Advanced Chemical Looping Materials for CO2 Utilization: A Review

Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO2-emission energy production. Bridged by the cyclic transformation of a looping material (CO2 carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporal...

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Vydáno v:Materials Ročník 11; číslo 7; s. 1187
Hlavní autoři: Hu, Jiawei, Galvita, Vladimir V., Poelman, Hilde, Marin, Guy B.
Médium: Journal Article
Jazyk:angličtina
Vydáno: Switzerland MDPI AG 10.07.2018
MDPI
Témata:
Carbon dioxide
Carbon sequestration
Catalysts
Catalytic converters
Chemicals
Climate change
Conversion
Decomposition
Efficiency
Emissions
Energy resources
Fluidized bed combustion
Fossil fuels
Fuels
Greenhouse gases
Industrial applications
Industrial plant emissions
Iron
Materials selection
Metal oxides
Nanomaterials
Natural gas
Nickel
Nuclear power plants
Organic chemistry
Oxygen
Reduction
Reforming
Review
Stability
Synthesis gas
Utilization
Value added
Ceram
structured nanomaterials
metal oxides
CH4 reforming
catalyst-assisted chemical looping
oxygen carrier
bifunctional materials
core-shell
ISSN:1996-1944, 1996-1944
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Abstract Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO2-emission energy production. Bridged by the cyclic transformation of a looping material (CO2 carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporally separated half-cycles. Firstly, the oxygen carrier material is reduced by fuel, producing power or chemicals. Then, the material is regenerated by an oxidizer. In chemical looping combustion, a separation-ready CO2 stream is produced, which significantly improves the CO2 capture efficiency. In chemical looping reforming, CO2 can be used as an oxidizer, resulting in a novel approach for efficient CO2 utilization through reduction to CO. Recently, the novel process of catalyst-assisted chemical looping was proposed, aiming at maximized CO2 utilization via the achievement of deep reduction of the oxygen carrier in the first half-cycle. It makes use of a bifunctional looping material that combines both catalytic function for efficient fuel conversion and oxygen storage function for redox cycling. For all of these chemical looping technologies, the choice of looping materials is crucial for their industrial application. Therefore, current research is focused on the development of a suitable looping material, which is required to have high redox activity and stability, and good economic and environmental performance. In this review, a series of commonly used metal oxide-based materials are firstly compared as looping material from an industrial-application perspective. The recent advances in the enhancement of the activity and stability of looping materials are discussed. The focus then proceeds to new findings in the development of the bifunctional looping materials employed in the emerging catalyst-assisted chemical looping technology. Among these, the design of core-shell structured Ni-Fe bifunctional nanomaterials shows great potential for catalyst-assisted chemical looping.
AbstractList Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO2-emission energy production. Bridged by the cyclic transformation of a looping material (CO2 carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporally separated half-cycles. Firstly, the oxygen carrier material is reduced by fuel, producing power or chemicals. Then, the material is regenerated by an oxidizer. In chemical looping combustion, a separation-ready CO2 stream is produced, which significantly improves the CO2 capture efficiency. In chemical looping reforming, CO2 can be used as an oxidizer, resulting in a novel approach for efficient CO2 utilization through reduction to CO. Recently, the novel process of catalyst-assisted chemical looping was proposed, aiming at maximized CO2 utilization via the achievement of deep reduction of the oxygen carrier in the first half-cycle. It makes use of a bifunctional looping material that combines both catalytic function for efficient fuel conversion and oxygen storage function for redox cycling. For all of these chemical looping technologies, the choice of looping materials is crucial for their industrial application. Therefore, current research is focused on the development of a suitable looping material, which is required to have high redox activity and stability, and good economic and environmental performance. In this review, a series of commonly used metal oxide-based materials are firstly compared as looping material from an industrial-application perspective. The recent advances in the enhancement of the activity and stability of looping materials are discussed. The focus then proceeds to new findings in the development of the bifunctional looping materials employed in the emerging catalyst-assisted chemical looping technology. Among these, the design of core-shell structured Ni-Fe bifunctional nanomaterials shows great potential for catalyst-assisted chemical looping.
Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO₂-emission energy production. Bridged by the cyclic transformation of a looping material (CO₂ carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporally separated half-cycles. Firstly, the oxygen carrier material is reduced by fuel, producing power or chemicals. Then, the material is regenerated by an oxidizer. In chemical looping combustion, a separation-ready CO₂ stream is produced, which significantly improves the CO₂ capture efficiency. In chemical looping reforming, CO₂ can be used as an oxidizer, resulting in a novel approach for efficient CO₂ utilization through reduction to CO. Recently, the novel process of catalyst-assisted chemical looping was proposed, aiming at maximized CO₂ utilization via the achievement of deep reduction of the oxygen carrier in the first half-cycle. It makes use of a bifunctional looping material that combines both catalytic function for efficient fuel conversion and oxygen storage function for redox cycling. For all of these chemical looping technologies, the choice of looping materials is crucial for their industrial application. Therefore, current research is focused on the development of a suitable looping material, which is required to have high redox activity and stability, and good economic and environmental performance. In this review, a series of commonly used metal oxide-based materials are firstly compared as looping material from an industrial-application perspective. The recent advances in the enhancement of the activity and stability of looping materials are discussed. The focus then proceeds to new findings in the development of the bifunctional looping materials employed in the emerging catalyst-assisted chemical looping technology. Among these, the design of core-shell structured Ni-Fe bifunctional nanomaterials shows great potential for catalyst-assisted chemical looping.Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO₂-emission energy production. Bridged by the cyclic transformation of a looping material (CO₂ carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporally separated half-cycles. Firstly, the oxygen carrier material is reduced by fuel, producing power or chemicals. Then, the material is regenerated by an oxidizer. In chemical looping combustion, a separation-ready CO₂ stream is produced, which significantly improves the CO₂ capture efficiency. In chemical looping reforming, CO₂ can be used as an oxidizer, resulting in a novel approach for efficient CO₂ utilization through reduction to CO. Recently, the novel process of catalyst-assisted chemical looping was proposed, aiming at maximized CO₂ utilization via the achievement of deep reduction of the oxygen carrier in the first half-cycle. It makes use of a bifunctional looping material that combines both catalytic function for efficient fuel conversion and oxygen storage function for redox cycling. For all of these chemical looping technologies, the choice of looping materials is crucial for their industrial application. Therefore, current research is focused on the development of a suitable looping material, which is required to have high redox activity and stability, and good economic and environmental performance. In this review, a series of commonly used metal oxide-based materials are firstly compared as looping material from an industrial-application perspective. The recent advances in the enhancement of the activity and stability of looping materials are discussed. The focus then proceeds to new findings in the development of the bifunctional looping materials employed in the emerging catalyst-assisted chemical looping technology. Among these, the design of core-shell structured Ni-Fe bifunctional nanomaterials shows great potential for catalyst-assisted chemical looping.
Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO₂-emission energy production. Bridged by the cyclic transformation of a looping material (CO₂ carrier or oxygen carrier), a chemical looping process is divided into two spatially or temporally separated half-cycles. Firstly, the oxygen carrier material is reduced by fuel, producing power or chemicals. Then, the material is regenerated by an oxidizer. In chemical looping combustion, a separation-ready CO₂ stream is produced, which significantly improves the CO₂ capture efficiency. In chemical looping reforming, CO₂ can be used as an oxidizer, resulting in a novel approach for efficient CO₂ utilization through reduction to CO. Recently, the novel process of catalyst-assisted chemical looping was proposed, aiming at maximized CO₂ utilization via the achievement of deep reduction of the oxygen carrier in the first half-cycle. It makes use of a bifunctional looping material that combines both catalytic function for efficient fuel conversion and oxygen storage function for redox cycling. For all of these chemical looping technologies, the choice of looping materials is crucial for their industrial application. Therefore, current research is focused on the development of a suitable looping material, which is required to have high redox activity and stability, and good economic and environmental performance. In this review, a series of commonly used metal oxide-based materials are firstly compared as looping material from an industrial-application perspective. The recent advances in the enhancement of the activity and stability of looping materials are discussed. The focus then proceeds to new findings in the development of the bifunctional looping materials employed in the emerging catalyst-assisted chemical looping technology. Among these, the design of core-shell structured Ni-Fe bifunctional nanomaterials shows great potential for catalyst-assisted chemical looping.
Author Marin, Guy B.
Galvita, Vladimir V.
Poelman, Hilde
Hu, Jiawei
AuthorAffiliation Laboratory for Chemical Technology, Ghent University, Technologiepark 914, B-9052 Ghent, Belgium; Jiawei.Hu@UGent.be (J.H.); Hilde.Poelman@UGent.be (H.P.); Guy.Marin@UGent.be (G.B.M.)
AuthorAffiliation_xml – name: Laboratory for Chemical Technology, Ghent University, Technologiepark 914, B-9052 Ghent, Belgium; Jiawei.Hu@UGent.be (J.H.); Hilde.Poelman@UGent.be (H.P.); Guy.Marin@UGent.be (G.B.M.)
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  givenname: Jiawei
  orcidid: 0000-0003-0792-054X
  surname: Hu
  fullname: Hu, Jiawei
– sequence: 2
  givenname: Vladimir V.
  orcidid: 0000-0001-9205-7917
  surname: Galvita
  fullname: Galvita, Vladimir V.
– sequence: 3
  givenname: Hilde
  orcidid: 0000-0003-4267-7397
  surname: Poelman
  fullname: Poelman, Hilde
– sequence: 4
  givenname: Guy B.
  surname: Marin
  fullname: Marin, Guy B.
BackLink https://www.ncbi.nlm.nih.gov/pubmed/29996567$$D View this record in MEDLINE/PubMed
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ContentType Journal Article
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2018 by the authors. 2018
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Issue 7
Keywords structured nanomaterials
metal oxides
CH4 reforming
catalyst-assisted chemical looping
oxygen carrier
bifunctional materials
core-shell
Language English
License Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
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Snippet Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO2-emission energy production. Bridged by the...
Combining chemical looping with a traditional fuel conversion process yields a promising technology for low-CO₂-emission energy production. Bridged by the...
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StartPage 1187
SubjectTerms Carbon dioxide
Carbon sequestration
Catalysts
Catalytic converters
Chemicals
Climate change
Conversion
Decomposition
Efficiency
Emissions
Energy resources
Fluidized bed combustion
Fossil fuels
Fuels
Greenhouse gases
Industrial applications
Industrial plant emissions
Iron
Materials selection
Metal oxides
Nanomaterials
Natural gas
Nickel
Nuclear power plants
Organic chemistry
Oxygen
Reduction
Reforming
Review
Stability
Synthesis gas
Utilization
Value added
Title Advanced Chemical Looping Materials for CO2 Utilization: A Review
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Volume 11
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