Principles of Water Electrolysis and Recent Progress in Cobalt‐, Nickel‐, and Iron‐Based Oxides for the Oxygen Evolution Reaction

Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large‐scale production of green hydrogen. A broad ra...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 61; H. 1; S. e202103824 - n/a
Hauptverfasser:	Yu, Mingquan, Budiyanto, Eko, Tüysüz, Harun
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 03.01.2022 John Wiley and Sons Inc
Ausgabe:	International ed. in English
Schlagworte:	Catalysts Circular economy Cobalt Crystal structure Electrocatalysts Electrolysis Electron spin Green hydrogen Heavy metals Hydrogen Hydrogen production Iron Nickel Noble metals Oxygen oxygen evolution reaction Oxygen evolution reactions Principles Review Reviews water splitting nickel oxygen evolution reaction iron cobalt water splitting
ISSN:	1433-7851, 1521-3773, 1521-3773
Online-Zugang:	Volltext
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Abstract	Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large‐scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half‐reaction. Co‐, Ni‐, and Fe‐based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co‐, Ni‐, and Fe‐based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis. This Review describes the basic principles of water electrolysis, key aspects of the oxygen evolution reaction (OER), and significant criteria for the development of new catalysts. Recent advances in catalysts based on Co, Ni, and Fe oxides are described, and a brief perspective is given on green hydrogen production and the challenges of water electrolysis.
AbstractList	Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large‐scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half‐reaction. Co‐, Ni‐, and Fe‐based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co‐, Ni‐, and Fe‐based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis. This Review describes the basic principles of water electrolysis, key aspects of the oxygen evolution reaction (OER), and significant criteria for the development of new catalysts. Recent advances in catalysts based on Co, Ni, and Fe oxides are described, and a brief perspective is given on green hydrogen production and the challenges of water electrolysis. Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large‐scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half‐reaction. Co‐, Ni‐, and Fe‐based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co‐, Ni‐, and Fe‐based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis. Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large-scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half-reaction. Co-, Ni-, and Fe-based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co-, Ni-, and Fe-based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis.Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large-scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half-reaction. Co-, Ni-, and Fe-based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co-, Ni-, and Fe-based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis. Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of oxygen evolution reaction (OER) electrocatalysts are the main bottlenecks of the process for large‐scale production of green hydrogen. A broad range of OER electrocatalysts have been explored to decrease the overpotential and boost the kinetics of this sluggish half‐reaction. Co‐, Ni‐, and Fe‐based catalysts have been considered to be potential candidates to replace noble metals due to their tunable 3d electron configuration and spin state, versatility in terms of crystal and electronic structures, as well as abundance in nature. This Review provides some basic principles of water electrolysis, key aspects of OER, and significant criteria for the development of the catalysts. It provides also some insights on recent advances of Co‐, Ni‐, and Fe‐based oxides and a brief perspective on green hydrogen production and the challenges of water electrolysis. This Review describes the basic principles of water electrolysis, key aspects of the oxygen evolution reaction (OER), and significant criteria for the development of new catalysts. Recent advances in catalysts based on Co, Ni, and Fe oxides are described, and a brief perspective is given on green hydrogen production and the challenges of water electrolysis.
Author	Budiyanto, Eko Yu, Mingquan Tüysüz, Harun
AuthorAffiliation	1 Department of Heterogeneous Catalysis Max-Planck-Institute für Kohlenforschung Kaiser-Wilhelm-Platz 1 45470 Mülheim an der Ruhr Germany
AuthorAffiliation_xml	– name: 1 Department of Heterogeneous Catalysis Max-Planck-Institute für Kohlenforschung Kaiser-Wilhelm-Platz 1 45470 Mülheim an der Ruhr Germany
Author_xml	– sequence: 1 givenname: Mingquan surname: Yu fullname: Yu, Mingquan organization: Max-Planck-Institute für Kohlenforschung – sequence: 2 givenname: Eko orcidid: 0000-0001-6184-8863 surname: Budiyanto fullname: Budiyanto, Eko organization: Max-Planck-Institute für Kohlenforschung – sequence: 3 givenname: Harun orcidid: 0000-0001-8552-7028 surname: Tüysüz fullname: Tüysüz, Harun email: tueysuez@kofo.mpg.de organization: Max-Planck-Institute für Kohlenforschung
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/34138511$$D View this record in MEDLINE/PubMed
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Snippet	Water electrolysis that results in green hydrogen is the key process towards a circular economy. The supply of sustainable electricity and availability of...
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SubjectTerms	Catalysts Circular economy Cobalt Crystal structure Electrocatalysts Electrolysis Electron spin Green hydrogen Heavy metals Hydrogen Hydrogen production Iron Nickel Noble metals Oxygen oxygen evolution reaction Oxygen evolution reactions Principles Review Reviews water splitting
Title	Principles of Water Electrolysis and Recent Progress in Cobalt‐, Nickel‐, and Iron‐Based Oxides for the Oxygen Evolution Reaction
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