C−H Functionalization of Commodity Polymers

Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high‐volume and low‐cost production of...

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Vydané v:Angewandte Chemie International Edition Ročník 58; číslo 26; s. 8654 - 8668
Hlavní autori: Williamson, Jill B., Lewis, Sally E., Johnson, Robert R., Manning, Irene M., Leibfarth, Frank A.
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: Germany Wiley Subscription Services, Inc 24.06.2019
Vydanie:International ed. in English
Predmet:
Catalysis
Commodities
C−H functionalization
Material properties
Organic chemistry
Photoredox catalysis
Plastic debris
Polymers
Substrates
sustainable chemistry
synthetic methods
upcycling
C−H functionalization
sustainable chemistry
polymers
upcycling
synthetic methods
ISSN:1433-7851, 1521-3773, 1521-3773
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Abstract Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high‐volume and low‐cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C−H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C−H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C−H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post‐consumer plastic waste. Hot commodities: This Review discusses the historical significance of and contemporary advances in the C−H functionalization of commodity polymers. Exciting new directions for the field are presented, including uncovering new material properties and upcycling post‐consumer plastic waste.
AbstractList Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high‐volume and low‐cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C−H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C−H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C−H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post‐consumer plastic waste.
Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high-volume and low-cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C-H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C-H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C-H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post-consumer plastic waste.
Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high-volume and low-cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C-H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C-H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C-H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post-consumer plastic waste.Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high-volume and low-cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C-H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C-H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C-H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post-consumer plastic waste.
Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying the chemical structure of polymers that are already produced on a commodity scale leverages the current high‐volume and low‐cost production of commodity plastics for the discovery of modern materials. A myriad of polymer C−H functionalization methods have been developed which enable the modification of material properties on both a laboratory and industrial scale. More recently, driven by advances in C−H activation, photoredox catalysis, and radical chemistry, chemoselective approaches have emerged as a means to impart precise functionality onto commodity polymer substrates. This Review discusses the historical significance of and contemporary advances in the C−H functionalization of commodity polymers. The conceptual approach outlined herein presents exciting new directions for the field, including increasing the value of otherwise pervasive materials, uncovering entirely new material properties, and a viable path to upcycle post‐consumer plastic waste. Hot commodities: This Review discusses the historical significance of and contemporary advances in the C−H functionalization of commodity polymers. Exciting new directions for the field are presented, including uncovering new material properties and upcycling post‐consumer plastic waste.
Author Johnson, Robert R.
Williamson, Jill B.
Manning, Irene M.
Lewis, Sally E.
Leibfarth, Frank A.
Author_xml – sequence: 1
  givenname: Jill B.
  orcidid: 0000-0002-9780-1343
  surname: Williamson
  fullname: Williamson, Jill B.
  organization: The University of North Carolina at Chapel Hill
– sequence: 2
  givenname: Sally E.
  orcidid: 0000-0002-0854-2141
  surname: Lewis
  fullname: Lewis, Sally E.
  organization: The University of North Carolina at Chapel Hill
– sequence: 3
  givenname: Robert R.
  orcidid: 0000-0001-5256-5853
  surname: Johnson
  fullname: Johnson, Robert R.
  organization: The University of North Carolina at Chapel Hill
– sequence: 4
  givenname: Irene M.
  orcidid: 0000-0001-7369-0709
  surname: Manning
  fullname: Manning, Irene M.
  organization: The University of North Carolina at Chapel Hill
– sequence: 5
  givenname: Frank A.
  orcidid: 0000-0001-7737-0331
  surname: Leibfarth
  fullname: Leibfarth, Frank A.
  email: FrankL@email.unc.edu
  organization: The University of North Carolina at Chapel Hill
BackLink https://www.ncbi.nlm.nih.gov/pubmed/30450640$$D View this record in MEDLINE/PubMed
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sustainable chemistry
polymers
upcycling
synthetic methods
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Snippet Synthetic manipulation of polymer substrates is one of the oldest and most reliable methods to increase the functional diversity of soft materials. Modifying...
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SubjectTerms Catalysis
Commodities
C−H functionalization
Material properties
Organic chemistry
Photoredox catalysis
Plastic debris
Polymers
Substrates
sustainable chemistry
synthetic methods
upcycling
Title C−H Functionalization of Commodity Polymers
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201810970
https://www.ncbi.nlm.nih.gov/pubmed/30450640
https://www.proquest.com/docview/2239485919
https://www.proquest.com/docview/2135641939
Volume 58
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