Role of Spin-Orbit Coupling and Hybridization Effects in the Electronic Structure of Ultrathin Bi Films

The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and first-principles calculations. In contrast with the semimetallic nature of bulk Bi, both the experiment and theory demonstrate the metallic...

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Vydané v:Physical review letters Ročník 97; číslo 14; s. 146803
Hlavní autori: Hirahara, T., Nagao, T., Matsuda, I., Bihlmayer, G., Chulkov, E. V., Koroteev, Yu. M., Echenique, P. M., Saito, M., Hasegawa, S.
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: United States 06.10.2006
ISSN:0031-9007, 1079-7114
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Abstract The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and first-principles calculations. In contrast with the semimetallic nature of bulk Bi, both the experiment and theory demonstrate the metallic character of the films with the Fermi surface formed by spin-orbit-split surface states (SSs) showing little thickness dependence. Below the Fermi level, we clearly detected quantum well states (QWSs) at the M point, which were surprisingly found to be non-spin-orbit split; the films are "electronically symmetric" despite the obvious structural nonequivalence of the top and bottom interfaces. We found that the SSs hybridize with the QWSs near M and lose their spin-orbit-split character.
AbstractList The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and first-principles calculations. In contrast with the semimetallic nature of bulk Bi, both the experiment and theory demonstrate the metallic character of the films with the Fermi surface formed by spin-orbit-split surface states (SSs) showing little thickness dependence. Below the Fermi level, we clearly detected quantum well states (QWSs) at the M point, which were surprisingly found to be non-spin-orbit split; the films are "electronically symmetric" despite the obvious structural nonequivalence of the top and bottom interfaces. We found that the SSs hybridize with the QWSs near M and lose their spin-orbit-split character.The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and first-principles calculations. In contrast with the semimetallic nature of bulk Bi, both the experiment and theory demonstrate the metallic character of the films with the Fermi surface formed by spin-orbit-split surface states (SSs) showing little thickness dependence. Below the Fermi level, we clearly detected quantum well states (QWSs) at the M point, which were surprisingly found to be non-spin-orbit split; the films are "electronically symmetric" despite the obvious structural nonequivalence of the top and bottom interfaces. We found that the SSs hybridize with the QWSs near M and lose their spin-orbit-split character.
The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and first-principles calculations. In contrast with the semimetallic nature of bulk Bi, both the experiment and theory demonstrate the metallic character of the films with the Fermi surface formed by spin-orbit-split surface states (SSs) showing little thickness dependence. Below the Fermi level, we clearly detected quantum well states (QWSs) at the M point, which were surprisingly found to be non-spin-orbit split; the films are "electronically symmetric" despite the obvious structural nonequivalence of the top and bottom interfaces. We found that the SSs hybridize with the QWSs near M and lose their spin-orbit-split character.
ArticleNumber 146803
Author Hasegawa, S.
Nagao, T.
Hirahara, T.
Bihlmayer, G.
Koroteev, Yu. M.
Matsuda, I.
Saito, M.
Chulkov, E. V.
Echenique, P. M.
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  surname: Nagao
  fullname: Nagao, T.
– sequence: 3
  givenname: I.
  surname: Matsuda
  fullname: Matsuda, I.
– sequence: 4
  givenname: G.
  surname: Bihlmayer
  fullname: Bihlmayer, G.
– sequence: 5
  givenname: E. V.
  surname: Chulkov
  fullname: Chulkov, E. V.
– sequence: 6
  givenname: Yu. M.
  surname: Koroteev
  fullname: Koroteev, Yu. M.
– sequence: 7
  givenname: P. M.
  surname: Echenique
  fullname: Echenique, P. M.
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  surname: Saito
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  surname: Hasegawa
  fullname: Hasegawa, S.
BackLink https://www.ncbi.nlm.nih.gov/pubmed/17155281$$D View this record in MEDLINE/PubMed
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Snippet The electronic structure of Bi(001) ultrathin films (thickness > or =7 bilayers) on Si(111)-7x7 was studied by angle-resolved photoemission spectroscopy and...
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Title Role of Spin-Orbit Coupling and Hybridization Effects in the Electronic Structure of Ultrathin Bi Films
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