Three individually addressable spin qubits in a single molecule

An asymmetric bis-phenol-β-diketone (H L) has been designed as a ligand programmed to promote the assembly of a molecular arrangement composed of three magnetically exchanged [NiCu] pairs, each exhibiting an = 1/2 spin. The latter are shown by EPR and magnetometry to be good qubit realizations and n...

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Bibliographic Details
Published in:	Chemical communications (Cambridge, England) Vol. 58; no. 54; p. 7530
Main Authors:	Borilovic, Ivana, Roubeau, Olivier, Le Guennic, Boris, van Slageren, Joris, Lenz, Samuel, Teat, Simon J, Aromí, Guillem
Format:	Journal Article
Language:	English
Published:	England 05.07.2022
ISSN:	1364-548X, 1364-548X
Online Access:	Get more information
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Summary:	An asymmetric bis-phenol-β-diketone (H L) has been designed as a ligand programmed to promote the assembly of a molecular arrangement composed of three magnetically exchanged [NiCu] pairs, each exhibiting an = 1/2 spin. The latter are shown by EPR and magnetometry to be good qubit realizations and non-equivalent within the molecule in the solid state, as required for conditional quantum gates.
Bibliography:	ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23
ISSN:	1364-548X 1364-548X
DOI:	10.1039/d2cc02495k