Heavy metal pollution caused by small-scale metal ore mining activities: A case study from a polymetallic mine in South China

Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic min...

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Veröffentlicht in:The Science of the total environment Jg. 639; S. 217 - 227
Hauptverfasser: Sun, Zehang, Xie, Xiande, Wang, Ping, Hu, Yuanan, Cheng, Hefa
Format: Journal Article
Sprache:Englisch
Veröffentlicht: Netherlands Elsevier B.V 15.10.2018
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ISSN:0048-9697, 1879-1026, 1879-1026
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Abstract Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739–4.15 × 103, 1.81 × 103–5.00 × 103, 118–1.26 × 103, 8.14–57.7, and 1.23 × 103–6.99 × 103 mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4–17.9 mg/L for Cu, 21.1–29.3 mg/L for Zn, 0.553–0.770 mg/L for Cd, and 1.17–2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines. [Display omitted] •Heavy metal pollution in a small-scale metal ore mining area was investigated.•Pollution generally decreased with increasing distance from the mining district.•Cu, Zn, Cd, and Pb in local farmland soils came primarily from the mining activities.•Heavy metal pollution of local farmland soils posed high potential ecological risk.•Significant attention needs to be paid to the dumped tailings of small-scale mines.
AbstractList Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739-4.15 × 10 , 1.81 × 10 -5.00 × 10 , 118-1.26 × 10 , 8.14-57.7, and 1.23 × 10 -6.99 × 10  mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4-17.9 mg/L for Cu, 21.1-29.3 mg/L for Zn, 0.553-0.770 mg/L for Cd, and 1.17-2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines.
Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739-4.15 × 103, 1.81 × 103-5.00 × 103, 118-1.26 × 103, 8.14-57.7, and 1.23 × 103-6.99 × 103 mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4-17.9 mg/L for Cu, 21.1-29.3 mg/L for Zn, 0.553-0.770 mg/L for Cd, and 1.17-2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines.Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739-4.15 × 103, 1.81 × 103-5.00 × 103, 118-1.26 × 103, 8.14-57.7, and 1.23 × 103-6.99 × 103 mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4-17.9 mg/L for Cu, 21.1-29.3 mg/L for Zn, 0.553-0.770 mg/L for Cd, and 1.17-2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines.
Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739–4.15 × 10³, 1.81 × 10³–5.00 × 10³, 118–1.26 × 10³, 8.14–57.7, and 1.23 × 10³–6.99 × 10³ mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4–17.9 mg/L for Cu, 21.1–29.3 mg/L for Zn, 0.553–0.770 mg/L for Cd, and 1.17–2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines.
Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long been overlooked. This study investigated the pollution of surface soils in an area surrounding a recently abandoned small-scale polymetallic mining district in Guangdong province of south China. A total of 13 tailing samples, 145 surface soil samples, and 29 water samples were collected, and the concentrations of major heavy metals, including Cr, Mn, Co, Ni, Cu, Zn, As, Cd, Pb, and Se, were determined. The results show that the tailings contained high levels of heavy metals, with Cu, Zn, As, Cd, and Pb occurring in the ranges of 739–4.15 × 103, 1.81 × 103–5.00 × 103, 118–1.26 × 103, 8.14–57.7, and 1.23 × 103–6.99 × 103 mg/kg, respectively. Heavy metals also occurred at high concentrations in the mine drainages (15.4–17.9 mg/L for Cu, 21.1–29.3 mg/L for Zn, 0.553–0.770 mg/L for Cd, and 1.17–2.57 mg/L for Pb), particularly those with pH below 3. The mean contents of Cu, Zn, As, Cd, and Pb in the surface soils of local farmlands were up to 7 times higher than the corresponding background values, and results of multivariate statistical analysis clearly indicate that Cu, Zn, Cd, and Pb were largely contributed by the mining activities. The surface soils from farmlands surrounding the mining district were moderately to seriously polluted, while the potential ecological risk of heavy metal pollution was extremely high. It was estimated that the input fluxes from the mining district to the surrounding farmlands were approximately 17.1, 59.2, 0.311, and 93.8 kg/ha/yr for Cu, Zn, Cd, and Pb, respectively, which probably occurred through transport of fine tailings by wind and runoff, and mine drainage as well. These findings indicate the significant need for proper containment of the mine tailings at small-scale metal ore mines. [Display omitted] •Heavy metal pollution in a small-scale metal ore mining area was investigated.•Pollution generally decreased with increasing distance from the mining district.•Cu, Zn, Cd, and Pb in local farmland soils came primarily from the mining activities.•Heavy metal pollution of local farmland soils posed high potential ecological risk.•Significant attention needs to be paid to the dumped tailings of small-scale mines.
Author Sun, Zehang
Xie, Xiande
Hu, Yuanan
Cheng, Hefa
Wang, Ping
Author_xml – sequence: 1
  givenname: Zehang
  surname: Sun
  fullname: Sun, Zehang
  organization: State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
– sequence: 2
  givenname: Xiande
  surname: Xie
  fullname: Xie, Xiande
  organization: MOE Key Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
– sequence: 3
  givenname: Ping
  surname: Wang
  fullname: Wang, Ping
  organization: MOE Key Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
– sequence: 4
  givenname: Yuanan
  surname: Hu
  fullname: Hu, Yuanan
  organization: MOE Laboratory of Groundwater Circulation and Evolution, School of Water Resources and Environment, China University of Geosciences (Beijing), Beijing 100083, China
– sequence: 5
  givenname: Hefa
  orcidid: 0000-0003-4911-6971
  surname: Cheng
  fullname: Cheng, Hefa
  email: hefac@umich.edu
  organization: MOE Key Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/29787905$$D View this record in MEDLINE/PubMed
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Keywords Mine tailings
Water pollution
Small-scale mining activities
Soil pollution
Heavy metals
Language English
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  article-title: Geochemical fractions of chromium, copper, and zinc and their vertical distribution in floodplain soil profiles along the Central Elbe River, Germany
  publication-title: Geoderma
  doi: 10.1016/j.geoderma.2013.10.012
– volume: 468–469
  start-page: 843
  year: 2014
  ident: 10.1016/j.scitotenv.2018.05.176_bb0160
  article-title: A review of soil heavy metal pollution from mines in China: pollution and health risk assessment
  publication-title: Sci. Total Environ.
  doi: 10.1016/j.scitotenv.2013.08.090
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Snippet Although metal ore mining activities are well known as an important source of heavy metals, soil pollution caused by small-scale mining activities has long...
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SubjectTerms agricultural land
arsenic
cadmium
case studies
China
chromium
cobalt
copper
drainage
Environmental Monitoring
Heavy metals
lead
manganese
Metals, Heavy - analysis
Mine tailings
Mining
multivariate analysis
nickel
risk
runoff
Small-scale mining activities
Soil
Soil Pollutants - analysis
Soil pollution
soil sampling
Water pollution
wind
zinc
Title Heavy metal pollution caused by small-scale metal ore mining activities: A case study from a polymetallic mine in South China
URI https://dx.doi.org/10.1016/j.scitotenv.2018.05.176
https://www.ncbi.nlm.nih.gov/pubmed/29787905
https://www.proquest.com/docview/2043183259
https://www.proquest.com/docview/2084070429
Volume 639
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