‐based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed. Electrode catalysts for the hydrogen evolution reaction are at the heart of electrochemical water splitting technology. Recent advances in the controllable synthesis, microstructural analysis, and electrocatalytic properties of graphene‐based hydrogen evolution electrocatalysts are presented, together with a discussion of the major challenges and opportunities in this emerging field.
Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy-production and energy-consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene-based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene-based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed.Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy-production and energy-consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene-based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene-based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed.
Author Xu, Xingtao
Yan, Minmin
Yang, Lu
Yang, Cuizhen
Lu, Zhiyong
Bando, Yoshio
Huang, Huajie
Jiang, Quanguo
Sun, Ziqi
He, Haiyan
Yamauchi, Yusuke
Author_xml – sequence: 1
  givenname: Huajie
  surname: Huang
  fullname: Huang, Huajie
  email: huanghuajie@hhu.edu.cn
  organization: Hohai University
– sequence: 2
  givenname: Minmin
  surname: Yan
  fullname: Yan, Minmin
  organization: Hohai University
– sequence: 3
  givenname: Cuizhen
  surname: Yang
  fullname: Yang, Cuizhen
  organization: Hohai University
– sequence: 4
  givenname: Haiyan
  surname: He
  fullname: He, Haiyan
  organization: Hohai University
– sequence: 5
  givenname: Quanguo
  surname: Jiang
  fullname: Jiang, Quanguo
  organization: Hohai University
– sequence: 6
  givenname: Lu
  surname: Yang
  fullname: Yang, Lu
  organization: Hohai University
– sequence: 7
  givenname: Zhiyong
  surname: Lu
  fullname: Lu, Zhiyong
  organization: Hohai University
– sequence: 8
  givenname: Ziqi
  surname: Sun
  fullname: Sun, Ziqi
  organization: Queensland University of Technology (QUT)
– sequence: 9
  givenname: Xingtao
  surname: Xu
  fullname: Xu, Xingtao
  email: xingtao.xu@hhu.eduv
  organization: Hohai University
– sequence: 10
  givenname: Yoshio
  surname: Bando
  fullname: Bando, Yoshio
  organization: National Institute for Materials Science
– sequence: 11
  givenname: Yusuke
  orcidid: 0000-0001-7854-927X
  surname: Yamauchi
  fullname: Yamauchi, Yusuke
  email: y.yamauchi@uq.edu.au
  organization: Kyung Hee University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31496036$$D View this record in MEDLINE/PubMed
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Keywords electrocatalysts
hybrid structures
nanoparticles
graphene
hydrogen evolution reaction
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2014 2018 2018 2015 2016 2017; 74 284 43 16 219 499
2014; 53
2013 2018 2018 2017 2015 2017 2018 2015 2015; 23 3 283 315 3 5 13 9 9
2015; 2
2015; 12
2018 2017; 11 5
2015; 16
2017 2016 2016 2016; 5 4 4 8
2015; 3
2012 2011; 5 4
2017 2015; 121 3
2015; 11
2016; 52
2015 2017 2017 2015; 6 8 7 137
2015 2018; 7 265
2008 2018 2012 2012; 3 6 204 22
2017 2018 2017 2017 2016 2018 2015; 29 10 232 9 100 6 285
2015; 7
2013 2016; 49 3
2016; 55
2007 2008; 6 3
2013 2016; 135 16
2015; 25
2015; 27
2018 2017 2016 2016 2017 2017; 47 255 4 4 5 29
2015 2016; 3 4
2016 2016 2016 2015 2015 2014 2014 2016 2015 2016 2015 2015; 8 107 222 3 7 6 2 22 119 8 51 293
2017; 11
2016 2016; 219 107
2016 2015 2015; 52 3 7
2015; 21
2016 2018 2017 2017 2019; 4 397 29 9 31
2016 2017 2018 2016 2018 2016 2017; 29 9 513 85 24 509 9
2013 2016 2018; 135 28 9
2016; 138
2018; 50
2009; 2
2018; 57
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Snippet Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power...
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SubjectTerms Electrical resistivity
Electrocatalysts
Graphene
hybrid structures
Hydrogen
hydrogen evolution reaction
Hydrogen evolution reactions
Hydrogen fuels
Hydrogen production
Mass production
Materials science
nanoparticles
Organic chemistry
Sustainable development
Title Graphene Nanoarchitectonics: Recent Advances in Graphene‐Based Electrocatalysts for Hydrogen Evolution Reaction
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201903415
https://www.ncbi.nlm.nih.gov/pubmed/31496036
https://www.proquest.com/docview/2317574598
https://www.proquest.com/docview/2287533234
Volume 31
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