Using Multi-Platform Satellite Observations to Study the Atmospheric Evolution of Brown Carbon in Siberian Biomass Burning Plumes

A bulk of evidence from in situ observations and lab experiments suggests that brown carbon (light-absorbing organic compounds in particles) can provide a significant yet highly variable contribution to the overall light absorption by aerosol particles from biomass burning (BB). Partly stemming from...

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Published in:	Remote sensing (Basel, Switzerland) Vol. 14; no. 11; p. 2625
Main Authors:	Konovalov, Igor B., Golovushkin, Nikolai A., Beekmann, Matthias, Turquety, Solène
Format:	Journal Article
Language:	English
Published:	Basel MDPI AG 31.05.2022 MDPI
Subjects:	Absorption aerosol absorption Aerosols Aircraft Atmospheric aerosols Atmospheric evolution Atmospheric models Biomass Biomass burning biomass burning aerosol Black carbon brown carbon Burning Carbon Climate models Daylight Electromagnetic absorption Environmental Sciences Evolution Feasibility studies Forest & brush fires Knowledge Light Mie scattering Monitoring instruments Monte Carlo simulation Optical properties organic aerosol Organic compounds Physics Plumes Refractivity Regions Remote sensing Satellite instruments Satellite observation satellite observations of aerosol Satellites Siberian wildfires Smoke Spectroradiometers Statistics Wildfires South America Arctic region Siberia Russia satellite observations of aerosol Siberian wildfires organic aerosol aerosol absorption aerosol atmospheric aging biomass burning aerosol MODIS MISR
ISSN:	2072-4292, 2072-4292
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Abstract	A bulk of evidence from in situ observations and lab experiments suggests that brown carbon (light-absorbing organic compounds in particles) can provide a significant yet highly variable contribution to the overall light absorption by aerosol particles from biomass burning (BB). Partly stemming from the complexity of the atmospheric evolution of organic aerosol (OA), the variability in brown carbon (BrC) absorption makes it difficult to partition the radiative effects of BrC and black carbon (BC) in atmospheric and climate models; as such, there are calls for satellite-based methods that could provide a statistical characterization of BrC absorption and its evolution in different regions of the world, especially in remote BB regions, such as Siberia. This study examined the feasibility of the statistical characterization of the evolution of BrC absorption and related parameters of BB aerosol in smoke plumes from intense wildfires in Siberia through the analysis of a combination of data from three satellite instruments: OMI (Ozone Monitoring Instrument), MISR (Multi-Angle Imaging SpectroRadiometer), and MODIS (Moderate Resolution Imaging Spectroradiometer). Using a Monte Carlo method, which related the satellite retrievals of the absorption and extinction aerosol optical depths to Mie theory calculations of the optical properties of BB aerosol, we found that the BrC absorption, as well as the imaginary refractive index for the OA, decreased significantly in Siberian BB smoke plumes during about 30 h of the daylight evolution, nevertheless remaining considerable until at least 70 h of the daylight evolution. Overall, the study indicated that the analysis of multi-platform satellite observations of BB plumes can provide useful insights into the atmospheric evolution of BrC absorption and the partitioning of BrC and BC contributions to the total light absorption by BB aerosol.
AbstractList	A bulk of evidence from in situ observations and lab experiments suggests that brown carbon (light-absorbing organic compounds in particles) can provide a significant yet highly variable contribution to the overall light absorption by aerosol particles from biomass burning (BB). Partly stemming from the complexity of the atmospheric evolution of organic aerosol (OA), the variability in brown carbon (BrC) absorption makes it difficult to partition the radiative effects of BrC and black carbon (BC) in atmospheric and climate models; as such, there are calls for satellite-based methods that could provide a statistical characterization of BrC absorption and its evolution in different regions of the world, especially in remote BB regions, such as Siberia. This study examined the feasibility of the statistical characterization of the evolution of BrC absorption and related parameters of BB aerosol in smoke plumes from intense wildfires in Siberia through the analysis of a combination of data from three satellite instruments: OMI (Ozone Monitoring Instrument), MISR (Multi-Angle Imaging SpectroRadiometer), and MODIS (Moderate Resolution Imaging Spectroradiometer). Using a Monte Carlo method, which related the satellite retrievals of the absorption and extinction aerosol optical depths to Mie theory calculations of the optical properties of BB aerosol, we found that the BrC absorption, as well as the imaginary refractive index for the OA, decreased significantly in Siberian BB smoke plumes during about 30 h of the daylight evolution, nevertheless remaining considerable until at least 70 h of the daylight evolution. Overall, the study indicated that the analysis of multi-platform satellite observations of BB plumes can provide useful insights into the atmospheric evolution of BrC absorption and the partitioning of BrC and BC contributions to the total light absorption by BB aerosol.
Author	Golovushkin, Nikolai A. Konovalov, Igor B. Beekmann, Matthias Turquety, Solène
Author_xml	– sequence: 1 givenname: Igor B. orcidid: 0000-0002-0716-4273 surname: Konovalov fullname: Konovalov, Igor B. – sequence: 2 givenname: Nikolai A. surname: Golovushkin fullname: Golovushkin, Nikolai A. – sequence: 3 givenname: Matthias surname: Beekmann fullname: Beekmann, Matthias – sequence: 4 givenname: Solène surname: Turquety fullname: Turquety, Solène
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Copyright	2022 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. Distributed under a Creative Commons Attribution 4.0 International License
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Snippet	A bulk of evidence from in situ observations and lab experiments suggests that brown carbon (light-absorbing organic compounds in particles) can provide a...
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SubjectTerms	Absorption aerosol absorption Aerosols Aircraft Atmospheric aerosols Atmospheric evolution Atmospheric models Biomass Biomass burning biomass burning aerosol Black carbon brown carbon Burning Carbon Climate models Daylight Electromagnetic absorption Environmental Sciences Evolution Feasibility studies Forest & brush fires Knowledge Light Mie scattering Monitoring instruments Monte Carlo simulation Optical properties organic aerosol Organic compounds Physics Plumes Refractivity Regions Remote sensing Satellite instruments Satellite observation satellite observations of aerosol Satellites Siberian wildfires Smoke Spectroradiometers Statistics Wildfires
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Title	Using Multi-Platform Satellite Observations to Study the Atmospheric Evolution of Brown Carbon in Siberian Biomass Burning Plumes
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